Retrieving plasmonic near-field information: A quantum-mechanical model for streaking photoelectron spectroscopy of gold nanospheres

Li, Jianxiong; Saydanzad, Erfan; Thumm, Uwe

doi:10.1103/physreva.94.051401

Title: Retrieving plasmonic near-field information: A quantum-mechanical model for streaking photoelectron spectroscopy of gold nanospheres

Journal Article · Mon Nov 14 00:00:00 EST 2016 · Physical Review A

DOI:https://doi.org/10.1103/physreva.94.051401· OSTI ID:1535713

Li, Jianxiong ^[1]; Saydanzad, Erfan ^[1]; Thumm, Uwe ^[1]

Kansas State Univ., Manhattan, KS (United States)

Streaked photoemission from nanostructures is characterized by size- and material-dependent nanometer-scale variations of the induced nanoplasmonic response to the electronic field of the streaking pulse and thus holds promise of allowing photoelectron imaging with both subfemtosecond temporal and nanometer spatial resolution. In order to scrutinize the driven collective electronic dynamics in 10–200-nm-diameter gold nanospheres, we calculated the plasmonic field induced by streaking pulses in the infrared and visible spectral range and developed a quantum-mechanical model for streaked photoemission by extreme ultraviolet pulses. Overall, our simulated photoelectron spectra reveal a significant amplitude enhancement and phase shift of the photoelectron streaking trace relative to calculations that exclude the induced plasmonic field. Both are most pronounced for streaking pulses tuned to the plasmon frequency and retrace the plasmonic electromagnetic field enhancement and phase shift near the nanosphere surface.

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Research Organization:: Kansas State Univ., Manhattan, KS (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division; National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: FG02-86ER13491; PHY 1464417

OSTI ID:: 1535713

Alternate ID(s):: OSTI ID: 1332022

Journal Information:: Physical Review A, Vol. 94, Issue 5; ISSN 2469-9926

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 1 work

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Attosecond chronoscopy of electron scattering in dielectric nanoparticles Seiffert, L.; Liu, Q.; Zherebtsov, S. Nature Physics, Vol. 13, Issue 8 https://doi.org/10.1038/nphys4129	journal	May 2017
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Semiclassical approach for solving the time-dependent Schrödinger equation in spatially inhomogeneous electromagnetic pulses Li, Jianxiong; Thumm, Uwe Physical Review A, Vol. 101, Issue 1 https://doi.org/10.1103/physreva.101.013411	journal	January 2020
Attosecond chronoscopy of electron scattering in dielectric nanoparticles Seiffert, L.; Liu, Q.; Zherebtsov, S. Deutsches Elektronen-Synchrotron, DESY, Hamburg https://doi.org/10.3204/pubdb-2017-10449	text	January 2017

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