The growth and assembly of organic molecules and inorganic 2D materials on graphene for van der Waals heterostructures

Oyedele, Akinola D.; Rouleau, Christopher M.; Geohegan, David B.; Xiao, Kai

doi:10.1016/j.carbon.2018.02.020

Title: The growth and assembly of organic molecules and inorganic 2D materials on graphene for van der Waals heterostructures

Journal Article · Sat Feb 03 00:00:00 EST 2018 · Carbon

DOI:https://doi.org/10.1016/j.carbon.2018.02.020· OSTI ID:1523762

Oyedele, Akinola D. ^[1];

^[2];

^[3]

Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Univ. of Tennessee, Knoxville, TN (United States)

The unique properties of graphene have made it a promising material for integration in future electronic applications. The idealized surface of graphene, atomically-flat and without dangling bonds, offers the opportunity to understand the assembly of organic and inorganic molecules to form a wide range of ordered architectures and functional graphene-based heterostructures. In this review, we summarize recent progress in the growth of hierarchical nanostructures on graphene. The self-assembly of organic molecules and inorganic two-dimensional (2D) layers on graphene for the construction of various types of heterostructures are highlighted. Van der Waals interactions between the assembled molecules and graphene are shown to allow the formation of highly-ordered structures with preferred molecular orientations and stacking configurations that circumvent the strict lattice-matching requirements in traditional epitaxial growth. Lastly, we briefly discuss representative applications of graphene-based heterostructures in electronic and optoelectronics.

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Research Organization:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1523762

Alternate ID(s):: OSTI ID: 1619904

Journal Information:: Carbon, Vol. 131, Issue C; ISSN 0008-6223

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 21 works

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