Simultaneously achieved large reversible elastocaloric and magnetocaloric effects and their coupling in a magnetic shape memory alloy

Qu, Y. H.; Cong, D. Y.; Li, S. H.; Gui, W. Y.; Nie, Z. H.; Zhang, M. H.; Ren, Y.; Wang, Y. D.

doi:10.1016/j.actamat.2018.03.031

Title: Simultaneously achieved large reversible elastocaloric and magnetocaloric effects and their coupling in a magnetic shape memory alloy

Journal Article · Thu Mar 22 00:00:00 EDT 2018 · Acta Materialia

DOI:https://doi.org/10.1016/j.actamat.2018.03.031· OSTI ID:1466400

Qu, Y. H. ^[1]; Cong, D. Y. ^[1]; Li, S. H. ^[1]; Gui, W. Y. ^[1];

^[2]; Zhang, M. H. ^[1]; Ren, Y. ^[3]; Wang, Y. D. ^[1]

Univ. of Science and Technology Beijing, Beijing (People's Republic of China)
Beijing Institute of Technology, Beijing (People's Republic of China)
Argonne National Lab. (ANL), Argonne, IL (United States)

Large reversible caloric effects covering a broad temperature region are essential for high-efficiency and environment-friendly solid-state caloric refrigeration that can potentially replace the traditional vaporcompression-based cooling technology. Here, we report the simultaneously achieved large reversible magnetocaloric and elastocaloric effects in a Ni₄₃Co₆Mn₄₀Sn₁₁ magnetic shape memory alloy. A reversible near-room-temperature magnetic entropy change ΔS_m of as high as 19.3 J kg^–1 K^–1 under 5 T was experimentally obtained and the corresponding adiabatic temperature change ΔT_ad was estimated to be 7.7 K. Meanwhile, a large reversible elastocaloric effect with a directly measured ΔT_ad up to 7.1 K was attained. The elastocaloric effect exhibits high cyclic stability with no apparent degradation during 380 cycles of loading and unloading. Furthermore, we propose and demonstrate the utilization of the multicaloric approach under the coupled uniaxial stress and magnetic field to enlarge the refrigeration temperature region of reversible caloric effects. By combining the reversible magnetocaloric and elastocaloric effects and the reversible multicaloric effect under the coupling of uniaxial stress and magnetic field in the hysteresis region, large reversible caloric effects covering a broad temperature region from 257 K to 383 K can be obtained. Finally, this study may pave the way for designing advanced caloric materials with cyclically stable and reversible large caloric effects and wide refrigeration temperature region for solid-state refrigeration.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division; National Natural Science Foundation of China (NSFC); Chinese Academy of Sciences (CAS), State Key Laboratory for Advanced Metals and Materials

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1466400

Alternate ID(s):: OSTI ID: 1548568

Journal Information:: Acta Materialia, Vol. 151, Issue C; ISSN 1359-6454

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 89 works

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36 MATERIALS SCIENCE
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Title: Simultaneously achieved large reversible elastocaloric and magnetocaloric effects and their coupling in a magnetic shape memory alloy

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