Wettability impact on supercritical CO2 capillary trapping: Pore-scale visualization and quantification

Hu, Ran; Wan, Jiamin; Kim, Yongman; Tokunaga, Tetsu K.

doi:10.1002/2017WR020721

Title: Wettability impact on supercritical CO₂ capillary trapping: Pore-scale visualization and quantification

Journal Article · Thu Jul 13 00:00:00 EDT 2017 · Water Resources Research

DOI:https://doi.org/10.1002/2017WR020721· OSTI ID:1469958

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Wuhan Univ. of Technology (China). State Key Lab. of Water Resources and Hydropower Engineering Science; Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Energy Geosciences Division
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)

How the wettability of pore surfaces affects supercritical (sc) CO₂ capillary trapping in geologic carbon sequestration (GCS) is not well understood, and available evidence appears inconsistent. Using a high-pressure micromodel-microscopy system with image analysis, we studied the impact of wettability on scCO₂ capillary trapping during short-term brine flooding (80 s, 8–667 pore volumes). Experiments on brine displacing scCO₂ were conducted at 8.5 MPa and 45°C in water-wet (static contact angle θ = 20° ± 8°) and intermediate-wet (θ = 94° ± 13°) homogeneous micromodels under four different flow rates (capillary number Ca ranging from 9 × 10^-6 to 8 × 10^-4) with a total of eight conditions (four replicates for each). Brine invasion processes were recorded and statistical analysis was performed for over 2000 images of scCO₂ saturations, and scCO₂ cluster characteristics. The trapped scCO₂ saturation under intermediate-wet conditions is 15% higher than under water-wet conditions under the slowest flow rate (Ca ~ 9 × 10-6). Based on the visualization and scCO₂ cluster analysis, we show that the scCO₂ trapping process in our micromodels is governed by bypass trapping that is enhanced by the larger contact angle. Smaller contact angles enhance cooperative pore filling and widen brine fingers (or channels), leading to smaller volumes of scCO₂ being bypassed. Increased flow rates suppress this wettability effect.

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Research Organization:: Energy Frontier Research Centers (EFRC) (United States). Center for Nanoscale Control of Geologic CO2 (NCGC); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Washington, DC (United States); National Natural Science Foundation of China (NSFC), Beijing (China)

Grant/Contract Number:: AC02-05CH11231; 51409198; 51579188

OSTI ID:: 1469958

Alternate ID(s):: OSTI ID: 1580093

Journal Information:: Water Resources Research, Vol. 53, Issue 8; Related Information: NCGC partners with Lawrence Berkeley National Laboratory (lead); University of California, Davis; Lawrence Livermore National Laboratory; Massachusetts Institute of Technology; Ohio State University; Oak Ridge National Laboratory; Washington University, St. Louis; ISSN 0043-1397

Publisher:: American Geophysical Union (AGU)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 53 works

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wettability
micromodel
supercritical carbon dioxide
geologic carbon sequestration

Title: Wettability impact on supercritical CO2 capillary trapping: Pore-scale visualization and quantification

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Title: Wettability impact on supercritical CO₂ capillary trapping: Pore-scale visualization and quantification