The dual nature of magnetism in a uranium heavy fermion system

Lee, Jooseop; Matsuda, Masaaki; Mydosh, John A.; Zaliznyak, Igor; Kolesnikov, Alexander I.; Sullow, Stefan; Ruff, Jacob P. C.; Granroth, Garrett E.

doi:10.1103/PhysRevLett.121.057201

Title: The dual nature of magnetism in a uranium heavy fermion system

Journal Article · Mon Jul 30 00:00:00 EDT 2018 · Physical Review Letters

DOI:https://doi.org/10.1103/PhysRevLett.121.057201· OSTI ID:1460695

Lee, Jooseop ^[1]; Matsuda, Masaaki ^[2]; Mydosh, John A. ^[3]; Zaliznyak, Igor ^[4]; Kolesnikov, Alexander I. ^[2]; Sullow, Stefan ^[5]; Ruff, Jacob P. C. ^[6]; Granroth, Garrett E. ^[2]

Cornell Univ., Ithaca, NY (United States). Cornell High Energy Synchrotron Source (CHESS); Inst. for Basic Science, Pohang (Korea, Republic of). Center for Artificial Low Dimensional Electronic Systems (CALDES)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Neutron Scattering Division
Leiden Univ. (Netherlands). Kamerlingh Onnes Lab. Lorentz Inst.
Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics and Materials Science Dept.
Braunschweig Univ. of Technology (Germany)
Cornell Univ., Ithaca, NY (United States). Cornell High Energy Synchrotron Source (CHESS)

The duality between the localized and itinerant nature of magnetism in 5f-electron systems has been a long-standing puzzle. Here, we report inelastic neutron scattering measurements, which reveal both local and itinerant aspects of magnetism in a single-crystalline system of UPt2Si2. In the antiferromagnetic state, we observe a broad continuum of diffuse magnetic scattering with a resonancelike gap of ≈7 meV and the surprising absence of coherent spin waves, suggestive of itinerant magnetism. While the gap closes above the Néel temperature, strong dynamic spin correlations persist to a high temperature. Nevertheless, the size and temperature dependence of the total magnetic spectral weight can be well described by a local moment with J=4. Furthermore, polarized neutron measurements reveal that the magnetic fluctuations are mostly transverse, with little or none of the longitudinal component expected for itinerant moments. These results suggest that a dual description of local and itinerant magnetism is required to understand UPt2Si2 and, by extension, other 5f systems, in general.

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Cornell Univ., Ithaca, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); ORNL Laboratory Directed Research and Development (LDRD) Program; National Science Foundation (NSF); National Inst. of Health (NIH) (United States)

Grant/Contract Number:: SC0012704; DMR-1332208; AC05-00OR22725

OSTI ID:: 1460695

Alternate ID(s):: OSTI ID: 1462161; OSTI ID: 1474559

Report Number(s):: BNL-207824-2018-JAAM; TRN: US1901899

Journal Information:: Physical Review Letters, Vol. 121, Issue 5; ISSN 0031-9007

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 11 works

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References (36)

Magnetic excitations in uranium nitride Holden, T. M.; Buyers, W. J. L.; Svensson, E. C. Physical Review B, Vol. 30, Issue 1 https://doi.org/10.1103/PhysRevB.30.114	journal	July 1984
Mantid—Data analysis and visualization package for neutron scattering and $μ$ SR experiments Arnold, O.; Bilheux, J. C.; Borreguero, J. M. Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 764 https://doi.org/10.1016/j.nima.2014.07.029	journal	November 2014
Spin-liquid polymorphism in a correlated electron system on the threshold of superconductivity Zaliznyak, Igor; Savici, Andrei T.; Lumsden, Mark Proceedings of the National Academy of Sciences, Vol. 112, Issue 33 https://doi.org/10.1073/pnas.1503559112	journal	August 2015
Magnetic structure of ${UPd}_{2}$ ${Si}_{2}$ Shemirani, B.; Lin, H.; Collins, M. F. Physical Review B, Vol. 47, Issue 14 https://doi.org/10.1103/PhysRevB.47.8672	journal	April 1993
A magnetic phase transition in UCu2Ge2 Leciejewicz, J.; Chełmicki, L.; Zygmunt, A. Solid State Communications, Vol. 41, Issue 2 https://doi.org/10.1016/0038-1098(82)91059-6	journal	January 1982
The Spallation Neutron Source in Oak Ridge: A powerful tool for materials research Mason, T. E.; Abernathy, D.; Anderson, I. Physica B: Condensed Matter, Vol. 385-386 https://doi.org/10.1016/j.physb.2006.05.281	journal	November 2006
SEQUOIA: A Newly Operating Chopper Spectrometer at the SNS Granroth, G. E.; Kolesnikov, A. I.; Sherline, T. E. Journal of Physics: Conference Series, Vol. 251 https://doi.org/10.1088/1742-6596/251/1/012058	journal	November 2010
Superconductivity, antiferromagnetism, and neutron scattering Tranquada, John M.; Xu, Guangyong; Zaliznyak, Igor A. Journal of Magnetism and Magnetic Materials, Vol. 350 https://doi.org/10.1016/j.jmmm.2013.09.029	journal	January 2014
Field-induced phases in UPt $_{2}$ Si $_{2}$ Schulze Grachtrup, D.; Bleckmann, M.; Willenberg, B. Physical Review B, Vol. 85, Issue 5 https://doi.org/10.1103/PhysRevB.85.054410	journal	February 2012
Crystalline electric field effects in ${UPt}_{2}$ ${Si}_{2}$ and ${URu}_{2}$ ${Si}_{2}$ Nieuwenhuys, G. J. Physical Review B, Vol. 35, Issue 10 https://doi.org/10.1103/PhysRevB.35.5260	journal	April 1987
Antiferromagnetic criticality at a heavy-fermion quantum phase transition Knafo, W.; Raymond, S.; Lejay, P. Nature Physics, Vol. 5, Issue 10 https://doi.org/10.1038/nphys1374	journal	September 2009
Absolute cross-section normalization of magnetic neutron scattering data Xu, Guangyong; Xu, Zhijun; Tranquada, J. M. Review of Scientific Instruments, Vol. 84, Issue 8 https://doi.org/10.1063/1.4818323	journal	August 2013
Spin Resonance in the $d$ -Wave Superconductor ${CeCoIn}_{5}$ Stock, C.; Broholm, C.; Hudis, J. Physical Review Letters, Vol. 100, Issue 8 https://doi.org/10.1103/PhysRevLett.100.087001	journal	February 2008
High field magnetism of UPt2Si2 single crystals Amitsuka, H.; Sakakibara, T.; Sugiyama, K. Physica B: Condensed Matter, Vol. 177, Issue 1-4 https://doi.org/10.1016/0921-4526(92)90090-F	journal	March 1992
Spin Fluctuation Spectra and High Temperature Superconductivity Moriya, Tôru; Ueda, Kazuo Journal of the Physical Society of Japan, Vol. 63, Issue 5 https://doi.org/10.1143/JPSJ.63.1871	journal	May 1994
SEQUOIA: A fine resolution chopper spectrometer at the SNS Granroth, G. E.; Vandergriff, D. H.; Nagler, S. E. Physica B: Condensed Matter, Vol. 385-386 https://doi.org/10.1016/j.physb.2006.05.379	journal	November 2006
Magnetic correlations and quantum criticality in the insulating antiferromagnetic, insulating spin liquid, renormalized Fermi liquid, and metallic antiferromagnetic phases of the Mott system $V_{2} O_{3}$ Bao, Wei; Broholm, C.; Aeppli, G. Physical Review B, Vol. 58, Issue 19 https://doi.org/10.1103/PhysRevB.58.12727	journal	November 1998
Spin-density-wave antiferromagnetism in chromium Fawcett, Eric Reviews of Modern Physics, Vol. 60, Issue 1 https://doi.org/10.1103/RevModPhys.60.209	journal	January 1988
Colloquium : Hidden order, superconductivity, and magnetism: The unsolved case of ${URu}_{2} {Si}_{2}$ Mydosh, J. A.; Oppeneer, P. M. Reviews of Modern Physics, Vol. 83, Issue 4 https://doi.org/10.1103/RevModPhys.83.1301	journal	November 2011
Neutron scattering experiments on UPt2Si2 Steeman, R. A.; Frikkee, E.; van Dijk, C. Journal of Magnetism and Magnetic Materials, Vol. 76-77 https://doi.org/10.1016/0304-8853(88)90447-7	journal	December 1988
Itinerant to localized transition of f electrons in the antiferromagnetic superconductor UPd2Al3 Fujimori, Shin-Ichi; Saitoh, Yuji; Okane, Tetsuo Nature Physics, Vol. 3, Issue 9 https://doi.org/10.1038/nphys651	journal	July 2007
Magnetic phase diagram and electronic structure of ${UPt}_{2} {Si}_{2}$ at high magnetic fields: A possible field-induced Lifshitz transition Grachtrup, D. Schulze; Steinki, N.; Süllow, S. Physical Review B, Vol. 95, Issue 13 https://doi.org/10.1103/PhysRevB.95.134422	journal	April 2017
Effect of Spin Fluctuations on Itinerant Electron Antiferromagnetism Hasegawa, Hideo; Moriya, Tôru Journal of the Physical Society of Japan, Vol. 36, Issue 6 https://doi.org/10.1143/JPSJ.36.1542	journal	June 1974
Polarized Neutron on URu2Si2 Bourdarot, F.; Ressouche, E.; Ballou, R. Physics Procedia, Vol. 42 https://doi.org/10.1016/j.phpro.2013.03.168	journal	January 2013
Electronic structure and Fermi surface of paramagnetic and antiferromagnetic UPt $_{2}$ Si $_{2}$ Elgazzar, S.; Rusz, J.; Oppeneer, P. M. Physical Review B, Vol. 86, Issue 7 https://doi.org/10.1103/PhysRevB.86.075104	journal	August 2012
Magnetism and its microscopic origin in iron-based high-temperature superconductors Dai, Pengcheng; Hu, Jiangping; Dagotto, Elbio Nature Physics, Vol. 8, Issue 10 https://doi.org/10.1038/nphys2438	journal	October 2012
Quantitative Aspects of the Theory of Weak Itinerant Antiferromagnetism Nakayama, Kazuya; Moriya, Tôru Journal of the Physical Society of Japan, Vol. 56, Issue 8 https://doi.org/10.1143/JPSJ.56.2918	journal	August 1987
A magnetic phase transition in UNi2Si2 Chełmicki, L.; Leciejewicz, J.; Zygmunt, A. Solid State Communications, Vol. 48, Issue 2 https://doi.org/10.1016/0038-1098(83)90953-5	journal	October 1983
Spin Fluctuations in Itinerant Electron Magnetism Moriya, Tôru Springer Series in Solid-State Sciences https://doi.org/10.1007/978-3-642-82499-9	book	January 1985
Unusual magnetic excitations in the weakly ordered spin- $\frac{1}{2}$ chain antiferromagnet ${Sr}_{2} {CuO}_{3}$ : Possible evidence for Goldstone magnon coupled with the amplitude mode Sergeicheva, E. G.; Sosin, S. S.; Prozorova, L. A. Physical Review B, Vol. 95, Issue 2 https://doi.org/10.1103/PhysRevB.95.020411	journal	January 2017
Neutron diffraction study of magnetic ordering in UPd ₂ Si ₂ , UPd ₂ Ge ₂ , URh ₂ Si ₂ and URh ₂ Ge ₂ Ptasiewicz-Bak, H. Journal of Physics F: Metal Physics, Vol. 11, Issue 6 https://doi.org/10.1088/0305-4608/11/6/009	journal	June 1981
Electronic Localization and Two-Dimensional Metallic State in UPt ₂ Si ₂ Süllow, Stefan; Otop, Anna; Loose, Anja Journal of the Physical Society of Japan, Vol. 77, Issue 2 https://doi.org/10.1143/JPSJ.77.024708	journal	February 2008
Frustration-induced two-dimensional quantum disordered phase in piperazinium hexachlorodicuprate Stone, M. B.; Zaliznyak, I.; Reich, Daniel H. Physical Review B, Vol. 64, Issue 14 https://doi.org/10.1103/PhysRevB.64.144405	journal	September 2001
Horace : Software for the analysis of data from single crystal spectroscopy experiments at time-of-flight neutron instruments Ewings, R. A.; Buts, A.; Le, M. D. Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 834 https://doi.org/10.1016/j.nima.2016.07.036	journal	October 2016
Unconventional Temperature Enhanced Magnetism in ${Fe}_{1.1} Te$ Zaliznyak, Igor A.; Xu, Zhijun; Tranquada, John M. Physical Review Letters, Vol. 107, Issue 21 https://doi.org/10.1103/PhysRevLett.107.216403	journal	November 2011
Hybridisation effects in UPt ₂ Si ₂ Steeman, R. A.; Frikkee, E.; Mentink, S. A. M. Journal of Physics: Condensed Matter, Vol. 2, Issue 18 https://doi.org/10.1088/0953-8984/2/18/003	journal	May 1990

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