Electronic friction in interacting systems

Chen, Feng; Miwa, Kuniyuki; Galperin, Michael

doi:10.1063/1.5095425

Title: Electronic friction in interacting systems

Journal Article · Wed May 01 00:00:00 EDT 2019 · Journal of Chemical Physics

DOI:https://doi.org/10.1063/1.5095425· OSTI ID:1510264

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Univ. of California San Diego, La Jolla, CA (United States)

We consider the effects of strong light-matter interaction on electronic friction in molecular junctions within the generic model of a single molecule nanocavity junction. Results of the Hubbard nonequilibrium Green function (NEGF) simulations are compared with mean-field NEGF and generalized Head-Gordon and Tully (HGT) approaches. Mean-field NEGF is shown to fail qualitatively at strong intrasystem interactions, while accuracy of the generalized HGT results is restricted to situations of well separated intramolecular excitations when bath induced coherences are negligible. Numerical results show effects of bias and cavity mode pumping on electronic friction. Here, we demonstrate nonmonotonic behavior of the friction on the bias and intensity of the pumping field and indicate possibility of engineering friction control in single molecule junctions.

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Research Organization:: Univ. of California, San Diego, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0018201

OSTI ID:: 1510264

Alternate ID(s):: OSTI ID: 1510162

Journal Information:: Journal of Chemical Physics, Vol. 150, Issue 17; ISSN 0021-9606

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 9 works

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Title: Electronic friction in interacting systems

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