Atomic Layer Co3O4 Nanosheets: The Key to Knittable Zn-Air Batteries

Chen, Xu; Zhong, Cheng; Liu, Bin; Liu, Zhi; Bi, Xuanxuan; Zhao, Naiqing; Han, Xiaopeng; Deng, Yida; Lu, Jun; Hu, Wenbin

doi:10.1002/smll.201702987

Title: Atomic Layer Co₃O₄ Nanosheets: The Key to Knittable Zn-Air Batteries

Journal Article · Thu Feb 01 00:00:00 EST 2018 · Small

DOI:https://doi.org/10.1002/smll.201702987· OSTI ID:1487113

Chen, Xu ^[1];

^[2]; Liu, Bin ^[1]; Liu, Zhi ^[1]; Bi, Xuanxuan ^[3]; Zhao, Naiqing ^[4]; Han, Xiaopeng ^[4]; Deng, Yida ^[4]; Lu, Jun ^[3]; Hu, Wenbin ^[2]

Shanghai Jiao Tong Univ. (China). Dept. of Materials Science and Engineering
Univ. of Technology, Tianjing (China). Tianjin Key Lab. of Composite and Functional Materials, School of Materials Science and Engineering, Key Lab. of Advanced Ceramics and Machining Technology (Ministry of Education)
Argonne National Lab. (ANL), Argonne, IL (United States). Chemical Sciences and Engineering Division
Univ. of Technology, Tianjing (China). Tianjin Key Lab. of Composite and Functional Materials, School of Materials Science and Engineering

Flexible, wearable, and portable energy storage devices with high-energy density are crucial for next-generation electronics. However, the current battery technologies such as lithium ion batteries have limited theoretical energy density. Additionally, battery materials with small scale and high flexibility which could endure the large surface stress are highly required. In this study, a yarn-based 1D Zn-air battery is designed, which employs atomic layer thin Co₃O₄ nanosheets as the oxygen reduction reaction/oxygen evolution reaction catalyst. The ultrathin nanosheets are synthesized by a high-yield and facile chemical method and show a thickness of only 1.6 nm, corresponding to few atomic layers. The 1D Zn-air battery shows high cycling stability and high rate capability. The battery is successfully knitted into clothes and it shows high stability during the large deformation and knotting conditions.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: National Natural Science Foundation of China (NSFC)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1487113

Journal Information:: Small, Vol. 14, Issue 43; ISSN 1613-6810

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 73 works

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Title: Atomic Layer Co3O4 Nanosheets: The Key to Knittable Zn-Air Batteries

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