skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Accessing the Intrinsic Spin Transport in a Topological Insulator by Controlling the Crossover of Bulk-to-Surface Conductance

Journal Article · · Physical Review Letters

Here we report a method to control contributions of bulk and surface states in the topological insulator Bi2Te2Se that allows accessing the spin-polarized transport endowed by topological surface states. An intrinsic surface dominant transport is established when cooling the sample to low temperature or reducing the conduction channel length, both achieved in situ in the transport measurements with a four-probe scanning tunneling microscope without the need of further tailoring the sample. The topological surface states show characteristic transport behaviors with mobility about an order of magnitude higher than reported before, and a spin polarization approaching the theoretically predicted value. Our result demonstrates accessibility to the intrinsic high mobility spin transport of topological surface states, which paves a way to realizing topological spintronic devices.

Research Organization:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC05-00OR22725
OSTI ID:
1493127
Journal Information:
Physical Review Letters, Vol. 121, Issue 17; ISSN 0031-9007
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 11 works
Citation information provided by
Web of Science

References (61)

Observation of Dirac Holes and Electrons in a Topological Insulator journal June 2011
Bulk Band Gap and Surface State Conduction Observed in Voltage-Tuned Crystals of the Topological Insulator Bi 2 Se 3 journal May 2011
Surface-Dominated Transport on a Bulk Topological Insulator journal June 2014
Charge puddles in the bulk and on the surface of the topological insulator BiSbTeSe 2 studied by scanning tunneling microscopy and optical spectroscopy journal November 2017
Manifestation of Topological Protection in Transport Properties of Epitaxial Bi 2 Se 3 Thin Films journal August 2012
Intrinsic and extrinsic performance limits of graphene devices on SiO2 journal March 2008
Unoccupied topological surface state in Bi 2 Te 2 Se journal August 2013
Nanoscale electron transport at the surface of a topological insulator journal April 2016
Fermi-level-dependent charge-to-spin current conversion by Dirac surface states of topological insulators journal July 2016
Differentiation of Surface and Bulk Conductivities in Topological Insulators via Four-Probe Spectroscopy journal March 2016
Electrical resistance of individual defects at a topological insulator surface journal June 2017
Oscillatory crossover from two-dimensional to three-dimensional topological insulators journal January 2010
Energy Gap Induced by Friedel Oscillations Manifested as Transport Asymmetry at Monolayer-Bilayer Graphene Boundaries journal February 2014
Quantum Spin Hall Effect in Graphene journal November 2005
Optimizing Bi 2 x Sb x Te 3 y Se y solid solutions to approach the intrinsic topological insulator regime journal October 2011
Electron Transport at the Nanometer-Scale Spatially Revealed by Four-Probe Scanning Tunneling Microscopy journal March 2013
Record Surface State Mobility and Quantum Hall Effect in Topological Insulator Thin Films via Interface Engineering journal November 2015
Carrier statistics and quantum capacitance of graphene sheets and ribbons journal August 2007
Experimental Realization of a Three-Dimensional Topological Insulator, Bi2Te3 journal June 2009
Surface conduction of topological Dirac electrons in bulk insulating Bi2Se3 journal April 2012
Spatially Resolved Mapping of Electrical Conductivity across Individual Domain (Grain) Boundaries in Graphene journal August 2013
Mapping the chemical potential dependence of current-induced spin polarization in a topological insulator journal October 2015
Quantum Oscillations and Hall Anomaly of Surface States in the Topological Insulator Bi2Te3 journal July 2010
A cryogenic Quadraprobe scanning tunneling microscope system with fabrication capability for nanotransport research journal December 2007
Atomic-Scale Mapping of Thermoelectric Power on Graphene: Role of Defects and Boundaries journal June 2013
Topological Insulators in Three Dimensions journal March 2007
Electrical injection and detection of spin-polarized currents in topological insulator Bi2Te2Se journal September 2015
Large bulk resistivity and surface quantum oscillations in the topological insulator Bi 2 Te 2 Se journal December 2010
Surface Magnetism of Cobalt Nanoislands Controlled by Atomic Hydrogen journal December 2016
Topological surface states and Dirac point tuning in ternary topological insulators journal June 2012
Spin Polarization and Transport of Surface States in the Topological Insulators Bi 2 Se 3 and Bi 2 Te 3 from First Principles journal December 2010
Modeling potentiometric measurements in topological insulators including parallel channels journal August 2012
Microscopic investigation of Bi2-xSbxTe3-ySey systems: On the origin of a robust intrinsic topological insulator journal May 2019
Electrical Detection of the Spin Polarization Due to Charge Flow in the Surface State of the Topological Insulator Bi 1.5 Sb 0.5 Te 1.7 Se 1.3 journal October 2014
Spin-transfer torque generated by a topological insulator journal July 2014
Detection of the Spin-Chemical Potential in Topological Insulators Using Spin-Polarized Four-Probe STM journal September 2017
Room Temperature Electrical Detection of Spin Polarized Currents in Topological Insulators journal November 2015
Electrical detection of charge-current-induced spin polarization due to spin-momentum locking in Bi2Se3 journal February 2014
Crossover of the three-dimensional topological insulator Bi2Se3 to the two-dimensional limit journal June 2010
Interpreting current-induced spin polarization in topological insulator surface states journal June 2016
Electron transport in stepped Bi 2 Se 3 thin films journal July 2017
Local potential fluctuation of topological surface states in Bi 1.5 Sb 0.5 Te 1.7 Se 1.3 observed by Landau level spectroscopy journal February 2016
Electronic Transport on the Nanoscale: Ballistic Transmission and Ohm’s Law journal April 2009
Imaging and manipulation of the competing electronic phases near the Mott metal-insulator transition journal March 2010
Scattering times and surface conductivity of Dirac fermions in a 3D topological insulator film with localised impurities journal September 2015
Observation of topological surface state quantum Hall effect in an intrinsic three-dimensional topological insulator journal November 2014
Atomic-scale transport in epitaxial graphene journal November 2011
Atomic-Scale Mapping of Thermoelectric Power on Graphene: Role of Defects and Boundaries text January 2018
Atomic-Scale Mapping of Thermoelectric Power on Graphene: Role of Defects and Boundaries text January 2013
Spatially Resolved Mapping of Electrical Conductivity across Individual Domain (Grain) Boundaries in Graphene text January 2013
Spatially Resolved Mapping of Electrical Conductivity across Individual Domain (Grain) Boundaries in Graphene text January 2013
Intrinsic and Extrinsic Performance Limits of Graphene Devices on SiO2 text January 2007
Observation of Dirac Holes and Electrons in a Topological Insulator text January 2011
Manifestation of Topological Protection in Transport Properties of Epitaxial Bi2Se3 Thin Films text January 2012
Unoccupied topological surface state in Bi$_{2}$Te$_{2}$Se text January 2013
Electrical detection of the spin polarization due to charge flow in the surface state of the topological insulator Bi_1.5 Sb_0.5 Te_1.7 Se_1.3 text January 2014
Electrical injection and detection of spin-polarized currents in topological insulator Bi2Te2Se text January 2015
Mapping the chemical potential dependence of current-induced spin polarization in a topological insulator text January 2015
Interpreting current-induced spin polarization in topological insulator surface states text January 2016
Charge puddles in the bulk and on the surface of the topological insulator BiSbTeSe$_2$ studied by scanning tunneling microscopy and optical spectroscopy text January 2017
Topological Insulators in Three Dimensions text January 2006

Cited By (3)

Atomic‐Scale Manipulation and In Situ Characterization with Scanning Tunneling Microscopy journal October 2019
Electronic transport in planar atomic-scale structures measured by two-probe scanning tunneling spectroscopy journal April 2019
Millimetre-long transport of photogenerated carriers in topological insulators journal December 2019

Figures / Tables (3)