Local orthorhombic lattice distortions in the paramagnetic tetragonal phase of superconducting NaFe1-xNixAs

Wang, Weiyi; Song, Yu; Cao, Chongde; Tseng, Kuo-Feng; Keller, Thomas; Li, Yu; Harriger, L. W.; Tian, Wei; Chi, Songxue; Yu, Rong; Nevidomskyy, Andriy H.; Dai, Pengcheng

doi:10.1038/s41467-018-05529-2

Title: Local orthorhombic lattice distortions in the paramagnetic tetragonal phase of superconducting NaFe1-xNixAs

Journal Article · Tue Aug 07 00:00:00 EDT 2018 · Nature Communications

DOI:https://doi.org/10.1038/s41467-018-05529-2· OSTI ID:1463970

Wang, Weiyi ^[1]; Song, Yu ^[1]; Cao, Chongde ^[2]; Tseng, Kuo-Feng ^[3];

^[3]; Li, Yu ^[1]; Harriger, L. W. ^[4]; Tian, Wei ^[5]; Chi, Songxue ^[5]; Yu, Rong ^[6]; Nevidomskyy, Andriy H. ^[1];

^[1]

Rice Univ., Houston, TX (United States). Dept. of Physics and Astronomy
Northwestern Polytechnical Univ., Xian (China). Dept. of Applied Physics
Max-Planck-Inst. fur Festkorperforschung, Stuttgart (Germany); Max Planck Society Outstation at the Forschungsneutronenquelle Heinz Maier-Leibnitz (MLZ), Garching (Germany)
National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States). Center for Neutron Research
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Neutron Scattering Division
Renmin Univ. of China, Beijing (China). Dept. of Physics and Beijing Key Lab. of Opto-electronic Functional Materials and Micro-nano Devices

Understanding the interplay between nematicity, magnetism and superconductivity is pivotal for elucidating the physics of iron-based superconductors. Here we use neutron scattering to probe magnetic and nematic orders throughout the phase diagram of NaFe_1-xNi_xAs, finding that while both static antiferromagnetic and nematic orders compete with superconductivity, the onset temperatures for these two orders remain well separated approaching the putative quantum critical points. We uncover local orthorhombic distortions that persist well above the tetragonal-to-orthorhombic structural transition temperature T_s in underdoped samples and extend well into the overdoped regime that exhibits neither magnetic nor structural phase transitions. These unexpected local orthorhombic distortions display Curie–Weiss temperature dependence and become suppressed below the superconducting transition temperature T_c, suggesting that they result from the large nematic susceptibility near optimal superconductivity. Finally, our results account for observations of rotational symmetry breaking above T_s, and attest to the presence of significant nematic fluctuations near optimal superconductivity.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC); National Science Foundation (NSF)

Grant/Contract Number:: AC05-00OR22725; SC0012311; C-1839; C-1818; DMR-1350237

OSTI ID:: 1463970

Journal Information:: Nature Communications, Vol. 9, Issue 1; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 19 works

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