Magnetooptics of Exciton Rydberg States in a Monolayer Semiconductor

Stier, A. V.; Wilson, N. P.; Velizhanin, K. A.; Kono, J.; Xu, X.; Crooker, S. A.

doi:10.1103/PhysRevLett.120.057405

Title: Magnetooptics of Exciton Rydberg States in a Monolayer Semiconductor

Journal Article · Thu Feb 01 00:00:00 EST 2018 · Physical Review Letters

DOI:https://doi.org/10.1103/PhysRevLett.120.057405· OSTI ID:1475347

Stier, A. V. ^[1]; Wilson, N. P. ^[2]; Velizhanin, K. A. ^[3]; Kono, J. ^[4]; Xu, X. ^[2]; Crooker, S. A. ^[1]

National High Magnetic Field Lab. (MagLab), Los Alamos, NM (United States)
Univ. of Washington, Seattle, WA (United States). Dept. of Physics
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Rice Univ., Houston, TX (United States). Dept. of Electrical and Computer Engineering. Dept. of Physics and Astronomy. Dept. of Materials Science and NanoEngineering

In this paper, we report 65 T magnetoabsorption spectroscopy of exciton Rydberg states in the archetypal monolayer semiconductor ${WSe}_{2}$ . The strongly field-dependent and distinct energy shifts of the $2 s$ , $3 s$ , and $4 s$ excited neutral excitons permits their unambiguous identification and allows for quantitative comparison with leading theoretical models. Both the sizes (via low-field diamagnetic shifts) and the energies of the $n s$ exciton states agree remarkably well with detailed numerical simulations using the nonhydrogenic screened Keldysh potential for 2D semiconductors. Finally and moreover, at the highest magnetic fields, the nearly linear diamagnetic shifts of the weakly bound $3 s$ and $4 s$ excitons provide a direct experimental measure of the exciton’s reduced mass $m_{r} = 0.20 \pm 0.01 m_{0}$ .

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Research Organization:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States); Univ. of Washington, Seattle, WA (United States); National High Magnetic Field Lab. (MagLab), Los Alamos, NM (United States); Rice Univ., Houston, TX (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF); US Air Force Office of Scientific Research (AFOSR)

Grant/Contract Number:: AC52-06NA25396; SC0018171; DMR-1157490; FA9550-14-1-0268

OSTI ID:: 1475347

Alternate ID(s):: OSTI ID: 1419092

Report Number(s):: LA-UR-17-27395

Journal Information:: Physical Review Letters, Vol. 120, Issue 5; ISSN 0031-9007

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 159 works

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