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Title: Threshold characteristics of ultraviolet and near infrared nanosecond laser induced plasmas

Journal Article · · Physics of Plasmas
DOI:https://doi.org/10.1063/1.4963248· OSTI ID:1468934

The present contribution compares the energy absorption, optical emission, temperature, and fluid dynamics of ultraviolet (UV) λ = 266 nm and near infrared (NIR) λ = 1064 nm nanosecond laser induced plasmas in ambient air. For UV pulses at the conditions studied, energy absorption by the plasmas increases relatively gradually with laser pulse energy starting at delivered energy of E~ 8 mJ. Corresponding measurements of plasma luminosity show that the absorption of UV radiation does not necessarily result in visible plasma emission. For the NIR induced plasmas, the energy absorption profile is far more abrupt and begins at ~55 mJ. In contrast with UV, the absorption of NIR radiation is always accompanied by intense optical emission. The temperatures of both types of plasma have been measured with Rayleigh scattering thermometry (at times after the Thomson signal sufficiently diminishes). The UV plasmas can attain a wider range of temperatures, including lower temperatures, depending on the pulse energy (e.g., T~400–2000 K for E~7–35 mJ at Δt = 10 μs after the pulse) while the NIR plasmas show only hotter temperatures (e.g., T~12 000 K for E = 75 mJ at Δt = 10 μs after the pulse) as is consistent with the literature. Differences in the fluid dynamics for UV versus NIR pulses are shown with Schlieren imaging. Finally, the contrast in the UV and NIR plasma threshold behavior is attributed to differing roles of avalanche ionization and multiphoton ionization as is also illustrated by a simple numerical model.

Research Organization:
Colorado State Univ., Fort Collins, CO (United States). Mechanical Engineering
Sponsoring Organization:
USDOE; National Science Foundation (NSF)
Grant/Contract Number:
SC0012454
OSTI ID:
1468934
Alternate ID(s):
OSTI ID: 1328457
Journal Information:
Physics of Plasmas, Vol. 23, Issue 9; ISSN 1070-664X
Publisher:
American Institute of Physics (AIP)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 18 works
Citation information provided by
Web of Science

References (34)

Laser-induced breakdown of gases journal May 1975
Laser‐induced breakdown studies of laboratory air at 0.266, 0.355, 0.532, and 1.06 μm journal September 1991
Temperature measurements from first-negative N2+ spectra produced by laser-induced multiphoton ionization and optical breakdown of nitrogen journal January 1995
Pressure dependence of the laser-induced breakdown thresholds of gases and droplets journal January 1990
Laser Rayleigh scattering journal April 2001
Two Wavelength Interferometry of a Laser‐Induced Spark in air journal April 1966
Standoff spectroscopy via remote generation of a backward-propagating laser beam journal February 2011
Schlieren and Shadowgraph Techniques book January 2001
Laser-induced plasma formation in Xe, Ar, N_2, and O_2 at the first four Nd:YAG harmonics journal January 1991
Measurements of minimum ignition energy in premixed laminar methane/air flow by using laser induced spark journal March 2003
Laser-induced fluorescence in N2 and N+2 by multiple-photon excitation at 266 nm journal March 1981
Control of extended high-voltage electric discharges in atmospheric air by UV KrF-laser radiation journal March 2011
Laser-induced optical breakdown applied for laser spark ignition journal March 2010
Fundamentals of high-energy spark ignition with lasers journal July 2004
Frequency Dependence of Optically Induced GAS Breakdown journal November 1965
Laser spark ignition: experimental determination of laser-induced breakdown thresholds of combustion gases journal March 2000
Multiphoton Ionization of Hydrogen and Rare-Gas Atoms journal March 1966
Gas Discharge Physics book January 1991
An optical and spectroscopic study of laser-induced sparks to determine available ignition energy journal January 2002
Experimental Demonstration of Laser Temporal Coherence Effects on Multiphoton Ionization Processes journal February 1974
Novel miniaturized high-energy Nd-YAG laser for spark ignition in internal combustion engines journal January 2009
Experimental measurements of multiphoton enhanced air breakdown by a subthreshold intensity excimer laser journal October 2009
Laser rayleigh thermometry in turbulent flames journal January 1981
Laser induced breakdown of Ar, N2 and O2 gases using 1.064, 0.532, 0.355 and 0.266 μm radiation journal December 1996
New diagnostic methods for laser plasma- and microwave-enhanced combustion
  • Miles, Richard B.; Michael, James B.; Limbach, Christopher M.
  • Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 373, Issue 2048 https://doi.org/10.1098/rsta.2014.0338
journal August 2015
Laser-induced breakdown spectroscopy for detection of explosives residues: a review of recent advances, challenges, and future prospects journal May 2009
Long-lived laser-induced microwave plasma guides in the atmosphere: Self-consistent plasma-dynamic analysis and numerical simulations journal August 2010
Effect of Light Polarization on Multiphoton Ionization of Atoms journal March 1972
Temperature and Electron Density Measurements of Laser-Induced Plasmas in Air at Elevated Pressures journal February 2011
Laser spark in gases journal June 1974
Laser plasma formation assisted by ultraviolet pre-ionization journal October 2014
Kinetic scheme of the non-equilibrium discharge in nitrogen-oxygen mixtures journal August 1992
Laser-Induced Breakdown Spectroscopy for In-Cylinder Equivalence Ratio Measurements in Laser-Ignited Natural Gas Engines journal May 2009
Study of Laser-Induced Plasma Emission Spectra of N 2 , O 2 , and Ambient Air in the Region 350 nm to 950 nm journal October 1995

Cited By (5)

Laser-Induced Plasma Formation in Ar, N 2 , and CH 4 at Low Pressure: Energy Deposition and Flow Dynamics conference June 2019
The impact of nano-bubbles on the laser performance of hafnia films deposited by oxygen assisted ion beam sputtering method journal December 2019
Numerical Modeling of the Hydrodynamics Induced by Dual-Pulse Plasma conference January 2018
Control of Early Flame Kernel Growth by Multi-Wavelength Laser Pulses for Enhanced Ignition journal August 2017
Ultraviolet Raman spectroscopy of N2in a recombining atmospheric pressure plasma journal October 2017

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