Magnetic Field-Suppressed Lithium Dendrite Growth for Stable Lithium-Metal Batteries

Shen, Kang; Wang, Zeng; Bi, Xuanxuan; Ying, Yao; Zhang, Duo; Jin, Chengbin; Hou, Guangya; Cao, Huazhen; Wu, Liankui; Zheng, Guoqu; Tang, Yiping; Tao, Xinyong; Lu, Jun

doi:10.1002/aenm.201900260

Title: Magnetic Field-Suppressed Lithium Dendrite Growth for Stable Lithium-Metal Batteries

Journal Article · Wed Apr 03 00:00:00 EDT 2019 · Advanced Energy Materials

DOI:https://doi.org/10.1002/aenm.201900260· OSTI ID:1523651

Shen, Kang ^[1]; Wang, Zeng ^[1]; Bi, Xuanxuan ^[2]; Ying, Yao ^[1]; Zhang, Duo ^[1]; Jin, Chengbin ^[1]; Hou, Guangya ^[1]; Cao, Huazhen ^[1]; Wu, Liankui ^[1]; Zheng, Guoqu ^[1]; Tang, Yiping ^[1]; Tao, Xinyong ^[1];

^[2]

Zhejiang Univ. of Technology, Hangzhou (China). College of Material Science and Engineering
Argonne National Lab. (ANL), Argonne, IL (United States). Chemical Sciences and Engineering Division

Abstract Lithium metal is the most attractive anode material due to its extremely high specific capacity, minimum potential, and low density. However, uncontrollable growth of lithium dendrite results in severe safety and cycling stability concerns, which hinders the application in next generation secondary batteries. In this paper, a new and facile method imposing a magnetic field to lithium metal anodes is proposed. That is, the lithium ions suffering Lorentz force due to the electromagnetic fields are put into spiral motion causing magnetohydrodynamics (MHD) effect. This MHD effect can effectively promote mass transfer and uniform distribution of lithium ions to suppress the dendrite growth as well as obtain uniform and compact lithium deposition. The results show that the lithium metal electrodes within the magnetic field exhibit excellent cycling and rate performance in a symmetrical battery. Additionally, full batteries using limited lithium metal as anodes and commercial LiFePO ₄ as cathodes show improved performance within the magnetic field. In summary, a new and facile strategy of suppressing lithium dendrites using the MHD effect by imposing a magnetic field is proposed, which may be generalized to other advanced alkali metal batteries.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: National Natural Science Foundation of China (NSFC); USDOE Office of Energy Efficiency and Renewable Energy (EERE), Vehicle Technologies Office (EE-3V); USDOE

Grant/Contract Number:: AC02-06CH11357; DE‐AC02‐06CH11357

OSTI ID:: 1523651

Alternate ID(s):: OSTI ID: 1504790

Journal Information:: Advanced Energy Materials, Vol. 9, Issue 20; ISSN 1614-6832

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 178 works

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Lorentz force
dendrites
lithium metal
magnetic field
magnetohydrodynamics effect

Title: Magnetic Field-Suppressed Lithium Dendrite Growth for Stable Lithium-Metal Batteries

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