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Title: “Wiring” Fe-N x -Embedded Porous Carbon Framework onto 1D Nanotubes for Efficient Oxygen Reduction Reaction in Alkaline and Acidic Media

Abstract

Not provided.

Authors:
 [1];  [1];  [1]
  1. Materials Science and Engineering Program & Texas Materials Institute, The University of Texas at Austin, Austin TX 78712 USA
Publication Date:
Research Org.:
Univ. of Texas, Austin, TX (United States)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
1533036
DOE Contract Number:  
SC0005397
Resource Type:
Journal Article
Journal Name:
Advanced Materials
Additional Journal Information:
Journal Volume: 29; Journal Issue: 26; Journal ID: ISSN 0935-9648
Publisher:
Wiley
Country of Publication:
United States
Language:
English
Subject:
Chemistry; Science & Technology - Other Topics; Materials Science; Physics

Citation Formats

Ahn, Sung Hoon, Yu, Xingwen, and Manthiram, Arumugam. “Wiring” Fe-N x -Embedded Porous Carbon Framework onto 1D Nanotubes for Efficient Oxygen Reduction Reaction in Alkaline and Acidic Media. United States: N. p., 2017. Web. doi:10.1002/adma.201606534.
Ahn, Sung Hoon, Yu, Xingwen, & Manthiram, Arumugam. “Wiring” Fe-N x -Embedded Porous Carbon Framework onto 1D Nanotubes for Efficient Oxygen Reduction Reaction in Alkaline and Acidic Media. United States. doi:10.1002/adma.201606534.
Ahn, Sung Hoon, Yu, Xingwen, and Manthiram, Arumugam. Mon . "“Wiring” Fe-N x -Embedded Porous Carbon Framework onto 1D Nanotubes for Efficient Oxygen Reduction Reaction in Alkaline and Acidic Media". United States. doi:10.1002/adma.201606534.
@article{osti_1533036,
title = {“Wiring” Fe-N x -Embedded Porous Carbon Framework onto 1D Nanotubes for Efficient Oxygen Reduction Reaction in Alkaline and Acidic Media},
author = {Ahn, Sung Hoon and Yu, Xingwen and Manthiram, Arumugam},
abstractNote = {Not provided.},
doi = {10.1002/adma.201606534},
journal = {Advanced Materials},
issn = {0935-9648},
number = 26,
volume = 29,
place = {United States},
year = {2017},
month = {4}
}

Works referenced in this record:

Design principles for oxygen-reduction activity on perovskite oxide catalysts for fuel cells and metal–air batteries
journal, June 2011

  • Suntivich, Jin; Gasteiger, Hubert A.; Yabuuchi, Naoaki
  • Nature Chemistry, Vol. 3, Issue 7, p. 546-550
  • DOI: 10.1038/nchem.1069

Metal–air batteries: from oxygen reduction electrochemistry to cathode catalysts
journal, January 2012

  • Cheng, Fangyi; Chen, Jun
  • Chemical Society Reviews, Vol. 41, Issue 6, p. 2172-2192
  • DOI: 10.1039/c1cs15228a

Non-precious Co3O4 nano-rod electrocatalyst for oxygenreduction reaction in anion-exchange membranefuelcells
journal, January 2012

  • Xu, Jianbo; Gao, Ping; Zhao, T. S.
  • Energy Environ. Sci., Vol. 5, Issue 1
  • DOI: 10.1039/C1EE01431E

Co3O4 nanocrystals on graphene as a synergistic catalyst for oxygen reduction reaction
journal, August 2011

  • Liang, Yongye; Li, Yanguang; Wang, Hailiang
  • Nature Materials, Vol. 10, Issue 10, p. 780-786
  • DOI: 10.1038/nmat3087

Optimizing nanoparticle perovskite for bifunctional oxygen electrocatalysis
journal, January 2016

  • Jung, Jae-Il; Risch, Marcel; Park, Seungkyu
  • Energy & Environmental Science, Vol. 9, Issue 1
  • DOI: 10.1039/C5EE03124A

Iron-Based Catalysts with Improved Oxygen Reduction Activity in Polymer Electrolyte Fuel Cells
journal, April 2009

  • Lefèvre, Michel; Proietti, Eric; Jaouen, Frédéric
  • Science, Vol. 324, Issue 5923, p. 71-74
  • DOI: 10.1126/science.1170051

Rapid room-temperature synthesis of nanocrystalline spinels as oxygen reduction and evolution electrocatalysts
journal, December 2010

  • Cheng, Fangyi; Shen, Jian; Peng, Bo
  • Nature Chemistry, Vol. 3, Issue 1
  • DOI: 10.1038/nchem.931

Sulfur-Doped Graphene Derived from Cycled Lithium-Sulfur Batteries as a Metal-Free Electrocatalyst for the Oxygen Reduction Reaction
journal, December 2014

  • Ma, Zhaoling; Dou, Shuo; Shen, Anli
  • Angewandte Chemie International Edition, Vol. 54, Issue 6
  • DOI: 10.1002/anie.201410258

Controlling the Active Sites of Sulfur-Doped Carbon Nanotube-Graphene Nanolobes for Highly Efficient Oxygen Evolution and Reduction Catalysis
journal, December 2015

  • El-Sawy, Abdelhamid M.; Mosa, Islam M.; Su, Dong
  • Advanced Energy Materials, Vol. 6, Issue 5
  • DOI: 10.1002/aenm.201501966

Fe–P: A New Class of Electroactive Catalyst for Oxygen Reduction Reaction
journal, February 2015

  • Singh, Kiran Pal; Bae, Eun Jin; Yu, Jong-Sung
  • Journal of the American Chemical Society, Vol. 137, Issue 9
  • DOI: 10.1021/ja511759u

A metal-free bifunctional electrocatalyst for oxygen reduction and oxygen evolution reactions
journal, April 2015

  • Zhang, Jintao; Zhao, Zhenghang; Xia, Zhenhai
  • Nature Nanotechnology, Vol. 10, Issue 5
  • DOI: 10.1038/nnano.2015.48

Can Boron and Nitrogen Co-doping Improve Oxygen Reduction Reaction Activity of Carbon Nanotubes?
journal, January 2013

  • Zhao, Yu; Yang, Lijun; Chen, Sheng
  • Journal of the American Chemical Society, Vol. 135, Issue 4
  • DOI: 10.1021/ja310566z

Boron-Doped Carbon Nanotubes as Metal-Free Electrocatalysts for the Oxygen Reduction Reaction
journal, June 2011


Nitrogen-Doped Carbon Nanotube Arrays with High Electrocatalytic Activity for Oxygen Reduction
journal, February 2009


Metal–organic-framework-engaged formation of Co nanoparticle-embedded carbon@Co 9 S 8 double-shelled nanocages for efficient oxygen reduction
journal, January 2016

  • Hu, Han; Han, Lei; Yu, Mengzhou
  • Energy & Environmental Science, Vol. 9, Issue 1
  • DOI: 10.1039/C5EE02903A

High-Performance Electrocatalysts for Oxygen Reduction Derived from Polyaniline, Iron, and Cobalt
journal, April 2011


High-Rate Oxygen Electroreduction over Graphitic-N Species Exposed on 3D Hierarchically Porous Nitrogen-Doped Carbons
journal, July 2014

  • He, Wenhui; Jiang, Chunhuan; Wang, Jiabo
  • Angewandte Chemie International Edition, Vol. 53, Issue 36
  • DOI: 10.1002/anie.201404333

Opening of Bottleneck Pores for the Improvement of Nitrogen Doped Carbon Electrocatalysts
journal, January 2016

  • Pampel, Jonas; Fellinger, Tim-Patrick
  • Advanced Energy Materials, Vol. 6, Issue 8
  • DOI: 10.1002/aenm.201502389

ZIF-derived in situ nitrogen-doped porous carbons as efficient metal-free electrocatalysts for oxygen reduction reaction
journal, January 2014

  • Zhang, Peng; Sun, Fang; Xiang, Zhonghua
  • Energy Environ. Sci., Vol. 7, Issue 1
  • DOI: 10.1039/C3EE42799D

From Bimetallic Metal-Organic Framework to Porous Carbon: High Surface Area and Multicomponent Active Dopants for Excellent Electrocatalysis
journal, July 2015

  • Chen, Yu-Zhen; Wang, Chengming; Wu, Zhen-Yu
  • Advanced Materials, Vol. 27, Issue 34
  • DOI: 10.1002/adma.201502315

Nanowire-Directed Templating Synthesis of Metal–Organic Framework Nanofibers and Their Derived Porous Doped Carbon Nanofibers for Enhanced Electrocatalysis
journal, October 2014

  • Zhang, Wang; Wu, Zhen-Yu; Jiang, Hai-Long
  • Journal of the American Chemical Society, Vol. 136, Issue 41
  • DOI: 10.1021/ja5084128

Nitrogen-Doped Nanoporous Carbon/Graphene Nano-Sandwiches: Synthesis and Application for Efficient Oxygen Reduction
journal, August 2015

  • Wei, Jing; Hu, Yaoxin; Liang, Yan
  • Advanced Functional Materials, Vol. 25, Issue 36
  • DOI: 10.1002/adfm.201502311

Directed Growth of Metal-Organic Frameworks and Their Derived Carbon-Based Network for Efficient Electrocatalytic Oxygen Reduction
journal, January 2016


Identification of catalytic sites for oxygen reduction in iron- and nitrogen-doped graphene materials
journal, August 2015

  • Zitolo, Andrea; Goellner, Vincent; Armel, Vanessa
  • Nature Materials, Vol. 14, Issue 9
  • DOI: 10.1038/nmat4367

A Versatile Iron-Tannin-Framework Ink Coating Strategy to Fabricate Biomass-Derived Iron Carbide/Fe-N-Carbon Catalysts for Efficient Oxygen Reduction
journal, December 2015

  • Wei, Jing; Liang, Yan; Hu, Yaoxin
  • Angewandte Chemie International Edition, Vol. 55, Issue 4
  • DOI: 10.1002/anie.201509024

Iron Carbide Nanoparticles Encapsulated in Mesoporous Fe-N-Doped Carbon Nanofibers for Efficient Electrocatalysis
journal, May 2015

  • Wu, Zhen-Yu; Xu, Xing-Xing; Hu, Bi-Cheng
  • Angewandte Chemie International Edition, Vol. 54, Issue 28
  • DOI: 10.1002/anie.201502173

Highly active oxygen reduction non-platinum group metal electrocatalyst without direct metal–nitrogen coordination
journal, June 2015

  • Strickland, Kara; Miner, Elise; Jia, Qingying
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms8343

Iron-based cathode catalyst with enhanced power density in polymer electrolyte membrane fuel cells
journal, August 2011

  • Proietti, Eric; Jaouen, Frédéric; Lefèvre, Michel
  • Nature Communications, Vol. 2, Issue 1
  • DOI: 10.1038/ncomms1427

Minimizing Operando Demetallation of Fe-N-C Electrocatalysts in Acidic Medium
journal, April 2016

  • Choi, Chang Hyuck; Baldizzone, Claudio; Polymeros, George
  • ACS Catalysis, Vol. 6, Issue 5
  • DOI: 10.1021/acscatal.6b00643

Hierarchical pore-in-pore and wire-in-wire catalysts for rechargeable Zn– and Li–air batteries with ultra-long cycle life and high cell efficiency
journal, January 2015

  • Li, Longjun; Liu, Chao; He, Guang
  • Energy & Environmental Science, Vol. 8, Issue 11
  • DOI: 10.1039/C5EE02616D

Advanced hybrid Li–air batteries with high-performance mesoporous nanocatalysts
journal, January 2014

  • Li, Longjun; Chai, Song-Hai; Dai, Sheng
  • Energy & Environmental Science, Vol. 7, Issue 8
  • DOI: 10.1039/C4EE00814F

Decoupled bifunctional air electrodes for high-performance hybrid lithium-air batteries
journal, October 2014


Controlled Synthesis of Tellurium Nanostructures from Nanotubes to Nanorods and Nanowires and Their Template Applications
journal, March 2011

  • Zhu, Hangtian; Zhang, He; Liang, Jingkui
  • The Journal of Physical Chemistry C, Vol. 115, Issue 14
  • DOI: 10.1021/jp200316y

Density functional theory methods for characterization of porous materials
journal, November 2013

  • Landers, John; Gor, Gennady Yu.; Neimark, Alexander V.
  • Colloids and Surfaces A: Physicochemical and Engineering Aspects, Vol. 437
  • DOI: 10.1016/j.colsurfa.2013.01.007

On the Role of Metals in Nitrogen-Doped Carbon Electrocatalysts for Oxygen Reduction
journal, July 2015

  • Masa, Justus; Xia, Wei; Muhler, Martin
  • Angewandte Chemie International Edition, Vol. 54, Issue 35
  • DOI: 10.1002/anie.201500569

Iron Carbide Nanoparticles Encapsulated in Mesoporous Fe–N-Doped Graphene-Like Carbon Hybrids as Efficient Bifunctional Oxygen Electrocatalysts
journal, September 2015

  • Jiang, Hongliang; Yao, Yifan; Zhu, Yihua
  • ACS Applied Materials & Interfaces, Vol. 7, Issue 38
  • DOI: 10.1021/acsami.5b06708

High Performance Fe- and N- Doped Carbon Catalyst with Graphene Structure for Oxygen Reduction
journal, May 2013

  • Peng, Hongliang; Mo, Zaiyong; Liao, Shijun
  • Scientific Reports, Vol. 3, Issue 1
  • DOI: 10.1038/srep01765

Understanding the High Activity of Fe–N–C Electrocatalysts in Oxygen Reduction: Fe/Fe 3 C Nanoparticles Boost the Activity of Fe–N x
journal, March 2016

  • Jiang, Wen-Jie; Gu, Lin; Li, Li
  • Journal of the American Chemical Society, Vol. 138, Issue 10
  • DOI: 10.1021/jacs.6b00757

Alveoli-Inspired Facile Transport Structure of N-Doped Porous Carbon for Electrochemical Energy Applications
journal, October 2014

  • Chung, Dong Young; Lee, Kyung Jae; Yu, Seung-Ho
  • Advanced Energy Materials, Vol. 5, Issue 3
  • DOI: 10.1002/aenm.201401309

Bamboo-like Carbon Nanotube/Fe 3 C Nanoparticle Hybrids and Their Highly Efficient Catalysis for Oxygen Reduction
journal, January 2015

  • Yang, Wenxiu; Liu, Xiangjian; Yue, Xiaoyu
  • Journal of the American Chemical Society, Vol. 137, Issue 4
  • DOI: 10.1021/ja5129132

Structural and mechanistic basis for the high activity of Fe–N–C catalysts toward oxygen reduction
journal, January 2016

  • Li, Jingkun; Ghoshal, Shraboni; Liang, Wentao
  • Energy & Environmental Science, Vol. 9, Issue 7
  • DOI: 10.1039/C6EE01160H

Correlations between Mass Activity and Physicochemical Properties of Fe/N/C Catalysts for the ORR in PEM Fuel Cell via 57 Fe Mössbauer Spectroscopy and Other Techniques
journal, January 2014

  • Kramm, Ulrike I.; Lefèvre, Michel; Larouche, Nicholas
  • Journal of the American Chemical Society, Vol. 136, Issue 3
  • DOI: 10.1021/ja410076f

Hollow Spheres of Iron Carbide Nanoparticles Encased in Graphitic Layers as Oxygen Reduction Catalysts
journal, February 2014


A dual-metal–organic-framework derived electrocatalyst for oxygen reduction
journal, January 2016

  • Guan, Bu Yuan; Yu, Le; (David) Lou, Xiong Wen
  • Energy & Environmental Science, Vol. 9, Issue 10
  • DOI: 10.1039/C6EE02171A

Degradation by Hydrogen Peroxide of Metal-Nitrogen-Carbon Catalysts for Oxygen Reduction
journal, January 2015

  • Goellner, Vincent; Armel, Vanessa; Zitolo, Andrea
  • Journal of The Electrochemical Society, Vol. 162, Issue 6
  • DOI: 10.1149/2.1091506jes

Active sites of nitrogen-doped carbon materials for oxygen reduction reaction clarified using model catalysts
journal, January 2016


Meso-Structured Platinum Thin Films: Active and Stable Electrocatalysts for the Oxygen Reduction Reaction
journal, April 2012

  • Kibsgaard, Jakob; Gorlin, Yelena; Chen, Zhebo
  • Journal of the American Chemical Society, Vol. 134, Issue 18
  • DOI: 10.1021/ja2120162

Activity benchmarks and requirements for Pt, Pt-alloy, and non-Pt oxygen reduction catalysts for PEMFCs
journal, March 2005

  • Gasteiger, Hubert A.; Kocha, Shyam S.; Sompalli, Bhaskar
  • Applied Catalysis B: Environmental, Vol. 56, Issue 1-2, p. 9-35
  • DOI: 10.1016/j.apcatb.2004.06.021

Synthesis of mesoporous Fe/N/C oxygen reduction catalysts through NaCl crystallite-confined pyrolysis of polyvinylpyrrolidone
journal, January 2016

  • Wang, Wang; Luo, Jin; Chen, Wenhui
  • Journal of Materials Chemistry A, Vol. 4, Issue 33
  • DOI: 10.1039/C6TA05075A

Noble-Metal-Free Fe–N/C Catalyst for Highly Efficient Oxygen Reduction Reaction under Both Alkaline and Acidic Conditions
journal, July 2014

  • Lin, Ling; Zhu, Qing; Xu, An-Wu
  • Journal of the American Chemical Society, Vol. 136, Issue 31
  • DOI: 10.1021/ja504696r

An oxygen reduction electrocatalyst based on carbon nanotube–graphene complexes
journal, May 2012

  • Li, Yanguang; Zhou, Wu; Wang, Hailiang
  • Nature Nanotechnology, Vol. 7, Issue 6
  • DOI: 10.1038/nnano.2012.72

A review of the development of nitrogen-modified carbon-based catalysts for oxygen reduction at USC
journal, January 2011

  • Liu, Gang; Li, Xuguang; Lee, Jong-Won
  • Catalysis Science & Technology, Vol. 1, Issue 2
  • DOI: 10.1039/c0cy00053a

High-Yield Synthesis, Controllable Evolution, and Thermoelectric Properties of Te/Bi2Te3 Heterostructure Nanostrings
journal, February 2015


Water photolysis at 12.3% efficiency via perovskite photovoltaics and Earth-abundant catalysts
journal, September 2014


Long-Life, High-Voltage Acidic Zn-Air Batteries
journal, December 2015