Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

Observation of Dicke cooperativity in magnetic interactions

Journal Article · · Science

The interaction ofNtwo-level atoms with a single-mode light field is an extensively studied many-body problem in quantum optics, first analyzed by Dicke in the context of superradiance. A characteristic of such systems is the cooperative enhancement of the coupling strength by a factor of N. In this study, we extended this cooperatively enhanced coupling to a solid-state system, demonstrating that it also occurs in a magnetic solid in the form of matter-matter interaction. Specifically, the exchange interaction ofNparamagnetic erbium(III) (Er3+) spins with an iron(III) (Fe3+) magnon field in erbium orthoferrite (ErFeO3) exhibits a vacuum Rabi splitting whose magnitude is proportional to N. Our results provide a route for understanding, controlling, and predicting novel phases of condensed matter using concepts and tools available in quantum optics.

Research Organization:
Argonne National Lab. (ANL), Argonne, IL (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
DOE Contract Number:
AC02-06CH11357
OSTI ID:
1501365
Journal Information:
Science, Vol. 361, Issue 6404; ISSN 0036-8075
Publisher:
AAAS
Country of Publication:
United States
Language:
English

References (29)

Nonlinear spin control by terahertz-driven anisotropy fields October 2016
Diamagnetic shift of exciton energy levels in GaAs-Ga1−xAlxAs quantum wells November 1986
Resonance and high frequency susceptibility in canted antiferromagnetic substances May 1963
Ultrastrong Light-Matter Coupling Regime with Polariton Dots November 2010
Review of Recent Work on the Magnetic and Spectroscopic Properties of the Rare‐Earth Orthoferrites March 1969
Terahertz Time-Domain Observation of Spin Reorientation in Orthoferrite ErFeO 3 through Magnetic Free Induction Decay March 2013
Coherent Two-Dimensional Terahertz Magnetic Resonance Spectroscopy of Collective Spin Waves May 2017
On the superradiant phase transition for molecules in a quantized radiation field: the dicke maser model April 1973
Magnetic Structure of ErFe O 3 below 4.5°K October 1973
Coherence in Spontaneous Radiation Processes January 1954
Heavy-fermion systems October 1984
Exchange Fields and Optical Zeeman Effect in ErFe O 3 September 1969
Hybridizing Ferromagnetic Magnons and Microwave Photons in the Quantum Limit August 2014
Magneto- to Electroactive Transmutation of Spin Waves in ErMnO 3 April 2014
Raman Scattering from Magnon Excitations in RFeO 3 December 1988
Collective non-perturbative coupling of 2D electrons with high-quality-factor terahertz cavity photons August 2016
The quadratic Zeeman-effect in the principal series of caesium, rubidium and potassium February 1949
Approximate Solutions for an N -Molecule-Radiation-Field Hamiltonian December 1969
Resolving the spin reorientation and crystal-field transitions in TmFeO3 with terahertz transient March 2016
Sub-cycle switch-on of ultrastrong light–matter interaction March 2009
Asymmetric Splitting of an Antiferromagnetic Resonance via Quartic Exchange Interactions in Multiferroic Hexagonal HoMnO 3 December 2017
Observation of the coupled exciton-photon mode splitting in a semiconductor quantum microcavity December 1992
Magnetic phase control by an electric field July 2004
Are super-radiant phase transitions possible? April 1978
Effect of Y and Bi Substitution on Spin Reorientation and Optical Absorption in ErFeO 3 March 1969
Selective Excitation of Terahertz Magnetic and Electric Dipoles in Er 3 + Ions by Femtosecond Laser Pulses in ErFeO 3 January 2017
Inelastic neutron scattering studies of YFeO 3 January 2014
Quantum Simulation of the Cooperative Jahn-Teller Transition in 1D Ion Crystals June 2012
Theory of spin reorientation in rare-earth orthochromites and orthoferrites January 1974

Similar Records

Related Subjects