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Title: Freestanding 1T MoS 2 /graphene heterostructures as a highly efficient electrocatalyst for lithium polysulfides in Li–S batteries

Abstract

A novel approach to effectively suppress the “polysulfide shuttle” in Li–S batteries is presented by designing a freestanding, three-dimensional graphene/1T MoS 2 (3DG/TM) heterostructure with highly efficient electrocatalysis properties for lithium polysulfides (LiPSs).

Authors:
 [1];  [2];  [2]; ORCiD logo [2]; ORCiD logo [3]; ORCiD logo [4]
  1. Materials Science and Engineering Program & Texas Materials Institute, The University of Texas at Austin, Austin, USA, State Key Laboratory of Electronic Thin Films and Integrated Devices
  2. McKetta Department of Chemical Engineering, The University of Texas at Austin, Austin, USA
  3. State Key Laboratory of Electronic Thin Films and Integrated Devices, University of Electronic Science and Technology of China, Chengdu 610054, P. R. China
  4. Materials Science and Engineering Program & Texas Materials Institute, The University of Texas at Austin, Austin, USA
Publication Date:
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1485180
Grant/Contract Number:  
SC0005397
Resource Type:
Journal Article: Publisher's Accepted Manuscript
Journal Name:
Energy & Environmental Science
Additional Journal Information:
Journal Name: Energy & Environmental Science; Journal ID: ISSN 1754-5692
Publisher:
Royal Society of Chemistry (RSC)
Country of Publication:
United Kingdom
Language:
English

Citation Formats

He, Jiarui, Hartmann, Gregory, Lee, Myungsuk, Hwang, Gyeong S., Chen, Yuanfu, and Manthiram, Arumugam. Freestanding 1T MoS 2 /graphene heterostructures as a highly efficient electrocatalyst for lithium polysulfides in Li–S batteries. United Kingdom: N. p., 2019. Web. doi:10.1039/C8EE03252A.
He, Jiarui, Hartmann, Gregory, Lee, Myungsuk, Hwang, Gyeong S., Chen, Yuanfu, & Manthiram, Arumugam. Freestanding 1T MoS 2 /graphene heterostructures as a highly efficient electrocatalyst for lithium polysulfides in Li–S batteries. United Kingdom. doi:10.1039/C8EE03252A.
He, Jiarui, Hartmann, Gregory, Lee, Myungsuk, Hwang, Gyeong S., Chen, Yuanfu, and Manthiram, Arumugam. Tue . "Freestanding 1T MoS 2 /graphene heterostructures as a highly efficient electrocatalyst for lithium polysulfides in Li–S batteries". United Kingdom. doi:10.1039/C8EE03252A.
@article{osti_1485180,
title = {Freestanding 1T MoS 2 /graphene heterostructures as a highly efficient electrocatalyst for lithium polysulfides in Li–S batteries},
author = {He, Jiarui and Hartmann, Gregory and Lee, Myungsuk and Hwang, Gyeong S. and Chen, Yuanfu and Manthiram, Arumugam},
abstractNote = {A novel approach to effectively suppress the “polysulfide shuttle” in Li–S batteries is presented by designing a freestanding, three-dimensional graphene/1T MoS 2 (3DG/TM) heterostructure with highly efficient electrocatalysis properties for lithium polysulfides (LiPSs).},
doi = {10.1039/C8EE03252A},
journal = {Energy & Environmental Science},
number = ,
volume = ,
place = {United Kingdom},
year = {Tue Jan 01 00:00:00 EST 2019},
month = {Tue Jan 01 00:00:00 EST 2019}
}

Journal Article:
Free Publicly Available Full Text
This content will become publicly available on November 27, 2019
Publisher's Accepted Manuscript

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Works referenced in this record:

MoS2 Nanoparticles Grown on Graphene An Advanced Catalyst for the Hydrogen Evolution Reaction
journal, May 2011

  • Li, Yanguang; Wang, Hailiang; Xie, Liming
  • Journal of the American Chemical Society, Vol. 133, Issue 19, p. 7296-7299
  • DOI: 10.1021/ja201269b