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Title: Echo-Enabled Harmonic Generation Studies for the FERMI Free-Electron Laser

Abstract

Studying ultrafast processes on the nanoscale with element specificity requires a powerful femtosecond source of tunable extreme-ultraviolet (XUV) or x-ray radiation, such as a free-electron laser (FEL). Current efforts in FEL development are aimed at improving the wavelength tunability and multicolor operation, which will potentially lead to the development of new characterization techniques offering a higher chemical sensitivity and improved spatial resolution. One of the most promising approaches is the echo-enabled harmonic generation (EEHG), where two external seed lasers are used to precisely control the spectro-temporal properties of the FEL pulse. Here, we study the expected performance of EEHG at the FERMI FEL, using numerical simulations. We show that, by employing the existing FERMI layout with minor modifications, the EEHG scheme will be able to produce gigawatt peak-power pulses at wavelengths as short as 5 nm. We discuss some possible detrimental effects that may affect the performance of EEHG and compare the results to the existing double-stage FEL cascade, currently in operation at FERMI. Finally, our simulations show that, after substantial machine upgrades, EEHG has the potential to deliver coherent multicolor pulses reaching wavelengths as short as 3 nm, enabling x-ray pump-x-ray probe experiments in the water window.

Authors:
 [1];  [1];  [2];  [3];  [1];  [1];  [1]
  1. Elettra-Sincrotrone Trieste, Trieste (Italy)
  2. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  3. Elettra-Sincrotrone Trieste, Trieste (Italy); Univ. of Nova Gorica, Nova Gorica (Slovenia)
Publication Date:
Research Org.:
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1506273
DOE Contract Number:  
AC02-05CH11231
Resource Type:
Journal Article
Journal Name:
Photonics
Additional Journal Information:
Journal Volume: 4; Journal Issue: 4; Journal ID: ISSN 2304-6732
Publisher:
MDPI
Country of Publication:
United States
Language:
English
Subject:
47 OTHER INSTRUMENTATION; free-electron laser; harmonic up-conversion; high-harmonic generation; seeding; x-ray; pump-probe; microbunching instability

Citation Formats

Ribič, Primož Rebernik, Roussel, Eléonore, Penn, Gregory, De Ninno, Giovanni, Giannessi, Luca, Penco, Giuseppe, and Allaria, Enrico. Echo-Enabled Harmonic Generation Studies for the FERMI Free-Electron Laser. United States: N. p., 2017. Web. doi:10.3390/photonics4010019.
Ribič, Primož Rebernik, Roussel, Eléonore, Penn, Gregory, De Ninno, Giovanni, Giannessi, Luca, Penco, Giuseppe, & Allaria, Enrico. Echo-Enabled Harmonic Generation Studies for the FERMI Free-Electron Laser. United States. doi:10.3390/photonics4010019.
Ribič, Primož Rebernik, Roussel, Eléonore, Penn, Gregory, De Ninno, Giovanni, Giannessi, Luca, Penco, Giuseppe, and Allaria, Enrico. Tue . "Echo-Enabled Harmonic Generation Studies for the FERMI Free-Electron Laser". United States. doi:10.3390/photonics4010019. https://www.osti.gov/servlets/purl/1506273.
@article{osti_1506273,
title = {Echo-Enabled Harmonic Generation Studies for the FERMI Free-Electron Laser},
author = {Ribič, Primož Rebernik and Roussel, Eléonore and Penn, Gregory and De Ninno, Giovanni and Giannessi, Luca and Penco, Giuseppe and Allaria, Enrico},
abstractNote = {Studying ultrafast processes on the nanoscale with element specificity requires a powerful femtosecond source of tunable extreme-ultraviolet (XUV) or x-ray radiation, such as a free-electron laser (FEL). Current efforts in FEL development are aimed at improving the wavelength tunability and multicolor operation, which will potentially lead to the development of new characterization techniques offering a higher chemical sensitivity and improved spatial resolution. One of the most promising approaches is the echo-enabled harmonic generation (EEHG), where two external seed lasers are used to precisely control the spectro-temporal properties of the FEL pulse. Here, we study the expected performance of EEHG at the FERMI FEL, using numerical simulations. We show that, by employing the existing FERMI layout with minor modifications, the EEHG scheme will be able to produce gigawatt peak-power pulses at wavelengths as short as 5 nm. We discuss some possible detrimental effects that may affect the performance of EEHG and compare the results to the existing double-stage FEL cascade, currently in operation at FERMI. Finally, our simulations show that, after substantial machine upgrades, EEHG has the potential to deliver coherent multicolor pulses reaching wavelengths as short as 3 nm, enabling x-ray pump-x-ray probe experiments in the water window.},
doi = {10.3390/photonics4010019},
journal = {Photonics},
issn = {2304-6732},
number = 4,
volume = 4,
place = {United States},
year = {2017},
month = {3}
}

Works referenced in this record:

Using the Beam-Echo Effect for Generation of Short-Wavelength Radiation
journal, February 2009


First lasing of an echo-enabled harmonic generation free-electron laser
journal, May 2012


Single mimivirus particles intercepted and imaged with an X-ray laser
journal, February 2011

  • Seibert, M. Marvin; Ekeberg, Tomas; Maia, Filipe R. N. C.
  • Nature, Vol. 470, Issue 7332
  • DOI: 10.1038/nature09748

Injection of harmonics generated in gas in a free-electron laser providing intense and coherent extreme-ultraviolet light
journal, March 2008

  • Lambert, G.; Hara, T.; Garzella, D.
  • Nature Physics, Vol. 4, Issue 4
  • DOI: 10.1038/nphys889

Operation of a free-electron laser from the extreme ultraviolet to the water window
journal, June 2007


A compact X-ray free-electron laser emitting in the sub-ångström region
journal, June 2012


Echo-enabled harmonics up to the 75th order from precisely tailored electron beams
journal, June 2016


Fresh-slice multicolour X-ray free-electron lasers
journal, October 2016

  • Lutman, Alberto A.; Maxwell, Timothy J.; MacArthur, James P.
  • Nature Photonics, Vol. 10, Issue 11
  • DOI: 10.1038/nphoton.2016.201

Generation of Coherent 19- and 38-nm Radiation at a Free-Electron Laser Directly Seeded at 38 nm
journal, September 2013


Two-colour hard X-ray free-electron laser with wide tunability
journal, December 2013

  • Hara, Toru; Inubushi, Yuichi; Katayama, Tetsuo
  • Nature Communications, Vol. 4, Issue 1
  • DOI: 10.1038/ncomms3919

First lasing and operation of an ångstrom-wavelength free-electron laser
journal, August 2010


Generation of Phase-Locked Pulses from a Seeded Free-Electron Laser
journal, January 2016


GENESIS 1.3: a fully 3D time-dependent FEL simulation code
journal, June 1999

  • Reiche, S.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 429, Issue 1-3
  • DOI: 10.1016/S0168-9002(99)00114-X

Microbunching-instability-induced sidebands in a seeded free-electron laser
journal, May 2016


Four-wave mixing experiments with extreme ultraviolet transient gratings
journal, April 2015

  • Bencivenga, F.; Cucini, R.; Capotondi, F.
  • Nature, Vol. 520, Issue 7546
  • DOI: 10.1038/nature14341

Chirped Seeded Free-Electron Lasers: Self-Standing Light Sources for Two-Color Pump-Probe Experiments
journal, February 2013


Generation of Coherent Extreme-Ultraviolet Radiation Carrying Orbital Angular Momentum
journal, May 2014


Two-colour pump–probe experiments with a twin-pulse-seed extreme ultraviolet free-electron laser
journal, September 2013

  • Allaria, E.; Bencivenga, F.; Borghes, R.
  • Nature Communications, Vol. 4, Issue 1
  • DOI: 10.1038/ncomms3476

Demonstration of self-seeding in a hard-X-ray free-electron laser
journal, August 2012


Laser heater commissioning at an externally seeded free-electron laser
journal, December 2014

  • Spampinati, S.; Allaria, E.; Badano, L.
  • Physical Review Special Topics - Accelerators and Beams, Vol. 17, Issue 12
  • DOI: 10.1103/PhysRevSTAB.17.120705

Femtosecond X-ray protein nanocrystallography
journal, February 2011

  • Chapman, Henry N.; Fromme, Petra; Barty, Anton
  • Nature, Vol. 470, Issue 7332, p. 73-77
  • DOI: 10.1038/nature09750

Single-shot spectro-temporal characterization of XUV pulses from a seeded free-electron laser
journal, August 2015

  • De Ninno, Giovanni; Gauthier, David; Mahieu, Benoît
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms9075

Experimental Demonstration of a Soft X-Ray Self-Seeded Free-Electron Laser
journal, February 2015


Two-stage seeded soft-X-ray free-electron laser
journal, October 2013


Longitudinal space charge-driven microbunching instability in the TESLA Test Facility linac
journal, August 2004

  • Saldin, E. L.; Schneidmiller, E. A.; Yurkov, M. V.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 528, Issue 1-2
  • DOI: 10.1016/j.nima.2004.04.067

Collective instabilities and high-gain regime in a free electron laser
journal, July 1984


Status and prospects of x-ray free-electron lasers (X-FELs): a simple presentation
journal, May 2012


Multicolor High-Gain Free-Electron Laser Driven by Seeded Microbunching Instability
journal, November 2015


Highly coherent vacuum ultraviolet radiation at the 15th harmonic with echo-enabled harmonic generation technique
journal, July 2014

  • Hemsing, E.; Dunning, M.; Hast, C.
  • Physical Review Special Topics - Accelerators and Beams, Vol. 17, Issue 7
  • DOI: 10.1103/PhysRevSTAB.17.070702

Review of x-ray free-electron laser theory
journal, March 2007


Coherent control with a short-wavelength free-electron laser
journal, February 2016


Stable, coherent free-electron laser pulses using echo-enabled harmonic generation
journal, November 2014


Highly coherent and stable pulses from the FERMI seeded free-electron laser in the extreme ultraviolet
journal, September 2012


Bunching coefficients in echo-enabled harmonic generation
journal, July 2013


Modeling of the microbunching instability
journal, March 2008


Laser phase errors in seeded free electron lasers
journal, March 2012


Echo-enabled harmonic generation free electron laser
journal, March 2009


Spectrotemporal Shaping of Seeded Free-Electron Laser Pulses
journal, September 2015


Femtosecond diffractive imaging with a soft-X-ray free-electron laser
journal, November 2006

  • Chapman, Henry N.; Barty, Anton; Bogan, Michael J.
  • Nature Physics, Vol. 2, Issue 12
  • DOI: 10.1038/nphys461

High-gain harmonic generation of soft X-rays with the “fresh bunch” technique
journal, July 1997

  • Yu, Li-Hua; Ben-Zvi, Ilan
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 393, Issue 1-3
  • DOI: 10.1016/S0168-9002(97)00435-X

Double-core-hole spectroscopy for chemical analysis with an intense X-ray femtosecond laser
journal, October 2011

  • Berrah, N.; Fang, L.; Murphy, B.
  • Proceedings of the National Academy of Sciences, Vol. 108, Issue 41
  • DOI: 10.1073/pnas.1111380108

Widely tunable two-colour seeded free-electron laser source for resonant-pump resonant-probe magnetic scattering
journal, January 2016

  • Ferrari, Eugenio; Spezzani, Carlo; Fortuna, Franck
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms10343

Start-to-end simulation of self-amplified spontaneous emission free electron lasers from the gun through the undulator
journal, May 2002

  • Borland, M.; Chae, Y. C.; Emma, P.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 483, Issue 1-2
  • DOI: 10.1016/S0168-9002(02)00325-X

Extreme ultraviolet free electron laser seeded with high-order
harmonic of Ti:sapphire laser
journal, December 2010

  • Togashi, Tadashi; Takahashi, Eiji J.; Midorikawa, Katsumi
  • Optics Express, Vol. 19, Issue 1
  • DOI: 10.1364/OE.19.000317

High-intensity double-pulse X-ray free-electron laser
journal, March 2015

  • Marinelli, A.; Ratner, D.; Lutman, A. A.
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms7369

Klystron instability of a relativistic electron beam in a bunch compressor
journal, September 2002

  • Saldin, E. L.; Schneidmiller, E. A.; Yurkov, M. V.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 490, Issue 1-2
  • DOI: 10.1016/S0168-9002(02)00905-1