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Title: Controlling 3-D Morphology of Ni-Fe-Based Nanocatalysts for Oxygen Evolution Reaction

Abstract

Here, controlling the 3-D morphology of nanocatalysts is one of the underexplored but important approaches for improving the sluggish kinetics of oxygen evolution reaction (OER) in water electrolysis. This work reports a scalable, oil-based method based on thermal decomposition or organometallic complexes to yield highly uniform Ni-Fe-based nanocatalysts with well-defined morphology (i.e., Ni-Fe core-shell, Ni/Fe alloy, and Fe-Ni core shell).

Authors:
 [1]; ORCiD logo [2];  [1];  [3];  [1];  [4];  [4];  [2];  [5];  [1];  [1]
  1. Univ. of Arkansas, Fayetteville, AR (United States)
  2. Brookhaven National Lab. (BNL), Upton, NY (United States)
  3. Brookhaven National Lab. (BNL), Upton, NY (United States); Tsinghua Univ., Beijing (People's Republic of China)
  4. Argonne National Lab. (ANL), Lemont, IL (United States)
  5. Tsinghua Univ., Beijing (People's Republic of China)
Publication Date:
Research Org.:
Brookhaven National Lab. (BNL), Upton, NY (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1494044
Alternate Identifier(s):
OSTI ID: 1494964
Report Number(s):
BNL-211253-2019-JAAM
Journal ID: ISSN 2040-3364
Grant/Contract Number:  
SC0012704; AC02-06CH11357
Resource Type:
Journal Article: Accepted Manuscript
Journal Name:
Nanoscale
Additional Journal Information:
Journal Volume: 11; Journal Issue: 17; Journal ID: ISSN 2040-3364
Publisher:
Royal Society of Chemistry
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats

Manso, Ryan H., Zhu, Yimei, Acharya, Prashant, Deng, Shiqing, Crane, Cameron C., Reinhart, Benjamin, Lee, Sungsik, Tong, Xiao, Zhu, Jing, Greenlee, Lauren F., and Chen, Jingyi. Controlling 3-D Morphology of Ni-Fe-Based Nanocatalysts for Oxygen Evolution Reaction. United States: N. p., 2019. Web. doi:10.1039/C8NR10138H.
Manso, Ryan H., Zhu, Yimei, Acharya, Prashant, Deng, Shiqing, Crane, Cameron C., Reinhart, Benjamin, Lee, Sungsik, Tong, Xiao, Zhu, Jing, Greenlee, Lauren F., & Chen, Jingyi. Controlling 3-D Morphology of Ni-Fe-Based Nanocatalysts for Oxygen Evolution Reaction. United States. doi:10.1039/C8NR10138H.
Manso, Ryan H., Zhu, Yimei, Acharya, Prashant, Deng, Shiqing, Crane, Cameron C., Reinhart, Benjamin, Lee, Sungsik, Tong, Xiao, Zhu, Jing, Greenlee, Lauren F., and Chen, Jingyi. Mon . "Controlling 3-D Morphology of Ni-Fe-Based Nanocatalysts for Oxygen Evolution Reaction". United States. doi:10.1039/C8NR10138H. https://www.osti.gov/servlets/purl/1494044.
@article{osti_1494044,
title = {Controlling 3-D Morphology of Ni-Fe-Based Nanocatalysts for Oxygen Evolution Reaction},
author = {Manso, Ryan H. and Zhu, Yimei and Acharya, Prashant and Deng, Shiqing and Crane, Cameron C. and Reinhart, Benjamin and Lee, Sungsik and Tong, Xiao and Zhu, Jing and Greenlee, Lauren F. and Chen, Jingyi},
abstractNote = {Here, controlling the 3-D morphology of nanocatalysts is one of the underexplored but important approaches for improving the sluggish kinetics of oxygen evolution reaction (OER) in water electrolysis. This work reports a scalable, oil-based method based on thermal decomposition or organometallic complexes to yield highly uniform Ni-Fe-based nanocatalysts with well-defined morphology (i.e., Ni-Fe core-shell, Ni/Fe alloy, and Fe-Ni core shell).},
doi = {10.1039/C8NR10138H},
journal = {Nanoscale},
issn = {2040-3364},
number = 17,
volume = 11,
place = {United States},
year = {2019},
month = {2}
}

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