Spin reorientation and magnetoelastic properties of ferromagnetic Tb1-xNdxCo2 systems with a morphotropic phase boundary

doi:https://doi.org/10.1103/PhysRevB.97.104410

Title: Spin reorientation and magnetoelastic properties of ferromagnetic $T b_{1 - x} N d_{x} C o_{2}$ systems with a morphotropic phase boundary

Abstract

The spin reorientation (SR) and magnetoelastic properties of pseudobinary ferromagnetic Tb _1–xNd _xCo ₂ (0 ≤ x ≤ 1.0) systems involving a morphotropic phase boundary (MPB) were studied by high-resolution synchrotron x-ray diffraction (XRD), magnetization, and magnetostriction measurements. The easy magnetization direction of the Laves phase lies along the < 111 > axis with x < 0.65, whereas it lies along the < 100 > axis for x > 0.65 below Curie temperature (TC). The temperature-dependent magnetization curves showed SR; this can be explained by a two-sublattice model. Based on the synchrotron (XRD) and magnetization measurements, the SR phase diagram for a MPB composition of Tb _0.35Nd _0.65Co ₂ was obtained. Contrary to previously reported ferromagnetic systems involving MPB, the MPB composition of Tb _0.35Nd _0.65Co ₂ exhibits a low saturation magnetization (MS), indicating a compensation of the Tb and Nd magnetic moments at MPB. The anisotropic magnetostriction (λS) first decreased until x = 0.8 and then continuously increased in the negative direction with further increase of Nd concentration. The decrease in magnetostriction can be attributed to the decrease of spontaneous magnetostriction λ ₁₁₁ and increase of λ ₁₀₀ with opposite sign to λ ₁₁₁. In conclusion, this paper indicatesmore »« less

Authors:

Murtaza, Adil ^[1]; Yang, Sen ^[1]; Chang, Tieyan ^[1]; Ghani, Awais ^[1]; Khan, Muhammad Tahir ^[1]; Zhang, Rui ^[1]; Zhou, Chao ^[1]; Song, Xiaoping ^[1]; Suchomel, Matthew ^[2]; Ren, Yang ^[2]

Xi'an Jiaotong Univ., Xi'an (China)
Argonne National Lab. (ANL), Argonne, IL (United States)

Publication Date:: 2018-03-15

Research Org.:: Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Org.:: National Natural Science Foundation of China (NNSFC); USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division

OSTI Identifier:: 1481168

Alternate Identifier(s):: OSTI ID: 1426330

Grant/Contract Number:: AC02-06CH11357

Resource Type:: Journal Article: Accepted Manuscript

Journal Name:: Physical Review B

Additional Journal Information:: Journal Volume: 97; Journal Issue: 10; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE

Citation Formats


                    Murtaza, Adil, Yang, Sen, Chang, Tieyan, Ghani, Awais, Khan, Muhammad Tahir, Zhang, Rui, Zhou, Chao, Song, Xiaoping, Suchomel, Matthew, and Ren, Yang. Spin reorientation and magnetoelastic properties of ferromagnetic Tb1-xNdxCo2 systems with a morphotropic phase boundary.  United States: N. p., 2018. 
        Web.  doi:10.1103/PhysRevB.97.104410.

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                    Murtaza, Adil, Yang, Sen, Chang, Tieyan, Ghani, Awais, Khan, Muhammad Tahir, Zhang, Rui, Zhou, Chao, Song, Xiaoping, Suchomel, Matthew, & Ren, Yang. Spin reorientation and magnetoelastic properties of ferromagnetic Tb1-xNdxCo2 systems with a morphotropic phase boundary.  United States.  https://doi.org/10.1103/PhysRevB.97.104410

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                    Murtaza, Adil, Yang, Sen, Chang, Tieyan, Ghani, Awais, Khan, Muhammad Tahir, Zhang, Rui, Zhou, Chao, Song, Xiaoping, Suchomel, Matthew, and Ren, Yang. Thu .  
        "Spin reorientation and magnetoelastic properties of ferromagnetic Tb1-xNdxCo2 systems with a morphotropic phase boundary".  United States.  https://doi.org/10.1103/PhysRevB.97.104410.  https://www.osti.gov/servlets/purl/1481168.

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@article{osti_1481168,

  title        = {Spin reorientation and magnetoelastic properties of ferromagnetic Tb1-xNdxCo2 systems with a morphotropic phase boundary},

  author       = {Murtaza, Adil and Yang, Sen and Chang, Tieyan and Ghani, Awais and Khan, Muhammad Tahir and Zhang, Rui and Zhou, Chao and Song, Xiaoping and Suchomel, Matthew and Ren, Yang},

  abstractNote = {The spin reorientation (SR) and magnetoelastic properties of pseudobinary ferromagnetic Tb1–xNdxCo2 (0 ≤ x ≤ 1.0) systems involving a morphotropic phase boundary (MPB) were studied by high-resolution synchrotron x-ray diffraction (XRD), magnetization, and magnetostriction measurements. The easy magnetization direction of the Laves phase lies along the < 111 > axis with x < 0.65, whereas it lies along the < 100 > axis for x > 0.65 below Curie temperature (TC). The temperature-dependent magnetization curves showed SR; this can be explained by a two-sublattice model. Based on the synchrotron (XRD) and magnetization measurements, the SR phase diagram for a MPB composition of Tb0.35Nd0.65Co2 was obtained. Contrary to previously reported ferromagnetic systems involving MPB, the MPB composition of Tb0.35Nd0.65Co2 exhibits a low saturation magnetization (MS), indicating a compensation of the Tb and Nd magnetic moments at MPB. The anisotropic magnetostriction (λS) first decreased until x = 0.8 and then continuously increased in the negative direction with further increase of Nd concentration. The decrease in magnetostriction can be attributed to the decrease of spontaneous magnetostriction λ111 and increase of λ100 with opposite sign to λ111. In conclusion, this paper indicates an anomalous type of MPB in the ferromagnetic Tb1–xNdxCo2 system and provides an active way to design novel functional materials with exotic properties.},

  doi          = {10.1103/PhysRevB.97.104410},

  url          = {https://www.osti.gov/biblio/1481168},
  journal      = {Physical Review B},

  issn         = {2469-9950},

  number       = 10,

  volume       = 97,

  place        = {United States},

  year         = {2018},

  month        = {3}

}

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Works referencing / citing this record:

Electronic specific heat coefficient and magnetic properties of $Y {({Fe}_{1 - x} {Co}_{x})}_{2}$ Laves phases: A combined experimental and first-principles study
journal, October 2019

Wasilewski, Bartosz; Śniadecki, Zbigniew; Werwiński, Mirosław
Physical Review B, Vol. 100, Issue 13
https://doi.org/10.1103/physrevb.100.134436

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Title: Spin reorientation and magnetoelastic properties of ferromagnetic T b 1 - x N d x C o 2 systems with a morphotropic phase boundary

Abstract

Citation Formats

Origin of morphotropic phase boundaries in ferroelectrics journal, January 2008

Spin configurations in the absence of a magnetic field in a two-sublattice system journal, May 1995

Gd5(SixGe1-x)4: An Extremum Material journal, May 2001

Inverse effect of morphotropic phase boundary on the magnetostriction of ferromagnetic Tb 1 − x Gd x Co 2 journal, March 2014

Crystal and magnetic structures of Laves phase compound NdCo2 in the temperature range between 9 and 300K journal, August 2006

Magnetostrictive properties of Tbx(Pr0.5Nd0.5)1−xFe1.93 cubic Laves alloys journal, December 2013

Recent advances in magnetic structure determination by neutron powder diffraction journal, October 1993

Metamagnetic phase transition in Nd1−x TbxCo2 compounds journal, May 2007

Itinerant metamagnetism journal, August 1988

Magnetic properties of (Nd x Y 1-x )Co 2 (1⩾ x ⩾ 0) journal, June 1983

Itinerant metamagnetism [Зонный метамагнетизм] journal, January 1988

Large Magnetostriction from Morphotropic Phase Boundary in Ferromagnets journal, May 2010

Magnetic and magnetostrictive properties in high-pressure synthesized Dy1−xPrxFe1.9(0≤x≤1) cubic Laves alloys journal, September 2010

Physical properties of RCo 2 Laves phases journal, May 2001

Spontaneous magnetostriction of Laves phase Nd1−xTbxCo2 compounds journal, June 2004

Mixing effects of light and heavy rare earths in the Laves phase compounds Nd1−xTbxCo2 journal, July 2002

On the 4f-3d exchange interaction in intermetallic compounds journal, April 1994

Temperature dependent neutron powder diffraction study of the Laves phase compound TbCo2 journal, March 2005

Magnetic structure, magnetostriction, and magnetic transitions of the Laves-phase compound Nd Co 2 journal, February 2005

Magnetostriction and structural distortion in rare-earth intermetallics journal, May 1977

Morphotropic phase boundary and magnetoelastic behaviour in ferromagnetic Tb1−xGdxFe2 system journal, March 2015

Triple-point-type morphotropic phase boundary based large piezoelectric Pb-free material—Ba(Ti 0.8 Hf 0.2 )O 3 -(Ba 0.7 Ca 0.3 )TiO 3 journal, May 2012

Structure and magnetostriction of Nd 0.67 Tb 0.33 (Co 1 x Fe x ) 2 compounds journal, March 2003

Magnetoelastic properties of RE-3d intermetallics journal, March 1990

Low temperature rhombohedral distortion in TbCo2 journal, January 1980

Structural and magnetic properties of morphotropic phase boundary involved Tb1−xGdxFe2 compounds journal, September 2016

Temperature and magnetic field dependence of the elastic properties of the HoxTb1−xCo2 Laves phase compounds journal, January 1980

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Isotropic and anisotropic magnetoelastic interactions in heavy and light RCo 2 Laves phase compounds journal, August 1994

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Title: Spin reorientation and magnetoelastic properties of ferromagnetic $T b_{1 - x} N d_{x} C o_{2}$ systems with a morphotropic phase boundary

Origin of morphotropic phase boundaries in ferroelectrics
journal, January 2008

Spin configurations in the absence of a magnetic field in a two-sublattice system
journal, May 1995

Gd5(SixGe1-x)4: An Extremum Material
journal, May 2001

Inverse effect of morphotropic phase boundary on the magnetostriction of ferromagnetic Tb $_{1 - x}$ Gd $_{x}$ Co $_{2}$
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Crystal and magnetic structures of Laves phase compound NdCo2 in the temperature range between 9 and 300K
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Magnetostrictive properties of Tbx(Pr0.5Nd0.5)1−xFe1.93 cubic Laves alloys
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Recent advances in magnetic structure determination by neutron powder diffraction
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Metamagnetic phase transition in Nd1−x TbxCo2 compounds
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Itinerant metamagnetism
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Magnetic properties of (Nd x Y 1-x )Co 2 (1⩾ x ⩾ 0)
journal, June 1983

Itinerant metamagnetism [Зонный метамагнетизм]
journal, January 1988

Large Magnetostriction from Morphotropic Phase Boundary in Ferromagnets
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Magnetic and magnetostrictive properties in high-pressure synthesized Dy1−xPrxFe1.9(0≤x≤1) cubic Laves alloys
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Physical properties of RCo ₂ Laves phases
journal, May 2001

Spontaneous magnetostriction of Laves phase Nd1−xTbxCo2 compounds
journal, June 2004

Mixing effects of light and heavy rare earths in the Laves phase compounds Nd1−xTbxCo2
journal, July 2002

On the 4f-3d exchange interaction in intermetallic compounds
journal, April 1994

Temperature dependent neutron powder diffraction study of the Laves phase compound TbCo2
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Magnetic structure, magnetostriction, and magnetic transitions of the Laves-phase compound $Nd {Co}_{2}$
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Magnetostriction and structural distortion in rare-earth intermetallics
journal, May 1977

Morphotropic phase boundary and magnetoelastic behaviour in ferromagnetic Tb1−xGdxFe2 system
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Triple-point-type morphotropic phase boundary based large piezoelectric Pb-free material—Ba(Ti _0.8 Hf _0.2 )O ₃ -(Ba _0.7 Ca _0.3 )TiO ₃
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Structure and magnetostriction of Nd _0.67 Tb _0.33 (Co _{1 x} Fe _x ) ₂ compounds
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Magnetoelastic properties of RE-3d intermetallics
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Low temperature rhombohedral distortion in TbCo2
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Structural and magnetic properties of morphotropic phase boundary involved Tb1−xGdxFe2 compounds
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Temperature and magnetic field dependence of the elastic properties of the HoxTb1−xCo2 Laves phase compounds
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