Phonon mode links ferroicities in multiferroic [(CH3)2NH2]Mn(HCOO)3

Hughey, Kendall D.; Clune, Amanda J.; Yokosuk, Michael O.; al-Wahish, Amal; O'Neal, Kenneth R.; Fan, Shiyu; Abhyankar, Nandita; Xiang, Hongjun; Li, Zhiqiang; Singleton, John; Dalal, Naresh S.; Musfeldt, Janice L.

doi:10.1103/PhysRevB.96.180305

Title: Phonon mode links ferroicities in multiferroic $[{({CH}_{3})}_{2} {NH}_{2}] {Mn (HCOO)}_{3}$

Journal Article · Wed Nov 22 00:00:00 EST 2017 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.96.180305· OSTI ID:1512737

Hughey, Kendall D. ^[1]; Clune, Amanda J. ^[1]; Yokosuk, Michael O. ^[1]; al-Wahish, Amal ^[1]; O'Neal, Kenneth R. ^[1]; Fan, Shiyu ^[1]; Abhyankar, Nandita ^[2]; Xiang, Hongjun ^[3]; Li, Zhiqiang ^[4];

^[5]; Dalal, Naresh S. ^[6]; Musfeldt, Janice L. ^[1]

Univ. of Tennessee, Knoxville, TN (United States)
Florida State Univ., Tallahassee, FL (United States); National High Magnetic Lab., Tallahassee, FL (United States); ; National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States)
Fudan Univ., Shanghai (China); Collaborative Innovation Center of Advanced Microstructures, Nanjing (China)
National High Magnetic Lab., Tallahassee, FL (United States)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Florida State Univ., Tallahassee, FL (United States); National High Magnetic Lab., Tallahassee, FL (United States)

In this work, we combined magnetoinfrared spectroscopy, magnetization, and lattice dynamics calculations to explore the phase transitions in multiferroic $[{({CH}_{3})}_{2} {NH}_{2}] {Mn (HCOO)}_{3}$ Both the 185 K ferroelectric transition and the magnetically driven transition to the fully saturated state at 15.3 T involve the formate bending mode, direct evidence of a common connection between the two types of ferroicities and for how lattice distortions advance high-temperature magnetoelectric coupling in this system.

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Research Organization:: Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: 89233218CNA000001

OSTI ID:: 1512737

Alternate ID(s):: OSTI ID: 1409874

Report Number(s):: LA-UR-17-22717; PRBMDO

Journal Information:: Physical Review B, Vol. 96, Issue 18; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 13 works

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