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Title: The effect of low-temperature aging on the microstructure and deformation of uranium- 6 wt% niobium: An in-situ neutron diffraction study

Abstract

The mechanical properties of uranium-niobium alloys evolve with aging at relatively low temperatures due to subtle microstructural changes. In-situ neutron diffraction measurements during aging of a monoclinic U-6Nb alloy at temperatures to 573 K were performed to monitor these changes. Further, in-situ neutron diffraction studies during deformation of U-6Nb in the as-quenched state and after aging for two and eight hours at 473 K were completed to assess the influence of microstructural evolution on mechanical properties. With heating, large anisotropic changes in lattice parameter were observed followed by relaxation with time at the aging temperature. The lattice parameters return to nearly their initial values with cooling. Finally, the active plastic deformation mechanisms including, in order of occurrence, shape-memory de-twinning, mechanical twinning, and slip-mediated deformation do not change with prior aging. However, the resistance to motion of the as-quenched martensitic twin boundaries increases following aging, resulting in the observed increase in initial yield strength.

Authors:
ORCiD logo [1];  [1];  [2];  [1]; ORCiD logo [1];  [1];  [3]
  1. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
  2. Colorado School of Mines, Golden, CO (United States). Dept. of Metallurgical and Materials Engineering
  3. Univ. of Wisconsin, Madison, WI (United States). Dept. of Materials Science and Engineering
Publication Date:
Research Org.:
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1458938
Alternate Identifier(s):
OSTI ID: 1396805
Report Number(s):
LA-UR-16-22216
Journal ID: ISSN 0022-3115; TRN: US1901529
Grant/Contract Number:  
AC52-06NA25396
Resource Type:
Journal Article: Accepted Manuscript
Journal Name:
Journal of Nuclear Materials
Additional Journal Information:
Journal Volume: 481; Journal Issue: C; Journal ID: ISSN 0022-3115
Publisher:
Elsevier
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE

Citation Formats

Brown, Donald William, Bourke, Mark Andrew M., Clarke, Amy Jean, Field, Robert D., Hackenberg, Robert Errol, Hults, William L., and Thoma, Daniel J. The effect of low-temperature aging on the microstructure and deformation of uranium- 6 wt% niobium: An in-situ neutron diffraction study. United States: N. p., 2016. Web. doi:10.1016/j.jnucmat.2016.09.004.
Brown, Donald William, Bourke, Mark Andrew M., Clarke, Amy Jean, Field, Robert D., Hackenberg, Robert Errol, Hults, William L., & Thoma, Daniel J. The effect of low-temperature aging on the microstructure and deformation of uranium- 6 wt% niobium: An in-situ neutron diffraction study. United States. doi:10.1016/j.jnucmat.2016.09.004.
Brown, Donald William, Bourke, Mark Andrew M., Clarke, Amy Jean, Field, Robert D., Hackenberg, Robert Errol, Hults, William L., and Thoma, Daniel J. Thu . "The effect of low-temperature aging on the microstructure and deformation of uranium- 6 wt% niobium: An in-situ neutron diffraction study". United States. doi:10.1016/j.jnucmat.2016.09.004. https://www.osti.gov/servlets/purl/1458938.
@article{osti_1458938,
title = {The effect of low-temperature aging on the microstructure and deformation of uranium- 6 wt% niobium: An in-situ neutron diffraction study},
author = {Brown, Donald William and Bourke, Mark Andrew M. and Clarke, Amy Jean and Field, Robert D. and Hackenberg, Robert Errol and Hults, William L. and Thoma, Daniel J},
abstractNote = {The mechanical properties of uranium-niobium alloys evolve with aging at relatively low temperatures due to subtle microstructural changes. In-situ neutron diffraction measurements during aging of a monoclinic U-6Nb alloy at temperatures to 573 K were performed to monitor these changes. Further, in-situ neutron diffraction studies during deformation of U-6Nb in the as-quenched state and after aging for two and eight hours at 473 K were completed to assess the influence of microstructural evolution on mechanical properties. With heating, large anisotropic changes in lattice parameter were observed followed by relaxation with time at the aging temperature. The lattice parameters return to nearly their initial values with cooling. Finally, the active plastic deformation mechanisms including, in order of occurrence, shape-memory de-twinning, mechanical twinning, and slip-mediated deformation do not change with prior aging. However, the resistance to motion of the as-quenched martensitic twin boundaries increases following aging, resulting in the observed increase in initial yield strength.},
doi = {10.1016/j.jnucmat.2016.09.004},
journal = {Journal of Nuclear Materials},
issn = {0022-3115},
number = C,
volume = 481,
place = {United States},
year = {2016},
month = {9}
}

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Cited by: 6 works
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