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Title: Imaging Interfacial Electric Fields on Ultrafast Timescales (Final Report)

Technical Report ·
DOI:https://doi.org/10.2172/1525344· OSTI ID:1525344

The goal of this project is to dynamically probe interfacial electric fields on ultrafast timescales and sub-micron length scales. The proposed method could be applied to a variety of heterointerfaces, with particular emphasis on interfaces involving colloidal quantum dots. The primary objective is development of an ultrafast nonlinear optical imaging technique with this capability. A secondary objective is obtaining new insights into excited state charge carrier dynamics in colloidal quantum dot solids and at quantum dot interfaces. Research activities involve validation of the technical approach, construction of the microscope, and synthesis and characterization of materials to be studied using the instrument.

Research Organization:
Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences, and Biosciences Division
DOE Contract Number:
SC0010538
OSTI ID:
1525344
Report Number(s):
DOE-MIT-10538
Country of Publication:
United States
Language:
English

References (10)

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Optimal Bandgap in a 2D Ruddlesden–Popper Perovskite Chalcogenide for Single-Junction Solar Cells journal July 2018
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Inverse Temperature Dependence of Charge Carrier Hopping in Quantum Dot Solids journal June 2018
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