“Unleaded” Perovskites: Status Quo and Future Prospects of Tin-Based Perovskite Solar Cells
Abstract
The tremendous interest focused on organic–inorganic halide perovskites since 2012 derives from their unique optical and electrical properties, which make them excellent photovoltaic materials. Pb-based halide perovskite solar cells, in particular, currently stand at a record efficiency of ≈23%, fulfilling their potential toward commercialization. However, because of the toxicity concerns of Pb-based perovskite solar cells, their market prospects are hindered. In principle, Pb can be replaced with other less-toxic, environmentally benign metals. Sn-based perovskites are thus the far most promising alternative due to their very similar and perhaps even superior semiconductor characteristics. Additionally, after years of effort invested in Sn-based halide perovskites, sufficient breakthroughs have finally been achieved that make them the next runners up to the Pb halide perovskites. To help the reader better understand the nature of Sn-based halide perovskites, their optical and electrical properties are systematically discussed. Recent progress in Sn-based perovskite solar cells, focusing mainly on film fabrication methods and different device architectures, and highlighting roadblocks to progress and opportunities for future work are reviewed. Finally, a brief overview of mixed Sn/Pb-based systems with their anomalous yet beneficial optical trends are discussed. The current challenges and a future outlook for Sn-based perovskites are discussed.
- Authors:
-
- Northwestern Univ., Evanston, IL (United States)
- Publication Date:
- Research Org.:
- Energy Frontier Research Centers (EFRC) (United States). Center for Light Energy Activated Redox Processes (LEAP)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)
- OSTI Identifier:
- 1767508
- Alternate Identifier(s):
- OSTI ID: 1475216
- Grant/Contract Number:
- SC0001059; DMR-1121262
- Resource Type:
- Journal Article: Accepted Manuscript
- Journal Name:
- Advanced Materials
- Additional Journal Information:
- Journal Volume: 31; Journal Issue: 47; Journal ID: ISSN 0935-9648
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 14 SOLAR ENERGY; catalysis (homogeneous); catalysis (heterogeneous); solar (photovoltaic); solar (fuels); optics; phonons; photosynthesis (natural and artificial); bio-inspired; hydrogen and fuel cells; charge transport; magnetism and spin physics; materials and chemistry by design; mesostructured materials; synthesis (novel materials); synthesis (self-assembly); synthesis (scalable processing); halide perovskites; tin-based lead-free solar cells
Citation Formats
Ke, Weijun, Stoumpos, Constantinos C., and Kanatzidis, Mercouri G. “Unleaded” Perovskites: Status Quo and Future Prospects of Tin-Based Perovskite Solar Cells. United States: N. p., 2018.
Web. doi:10.1002/adma.201803230.
Ke, Weijun, Stoumpos, Constantinos C., & Kanatzidis, Mercouri G. “Unleaded” Perovskites: Status Quo and Future Prospects of Tin-Based Perovskite Solar Cells. United States. https://doi.org/10.1002/adma.201803230
Ke, Weijun, Stoumpos, Constantinos C., and Kanatzidis, Mercouri G. 2018.
"“Unleaded” Perovskites: Status Quo and Future Prospects of Tin-Based Perovskite Solar Cells". United States. https://doi.org/10.1002/adma.201803230. https://www.osti.gov/servlets/purl/1767508.
@article{osti_1767508,
title = {“Unleaded” Perovskites: Status Quo and Future Prospects of Tin-Based Perovskite Solar Cells},
author = {Ke, Weijun and Stoumpos, Constantinos C. and Kanatzidis, Mercouri G.},
abstractNote = {The tremendous interest focused on organic–inorganic halide perovskites since 2012 derives from their unique optical and electrical properties, which make them excellent photovoltaic materials. Pb-based halide perovskite solar cells, in particular, currently stand at a record efficiency of ≈23%, fulfilling their potential toward commercialization. However, because of the toxicity concerns of Pb-based perovskite solar cells, their market prospects are hindered. In principle, Pb can be replaced with other less-toxic, environmentally benign metals. Sn-based perovskites are thus the far most promising alternative due to their very similar and perhaps even superior semiconductor characteristics. Additionally, after years of effort invested in Sn-based halide perovskites, sufficient breakthroughs have finally been achieved that make them the next runners up to the Pb halide perovskites. To help the reader better understand the nature of Sn-based halide perovskites, their optical and electrical properties are systematically discussed. Recent progress in Sn-based perovskite solar cells, focusing mainly on film fabrication methods and different device architectures, and highlighting roadblocks to progress and opportunities for future work are reviewed. Finally, a brief overview of mixed Sn/Pb-based systems with their anomalous yet beneficial optical trends are discussed. The current challenges and a future outlook for Sn-based perovskites are discussed.},
doi = {10.1002/adma.201803230},
url = {https://www.osti.gov/biblio/1767508},
journal = {Advanced Materials},
issn = {0935-9648},
number = 47,
volume = 31,
place = {United States},
year = {Mon Sep 17 00:00:00 EDT 2018},
month = {Mon Sep 17 00:00:00 EDT 2018}
}
Web of Science
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