Pressure-induced amorphization in plagioclase feldspars: A time-resolved powder diffraction study during rapid compression

Sims, Melissa; Jaret, Steven J.; Carl, Eva -Regine; Rhymer, Brandon; Schrodt, Nadine; Mohrholz, Vivien; Smith, Jesse; Konopkova, Zuzana; Liermann, Hanns -Peter; Glotch, Timothy D.; Ehm, Lars

doi:10.1016/j.epsl.2018.11.038

Title: Pressure-induced amorphization in plagioclase feldspars: A time-resolved powder diffraction study during rapid compression

Journal Article · Mon Dec 17 00:00:00 EST 2018 · Earth and Planetary Science Letters

DOI:https://doi.org/10.1016/j.epsl.2018.11.038· OSTI ID:1495010

Sims, Melissa ^[1]; Jaret, Steven J. ^[1]; Carl, Eva -Regine ^[2]; Rhymer, Brandon ^[1]; Schrodt, Nadine ^[3]; Mohrholz, Vivien ^[4]; Smith, Jesse ^[5]; Konopkova, Zuzana ^[6]; Liermann, Hanns -Peter ^[7]; Glotch, Timothy D. ^[1]; Ehm, Lars ^[8]

Stony Brook Univ., Stony Brook, NY (United States)
Albert-Ludwig-Univ. Freiburg, Freiburg (Germany)
Goethe-Univ. Frankfurt, Frankfurt (Germany)
Friedrich-Schiller-Univ. Jena, Jena (Germany)
Carnegie Institution of Washington, Argonne, IL (United States)
European XFEL GmbH, Schenefeld (Germany)
Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany)
Stony Brook Univ., Stony Brook, NY (United States); Brookhaven National Lab. (BNL), Upton, NY (United States)

The pressure-induced amorphization of the two endmembers of the plagioclase ((Na_1–xCa_x)Al_1+xSi_3–xO₈) solid-solution, anorthite (CaAl₂Si₂O₈) and albite (NaAlSi₃O₈), has been studied as a function of compression rate by means of time-resolved powder diffraction. Anorthite and albite were compressed in a diamond anvil cell to 80 GPa at multiple rates from 0.05 GPa/s to 80 GPa/s. The amorphization pressure decreases with increasing compression rate. This negative strain rate sensitivity indicates a change in deformation mechanism in the plagioclase solid-solution endmembers from brittle to ductile with increasing compression rate. The presented data support the previously proposed shear deformation mechanism for the amorphization of plagioclase. Furthermore, amorphization progresses over a wide pressure range suggesting heterogeneous amorphization, similar to observations based on recovered material from shock-compression experiments of plagioclase. As a result, our experiments support the contention that amorphization pressures for plagioclase may occur at lower pressures than usually considered.

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: SC0012704; NA0001974; FG02-99ER45775; AC02-06CH11357

OSTI ID:: 1495010

Alternate ID(s):: OSTI ID: 1635864

Report Number(s):: BNL-211280-2019-JAAM

Journal Information:: Earth and Planetary Science Letters, Vol. 507, Issue C; ISSN 0012-821X

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 30 works

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Title: Pressure-induced amorphization in plagioclase feldspars: A time-resolved powder diffraction study during rapid compression

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