Odyssey of Multivalent Cathode Materials: Open Questions and Future Challenges

Canepa, Pieremanuele; Sai Gautam, Gopalakrishnan; Hannah, Daniel C.; Malik, Rahul; Liu, Miao; Gallagher, Kevin G.; Persson, Kristin A.; Ceder, Gerbrand

doi:10.1021/acs.chemrev.6b00614

Title: Odyssey of Multivalent Cathode Materials: Open Questions and Future Challenges

Journal Article · Mon Feb 13 00:00:00 EST 2017 · Chemical Reviews

DOI:https://doi.org/10.1021/acs.chemrev.6b00614· OSTI ID:1343461

^[1];

^[2]; Hannah, Daniel C. ^[3]; Malik, Rahul ^[4]; Liu, Miao ^[5]; Gallagher, Kevin G. ^[6]; Persson, Kristin A. ^[5]; Ceder, Gerbrand ^[2]

Materials Science Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, United States, Department of Materials Science and Engineering, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139, United States
Materials Science Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, United States, Department of Materials Science and Engineering, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139, United States, Department of Materials Science and Engineering, University of California Berkeley, California 94720, United States
Materials Science Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, United States
Department of Materials Science and Engineering, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139, United States
Energy and Environmental Science Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, United States
Chemical Sciences and Engineering, Argonne National Laboratory, Lemont, Illinois 60439, United States

We report that the rapidly expanding field of nonaqueous multivalent intercalation batteries offers a promising way to overcome safety, cost, and energy density limitations of state-of-the-art Li-ion battery technology. We present a critical and rigorous analysis of the increasing volume of multivalent battery research, focusing on a wide range of intercalation cathode materials and the mechanisms of multivalent ion insertion and migration within those frameworks. The present analysis covers a wide variety of material chemistries, including chalcogenides, oxides, and polyanions, highlighting merits and challenges of each class of materials as multivalent cathodes. The review underscores the overlap of experiments and theory, ranging from charting the design metrics useful for developing the next generation of MV-cathodes to targeted in-depth studies rationalizing complex experimental results. In conclusion, on the basis of our critical review of the literature, we provide suggestions for future multivalent cathode studies, including a strong emphasis on the unambiguous characterization of the intercalation mechanisms.

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Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: 3F-31144; AC02-05CH11231

OSTI ID:: 1343461

Alternate ID(s):: OSTI ID: 1476467

Journal Information:: Chemical Reviews, Journal Name: Chemical Reviews Vol. 117 Journal Issue: 5; ISSN 0009-2665

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 820 works

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Li2MnSiO4 cathodes modified by phosphorous substitution and the structural consequences Gummow, Rosalind J.; Han, Guihong; Sharma, Neeraj Solid State Ionics, Vol. 259 https://doi.org/10.1016/j.ssi.2014.02.002	journal	June 2014
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Influence of relative humidity on the structure and electrochemical performance of sustainable LiFeSO ₄ F electrodes for Li-ion batteries Zhang, Leiting; Tarascon, Jean-Marie; Sougrati, Moulay Tahar Journal of Materials Chemistry A, Vol. 3, Issue 33 https://doi.org/10.1039/C5TA05107J	journal	January 2015
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