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Title: Enhanced high-harmonic generation from an all-dielectric metasurface

Journal Article · · Nature Physics

The recent observation of high-harmonic generation from solids creates a new possibility for engineering fundamental strong-field processes by patterning the solid target with subwavelength nanostructures. All-dielectric metasurfaces exhibit high damage thresholds and strong enhancement of the driving field, making them attractive platforms to control high harmonics and other high-field processes at the nanoscale. Here we report enhanced non-perturbative high-harmonic emission from a Fano-resonant Si metasurface that possesses a classical analogue of electromagnetically induced transparency. The harmonic emission is enhanced by more than two orders of magnitude compared to unpatterned samples. The enhanced high harmonics are highly anisotropic with respect to the excitation polarization and are selective by the excitation wavelength due to its resonant features. Furthermore, by combining nanofabrication technology and ultrafast strong-field physics, our work paves the way for the design of new compact ultrafast photonic devices that operate under high intensities and at short wavelengths.

Research Organization:
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
Sponsoring Organization:
USDOE
Grant/Contract Number:
AC02-76SF00515
OSTI ID:
1490657
Journal Information:
Nature Physics, Vol. 14, Issue 10; ISSN 1745-2473
Publisher:
Nature Publishing Group (NPG)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 167 works
Citation information provided by
Web of Science

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Cited By (18)

Third‐Harmonic Generation from Plasmonic Metasurfaces Coupled to Intersubband Transitions journal February 2019
Gallium Oxide for High‐Power Optical Applications journal January 2020
Strain effect on the orientation-dependent harmonic spectrum of monolayer aluminum nitride journal December 2019
High-harmonic generation from an epsilon-near-zero material journal July 2019
All semiconductor enhanced high-harmonic generation from a single nanostructured cone journal April 2019
Strongly resonant metasurfaces supported by reflective substrates for highly efficient second- and high-harmonic generations with ultralow pump intensity journal January 2019
Resonant dielectric metasurfaces: active tuning and nonlinear effects journal July 2019
Overcoming the efficiency-bandwidth tradeoff for optical harmonics generation using nonlinear time-variant resonators journal December 2019
Nonlinear Vectorial Metasurface for Optical Encryption journal August 2019
Wave mixing and high harmonic generation at two-color multiphoton excitation in two-dimensional hexagonal nanostructures journal July 2019
Multiple toroidal dipole Fano resonances of asymmetric dielectric nanohole arrays journal November 2019
High- Q Quasibound States in the Continuum for Nonlinear Metasurfaces journal December 2019
High-harmonic generation at the nanoscale boosted by bound states in the continuum journal September 2019
Dependence of solid-HHG on relative potential energy of occupied sites journal October 2019
All-optical switch and logic gates based on hybrid silicon-Ge 2 Sb 2 Te 5 metasurfaces journal January 2019
Spontaneous photon-pair generation from a dielectric nanoantenna journal January 2019
Second-Harmonic Generation in Mie-Resonant GaAs Nanowires journal August 2019
High-Order Harmonic Generation in Au Nanoparticle-Contained Plasmas journal January 2020

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