skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Time- and angle-resolved photoemission spectroscopy of solids in the extreme ultraviolet at 500 kHz repetition rate

Abstract

Time- and angle-resolved photoemission spectroscopy (trARPES) employing a 500 kHz extreme-ultraviolet light source operating at 21.7 eV probe photon energy is reported. According to a high-power ytterbium laser, optical parametric chirped pulse amplification, and ultraviolet-driven high-harmonic generation, the light source produces an isolated high-harmonic with 110 meV bandwidth and a flux of more than 10 11 photons/s on the sample. Along with a state-of-the-art ARPES chamber, this table-top experiment allows high-repetition rate pump-probe experiments of electron dynamics in occupied and normally unoccupied (excited) states in the entire Brillouin zone and with a temporal system response function below 40 fs.

Authors:
ORCiD logo [1];  [2]; ORCiD logo [3];  [4]; ORCiD logo [2];  [4]; ORCiD logo [5];  [3]; ORCiD logo [4];  [4]; ORCiD logo [4]
  1. Fritz Haber Inst.of the Max Planck Society, Berlin (Germany); Ecole Polytechnique Federale Lausanne, Lausanne (Switzlerland)
  2. Fritz Haber Inst.of the Max Planck Society, Berlin (Germany); Paul Scherrer Inst. (PSI), Villigen (Switzerland)
  3. Fritz Haber Inst.of the Max Planck Society, Berlin (Germany); Univ. of Fribourg, Fribourg (Switzerland)
  4. Fritz Haber Inst.of the Max Planck Society, Berlin (Germany)
  5. SLAC National Accelerator Lab. (SLAC), Menlo Park, CA (United States)
Publication Date:
Research Org.:
SLAC National Accelerator Lab. (SLAC), Menlo Park, CA (United States)
Sponsoring Org.:
Max Planck Society, Dresden (Germany); European Research Council (ERC), Brussels (Belgium); German Research Foundation, Bonn (Germany); USDOE
OSTI Identifier:
1504724
Grant/Contract Number:  
AC02-76SF00515; PZ00P2-154867; ERC-2015-CoG-682843; 280879
Resource Type:
Journal Article: Accepted Manuscript
Journal Name:
Review of Scientific Instruments
Additional Journal Information:
Journal Volume: 90; Journal Issue: 2; Journal ID: ISSN 0034-6748
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
47 OTHER INSTRUMENTATION; 36 MATERIALS SCIENCE

Citation Formats

Puppin, Michele, Deng, Y., Nicholson, C. W., Feldl, J., Schröter, N. B. M., Vita, H., Kirchmann, P. S., Monney, C., Rettig, L., Wolf, M., and Ernstorfer, R.. Time- and angle-resolved photoemission spectroscopy of solids in the extreme ultraviolet at 500 kHz repetition rate. United States: N. p., 2019. Web. doi:10.1063/1.5081938.
Puppin, Michele, Deng, Y., Nicholson, C. W., Feldl, J., Schröter, N. B. M., Vita, H., Kirchmann, P. S., Monney, C., Rettig, L., Wolf, M., & Ernstorfer, R.. Time- and angle-resolved photoemission spectroscopy of solids in the extreme ultraviolet at 500 kHz repetition rate. United States. doi:10.1063/1.5081938.
Puppin, Michele, Deng, Y., Nicholson, C. W., Feldl, J., Schröter, N. B. M., Vita, H., Kirchmann, P. S., Monney, C., Rettig, L., Wolf, M., and Ernstorfer, R.. Tue . "Time- and angle-resolved photoemission spectroscopy of solids in the extreme ultraviolet at 500 kHz repetition rate". United States. doi:10.1063/1.5081938.
@article{osti_1504724,
title = {Time- and angle-resolved photoemission spectroscopy of solids in the extreme ultraviolet at 500 kHz repetition rate},
author = {Puppin, Michele and Deng, Y. and Nicholson, C. W. and Feldl, J. and Schröter, N. B. M. and Vita, H. and Kirchmann, P. S. and Monney, C. and Rettig, L. and Wolf, M. and Ernstorfer, R.},
abstractNote = {Time- and angle-resolved photoemission spectroscopy (trARPES) employing a 500 kHz extreme-ultraviolet light source operating at 21.7 eV probe photon energy is reported. According to a high-power ytterbium laser, optical parametric chirped pulse amplification, and ultraviolet-driven high-harmonic generation, the light source produces an isolated high-harmonic with 110 meV bandwidth and a flux of more than 1011 photons/s on the sample. Along with a state-of-the-art ARPES chamber, this table-top experiment allows high-repetition rate pump-probe experiments of electron dynamics in occupied and normally unoccupied (excited) states in the entire Brillouin zone and with a temporal system response function below 40 fs.},
doi = {10.1063/1.5081938},
journal = {Review of Scientific Instruments},
issn = {0034-6748},
number = 2,
volume = 90,
place = {United States},
year = {2019},
month = {2}
}

Journal Article:
Free Publicly Available Full Text
This content will become publicly available on February 12, 2020
Publisher's Version of Record

Save / Share:

Works referenced in this record:

X-Ray Interactions: Photoabsorption, Scattering, Transmission, and Reflection at E = 50-30,000 eV, Z = 1-92
journal, July 1993

  • Henke, B. L.; Gullikson, E. M.; Davis, J. C.
  • Atomic Data and Nuclear Data Tables, Vol. 54, Issue 2, p. 181-342
  • DOI: 10.1006/adnd.1993.1013

High power ultrafast lasers
journal, March 1998

  • Backus, Sterling; Durfee, Charles G.; Murnane, Margaret M.
  • Review of Scientific Instruments, Vol. 69, Issue 3, p. 1207-1223
  • DOI: 10.1063/1.1148795