Intrinsic homogeneous linewidth and broadening mechanisms of excitons in monolayer transition metal dichalcogenides

Moody, Galan; Dass, Chandriker Kavir; Hao, Kai; Chen, Chang -Hsiao; Li, Lain -Jong; Singh, Akshay; Tran, Kha; Clark, Genevieve; Xu, Xiaodong; Berghauser, Gunnar; Malic, Ermin; Knorr, Andreas; Li, Xiaoqin

doi:10.1038/ncomms9315

Title: Intrinsic homogeneous linewidth and broadening mechanisms of excitons in monolayer transition metal dichalcogenides

Journal Article · Fri Sep 18 00:00:00 EDT 2015 · Nature Communications

DOI:https://doi.org/10.1038/ncomms9315· OSTI ID:1441157

Moody, Galan ^[1]; Dass, Chandriker Kavir ^[2]; Hao, Kai ^[3]; Chen, Chang -Hsiao ^[4]; Li, Lain -Jong ^[2]; Singh, Akshay ^[2]; Tran, Kha ^[2]; Clark, Genevieve ^[5]; Xu, Xiaodong ^[5]; Berghauser, Gunnar ^[6]; Malic, Ermin ^[7]; Knorr, Andreas ^[6]; Li, Xiaoqin ^[2]

Univ. of Texas at Austin, Austin, TX (United States); National Institute of Standards & Technology, Boulder, CO (United States)
Univ. of Texas at Austin, Austin, TX (United States)
Feng Chia Univ., Taichung (Taiwan)
King Abdullah Univ. of Science & Technology (KAUST), Thuwal (Saudi Arabia)
Univ. of Washington, Seattle, WA (United States)
Technische Univ. Berlin, Berlin (Germany)
Chalmers Univ. of Technology, Gothenburg (Sweden)

In this paper, the band-edge optical response of transition metal dichalcogenides, an emerging class of atomically thin semiconductors, is dominated by tightly bound excitons localized at the corners of the Brillouin zone (valley excitons). A fundamental yet unknown property of valley excitons in these materials is the intrinsic homogeneous linewidth, which reflects irreversible quantum dissipation arising from system (exciton) and bath (vacuum and other quasiparticles) interactions and determines the timescale during which excitons can be coherently manipulated. Here we use optical two-dimensional Fourier transform spectroscopy to measure the exciton homogeneous linewidth in monolayer tungsten diselenide (WSe₂). The homogeneous linewidth is found to be nearly two orders of magnitude narrower than the inhomogeneous width at low temperatures. We evaluate quantitatively the role of exciton–exciton and exciton–phonon interactions and population relaxation as linewidth broadening mechanisms. The key insights reported here—strong many-body effects and intrinsically rapid radiative recombination—are expected to be ubiquitous in atomically thin semiconductors.

View Accepted Manuscript (DOE)

Cite

Export

Save

Research Organization:: Univ. of Washington, Seattle, WA (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: SC0008145

OSTI ID:: 1441157

Journal Information:: Nature Communications, Vol. 6, Issue 1; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

Citation Metrics:

Cited by: 367 works

Citation information provided by
Web of Science

References (40)

Coupled Spin and Valley Physics in Monolayers of ${MoS}_{2}$ and Other Group-VI Dichalcogenides Xiao, Di; Liu, Gui-Bin; Feng, Wanxiang Physical Review Letters, Vol. 108, Issue 19 https://doi.org/10.1103/PhysRevLett.108.196802	journal	May 2012
Valley dynamics probed through charged and neutral exciton emission in monolayer ${WSe}_{2}$ Wang, G.; Bouet, L.; Lagarde, D. Physical Review B, Vol. 90, Issue 7 https://doi.org/10.1103/PhysRevB.90.075413	journal	August 2014
Transient nonlinear optical response from excitation induced dephasing in GaAs Wang, Hailin; Ferrio, Kyle; Steel, Duncan G. Physical Review Letters, Vol. 71, Issue 8 https://doi.org/10.1103/PhysRevLett.71.1261	journal	August 1993
Fluorescence transient and optical free induction decay spectroscopy of pentacene in mixed crystals at 2 K. Determination of intersystem crossing and internal conversion rates de Vries, Harmen; Wiersma, Douwe A. The Journal of Chemical Physics, Vol. 70, Issue 12 https://doi.org/10.1063/1.437411	journal	June 1979
Giant Enhancement of the Optical Second-Harmonic Emission of ${WSe}_{2}$ Monolayers by Laser Excitation at Exciton Resonances Wang, G.; Marie, X.; Gerber, I. Physical Review Letters, Vol. 114, Issue 9 https://doi.org/10.1103/PhysRevLett.114.097403	journal	March 2015
Mechanism of excitonic dephasing in layered InSe crystals Dey, P.; Paul, J.; Glikin, N. Physical Review B, Vol. 89, Issue 12 https://doi.org/10.1103/PhysRevB.89.125128	journal	March 2014
Optical generation of excitonic valley coherence in monolayer WSe2 Jones, Aaron M.; Yu, Hongyi; Ghimire, Nirmal J. Nature Nanotechnology, Vol. 8, Issue 9 https://doi.org/10.1038/nnano.2013.151	journal	August 2013
Exciton Radiative Lifetimes in Two-Dimensional Transition Metal Dichalcogenides Palummo, Maurizia; Bernardi, Marco; Grossman, Jeffrey C. Nano Letters, Vol. 15, Issue 5 https://doi.org/10.1021/nl503799t	journal	March 2015
Tightly Bound Excitons in Monolayer ${WSe}_{2}$ He, Keliang; Kumar, Nardeep; Zhao, Liang Physical Review Letters, Vol. 113, Issue 2 https://doi.org/10.1103/PhysRevLett.113.026803	journal	July 2014
Emerging Photoluminescence in Monolayer MoS₂ Splendiani, Andrea; Sun, Liang; Zhang, Yuanbo Nano Letters, Vol. 10, Issue 4, p. 1271-1275 https://doi.org/10.1021/nl903868w	journal	April 2010
Electronics and optoelectronics of two-dimensional transition metal dichalcogenides Wang, Qing Hua; Kalantar-Zadeh, Kourosh; Kis, Andras Nature Nanotechnology, Vol. 7, Issue 11, p. 699-712 https://doi.org/10.1038/nnano.2012.193	journal	November 2012
Transform-Limited, Narrow-Linewidth Lasing Action in Organic Semiconductor Microcavities Bulovi, V. Science, Vol. 279, Issue 5350 https://doi.org/10.1126/science.279.5350.553	journal	January 1998
Enhanced radiative recombination of free excitons in GaAs quantum wells Deveaud, B.; Clérot, F.; Roy, N. Physical Review Letters, Vol. 67, Issue 17 https://doi.org/10.1103/PhysRevLett.67.2355	journal	October 1991
Electric field dependence of optical absorption near the band gap of quantum-well structures Miller, D. A. B.; Chemla, D. S.; Damen, T. C. Physical Review B, Vol. 32, Issue 2 https://doi.org/10.1103/PhysRevB.32.1043	journal	July 1985
Coherent Electronic Coupling in Atomically Thin ${MoSe}_{2}$ Singh, Akshay; Moody, Galan; Wu, Sanfeng Physical Review Letters, Vol. 112, Issue 21 https://doi.org/10.1103/PhysRevLett.112.216804	journal	May 2014
Atomically Thin ${MoS}_{2}$ A New Direct-Gap Semiconductor Mak, Kin Fai; Lee, Changgu; Hone, James Physical Review Letters, Vol. 105, Issue 13, Article No.136805 https://doi.org/10.1103/PhysRevLett.105.136805	journal	September 2010
Low-temperature photocarrier dynamics in monolayer MoS ₂ Korn, T.; Heydrich, S.; Hirmer, M. Applied Physics Letters, Vol. 99, Issue 10 https://doi.org/10.1063/1.3636402	journal	September 2011
Strong light–matter coupling in two-dimensional atomic crystals Liu, Xiaoze; Galfsky, Tal; Sun, Zheng Nature Photonics, Vol. 9, Issue 1 https://doi.org/10.1038/nphoton.2014.304	journal	December 2014
Resonance lineshapes in two-dimensional Fourier transform spectroscopy Siemens, Mark E.; Moody, Galan; Li, Hebin Optics Express, Vol. 18, Issue 17 https://doi.org/10.1364/OE.18.017699	journal	January 2010
Many-Body Theory for the Dense Exciton Gas of Direct Semiconductors II. Calculation of Exciton Level Shift and Damping in Dependence on Exciton Density Boldt, F.; Henneberger, K.; May, V. physica status solidi (b), Vol. 130, Issue 2 https://doi.org/10.1002/pssb.2221300231	journal	August 1985
Two-Dimensional Metal–Chalcogenide Films in Tunable Optical Microcavities Schwarz, S.; Dufferwiel, S.; Walker, P. M. Nano Letters, Vol. 14, Issue 12 https://doi.org/10.1021/nl503312x	journal	November 2014
Exciton–polariton spin switches Amo, A.; Liew, T. C. H.; Adrados, C. Nature Photonics, Vol. 4, Issue 6 https://doi.org/10.1038/nphoton.2010.79	journal	April 2010
Coherent optical nonlinearities and phase relaxation of quasi-three-dimensional and quasi-two-dimensional excitons in ${ZnS}_{x} {Se}_{1 - x} / ZnSe$ structures Wagner, H. P.; Schätz, A.; Maier, R. Physical Review B, Vol. 56, Issue 19 https://doi.org/10.1103/PhysRevB.56.12581	journal	November 1997
Evolution of Electronic Structure in Atomically Thin Sheets of WS ₂ and WSe ₂ Zhao, Weijie; Ghorannevis, Zohreh; Chu, Leiqiang ACS Nano, Vol. 7, Issue 1 https://doi.org/10.1021/nn305275h	journal	December 2012
Exciton Binding Energy and Nonhydrogenic Rydberg Series in Monolayer ${WS}_{2}$ Chernikov, Alexey; Berkelbach, Timothy C.; Hill, Heather M. Physical Review Letters, Vol. 113, Issue 7 https://doi.org/10.1103/PhysRevLett.113.076802	journal	August 2014
Large-Area Synthesis of Highly Crystalline WSe ₂ Monolayers and Device Applications Huang, Jing-Kai; Pu, Jiang; Hsu, Chang-Lung ACS Nano, Vol. 8, Issue 1 https://doi.org/10.1021/nn405719x	journal	December 2013
Radiative lifetime of free excitons in quantum wells Andreani, Lucio Claudio; Tassone, Francesco; Bassani, Franco Solid State Communications, Vol. 77, Issue 9 https://doi.org/10.1016/0038-1098(91)90761-J	journal	March 1991
Control of valley polarization in monolayer MoS2 by optical helicity Mak, Kin Fai; He, Keliang; Shan, Jie Nature Nanotechnology, Vol. 7, Issue 8 https://doi.org/10.1038/nnano.2012.96	journal	June 2012
Observation of long-lived interlayer excitons in monolayer MoSe2–WSe2 heterostructures Rivera, Pasqual; Schaibley, John R.; Jones, Aaron M. Nature Communications, Vol. 6, Issue 1 https://doi.org/10.1038/ncomms7242	journal	February 2015
Collision broadening of two-dimensional excitons in a GaAs single quantum well Honold, A.; Schultheis, L.; Kuhl, J. Physical Review B, Vol. 40, Issue 9 https://doi.org/10.1103/PhysRevB.40.6442	journal	September 1989
Quantum Optics Scully, Marlan O.; Zubairy, M. Suhail Cambridge University Press https://doi.org/10.1017/CBO9780511813993	book	January 2012
Quantum Optics Walls, D. F.; Milburn, G. J.; Garrison, John C. American Journal of Physics, Vol. 63, Issue 5 https://doi.org/10.1119/1.17886	journal	May 1995
Quantum Optics Walls, Daniel F.; Milburn, Gerard J.; Schleich, Wolfgang P. Physics Today, Vol. 48, Issue 6 https://doi.org/10.1063/1.2808065	journal	June 1995
Resonance lineshapes in two-dimensional Fourier transform spectroscopy Siemens, Mark E.; Moody, Galan; Li, Hebin Frontiers in Optics 2010/Laser Science XXVI https://doi.org/10.1364/ls.2010.ltha3	conference	January 2010
Evolution of Electronic Structure in Atomically Thin Sheets of WS2 and WSe2 Zhao, Weijie; Ghorannevis, Zohreh; Chua, Leiqiang arXiv https://doi.org/10.48550/arxiv.1212.5415	text	January 2012
Optical dephasing of homogeneously broadened two-dimensional exciton transitions in GaAs quantum wells Schultheis, L.; Honold, A.; Kuhl, J. Physical Review B, Vol. 34, Issue 12 https://doi.org/10.1103/physrevb.34.9027	journal	December 1986
Optical Generation of Excitonic Valley Coherence in Monolayer WSe2 Jones, Aaron Mitchell; Yu, Hongyi; Ghimire, Nirmal arXiv https://doi.org/10.48550/arxiv.1303.5318	text	January 2013
Exciton Binding Energy and Nonhydrogenic Rydberg Series in Monolayer WS2 Chernikov, Alexey; Berkelbach, Timothy C.; Hill, Heather M. arXiv https://doi.org/10.48550/arxiv.1403.4270	text	January 2014
Observation of Long-Lived Interlayer Excitons in Monolayer MoSe2-WSe2 Heterostructures Rivera, Pasqual; Schaibley, John R.; Jones, Aaron M. arXiv https://doi.org/10.48550/arxiv.1403.4985	text	January 2014
Low-temperature photocarrier dynamics in monolayer MoS2 Korn, Tobias; Heydrich, Stefanie; Hirmer, Michael Universität Regensburg https://doi.org/10.5283/epub.26514	text	January 2011

Cited By (115)

High-Quality Whispering-Gallery-Mode Lasing from Cesium Lead Halide Perovskite Nanoplatelets Zhang, Qing; Su, Rui; Liu, Xinfeng Advanced Functional Materials, Vol. 26, Issue 34 https://doi.org/10.1002/adfm.201601690	journal	July 2016
Ultrafast Laser Spectroscopy of Two-Dimensional Materials Beyond Graphene Ceballos, Frank; Zhao, Hui Advanced Functional Materials, Vol. 27, Issue 19 https://doi.org/10.1002/adfm.201604509	journal	December 2016
Continuous Control and Enhancement of Excitonic Valley Polarization in Monolayer WSe ₂ by Electrostatic Doping Shinokita, Keisuke; Wang, Xiaofan; Miyauchi, Yuhei Advanced Functional Materials, Vol. 29, Issue 26 https://doi.org/10.1002/adfm.201900260	journal	March 2019
Experimental Evidence of Anisotropic and Stable Charged Excitons (Trions) in Atomically Thin 2D ReS ₂ Wang, Xiaofan; Shinokita, Keisuke; Miyauchi, Yuhei Advanced Functional Materials, Vol. 29, Issue 51 https://doi.org/10.1002/adfm.201905961	journal	October 2019
Exciton-Plasmon Coupling and Electromagnetically Induced Transparency in Monolayer Semiconductors Hybridized with Ag Nanoparticles Zhao, Weijie; Wang, Shunfeng; Liu, Bo Advanced Materials, Vol. 28, Issue 14 https://doi.org/10.1002/adma.201504478	journal	February 2016
Engineering Bandgaps of Monolayer MoS ₂ and WS ₂ on Fluoropolymer Substrates by Electrostatically Tuned Many-Body Effects Liu, Bo; Zhao, Weijie; Ding, Zijing Advanced Materials, Vol. 28, Issue 30 https://doi.org/10.1002/adma.201504876	journal	May 2016
Multidimensional Coherent Spectroscopy of Semiconductors Smallwood, Christopher L.; Cundiff, Steven T. Laser & Photonics Reviews, Vol. 12, Issue 12 https://doi.org/10.1002/lpor.201800171	journal	November 2018
Ultra‐Long Lifetimes of Single Quantum Emitters in Monolayer WSe ₂ /hBN Heterostructures Dass, Chandriker Kavir; Khan, Mahtab A.; Clark, Genevieve Advanced Quantum Technologies, Vol. 2, Issue 5-6 https://doi.org/10.1002/qute.201900022	journal	April 2019
Environmental engineering of transition metal dichalcogenide optoelectronics LaMountain, Trevor; Lenferink, Erik J.; Chen, Yen-Jung Frontiers of Physics, Vol. 13, Issue 4 https://doi.org/10.1007/s11467-018-0795-x	journal	June 2018
Effect of Phonons on Valley Depolarization in Monolayer WSe2 Chellappan, Vijila; Pang, Ai Lin Christina; Sarkar, Soumya Electronic Materials Letters, Vol. 14, Issue 6 https://doi.org/10.1007/s13391-018-0086-2	journal	July 2018
Excitonic linewidth and coherence lifetime in monolayer transition metal dichalcogenides Selig, Malte; Berghäuser, Gunnar; Raja, Archana Nature Communications, Vol. 7, Issue 1 https://doi.org/10.1038/ncomms13279	journal	November 2016
Enabling valley selective exciton scattering in monolayer WSe2 through upconversion Manca, M.; Glazov, M. M.; Robert, C. Nature Communications, Vol. 8, Issue 1 https://doi.org/10.1038/ncomms14927	journal	April 2017
Valley-addressable polaritons in atomically thin semiconductors Dufferwiel, S.; Lyons, T. P.; Solnyshkov, D. D. Nature Photonics, Vol. 11, Issue 8 https://doi.org/10.1038/nphoton.2017.125	journal	July 2017
Optical manipulation of valley pseudospin Ye, Ziliang; Sun, Dezheng; Heinz, Tony F. Nature Physics, Vol. 13, Issue 1 https://doi.org/10.1038/nphys3891	journal	September 2016
Ultrafast quantum beats of anisotropic excitons in atomically thin ReS2 Sim, Sangwan; Lee, Doeon; Trifonov, Artur V. Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-017-02802-8	journal	January 2018
Inverted valley polarization in optically excited transition metal dichalcogenides Berghäuser, Gunnar; Bernal-Villamil, Ivan; Schmidt, Robert Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-03354-1	journal	March 2018
Giant optical nonlinearities from Rydberg excitons in semiconductor microcavities Walther, Valentin; Johne, Robert; Pohl, Thomas Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-03742-7	journal	April 2018
Two-dimensional semiconductors in the regime of strong light-matter coupling Schneider, Christian; Glazov, Mikhail M.; Korn, Tobias Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-04866-6	journal	July 2018
Evidence for line width and carrier screening effects on excitonic valley relaxation in 2D semiconductors Miyauchi, Yuhei; Konabe, Satoru; Wang, Feijiu Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-04988-x	journal	July 2018
Many-body simulation of two-dimensional electronic spectroscopy of excitons and trions in monolayer transition metal dichalcogenides Tempelaar, Roel; Berkelbach, Timothy C. Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-11497-y	journal	July 2019
Carrier multiplication in van der Waals layered transition metal dichalcogenides Kim, Ji-Hee; Bergren, Matthew R.; Park, Jin Cheol Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-13325-9	journal	December 2019
Polarized resonant emission of monolayer WS2 coupled with plasmonic sawtooth nanoslit array Han, Chunrui; Ye, Jianting Nature Communications, Vol. 11, Issue 1 https://doi.org/10.1038/s41467-020-14597-2	journal	February 2020
Exchange-driven intravalley mixing of excitons in monolayer transition metal dichalcogenides Guo, Liang; Wu, Meng; Cao, Ting Nature Physics, Vol. 15, Issue 3 https://doi.org/10.1038/s41567-018-0362-y	journal	December 2018
Quantum interference in second-harmonic generation from monolayer WSe2 Lin, Kai-Qiang; Bange, Sebastian; Lupton, John M. Nature Physics, Vol. 15, Issue 3 https://doi.org/10.1038/s41567-018-0384-5	journal	January 2019
Exciton Relaxation Cascade in two-dimensional Transition Metal Dichalcogenides Brem, Samuel; Selig, Malte; Berghaeuser, Gunnar Scientific Reports, Vol. 8, Issue 1 https://doi.org/10.1038/s41598-018-25906-7	journal	May 2018
Study on photoelectric characteristics of monolayer WS ₂ films Wang, Lin; Wang, Wenyan; Wang, Quan RSC Advances, Vol. 9, Issue 64 https://doi.org/10.1039/c9ra07924f	journal	January 2019
Realization of an all optical exciton-polariton router Marsault, Félix; Nguyen, Hai Son; Tanese, Dimitrii Applied Physics Letters, Vol. 107, Issue 20 https://doi.org/10.1063/1.4936158	journal	November 2015
Exciton valley dynamics in monolayer Mo _1-x W _x Se ₂ (x = 0, 0.5, 1) Ye, Jialiang; Niu, Binghui; Li, Ying Applied Physics Letters, Vol. 111, Issue 15 https://doi.org/10.1063/1.4995517	journal	October 2017
The interplay between excitons and trions in a monolayer of MoSe ₂ Lundt, N.; Cherotchenko, E.; Iff, O. Applied Physics Letters, Vol. 112, Issue 3 https://doi.org/10.1063/1.5019177	journal	January 2018
Modulation of THz radiation via enhanced Dirac plasmon-dual phonon interaction Lu, Junpeng; Liu, Hongwei; Yu, Yuanfang Applied Physics Letters, Vol. 115, Issue 25 https://doi.org/10.1063/1.5128891	journal	December 2019
Advances in multi-dimensional coherent spectroscopy of semiconductor nanostructures Moody, Galan; Cundiff, Steven T. Advances in Physics: X, Vol. 2, Issue 3 https://doi.org/10.1080/23746149.2017.1346482	journal	May 2017
Dynamical screening in monolayer transition-metal dichalcogenides and its manifestations in the exciton spectrum Scharf, Benedikt; Van Tuan, Dinh; Žutić, Igor Journal of Physics: Condensed Matter, Vol. 31, Issue 20 https://doi.org/10.1088/1361-648x/ab071f	journal	March 2019
Nonequilibrium carrier dynamics in transition metal dichalcogenide semiconductors Steinhoff, A.; Florian, M.; Rösner, M. 2D Materials, Vol. 3, Issue 3 https://doi.org/10.1088/2053-1583/3/3/031006	journal	August 2016
Many-body effects in nonlinear optical responses of 2D layered semiconductors Aivazian, Grant; Yu, Hongyi; Wu, Sanfeng 2D Materials, Vol. 4, Issue 2 https://doi.org/10.1088/2053-1583/aa56f1	journal	February 2017
Unconventional electroabsorption in monolayer MoS ₂ Vella, D.; Ovchinnikov, D.; Martino, N. 2D Materials, Vol. 4, Issue 2 https://doi.org/10.1088/2053-1583/aa5784	journal	January 2017
Approaching the intrinsic photoluminescence linewidth in transition metal dichalcogenide monolayers Ajayi, Obafunso A.; Ardelean, Jenny V.; Shepard, Gabriella D. 2D Materials, Vol. 4, Issue 3 https://doi.org/10.1088/2053-1583/aa6aa1	journal	July 2017
Exciton broadening and band renormalization due to Dexter-like intervalley coupling Bernal-Villamil, Ivan; Berghäuser, Gunnar; Selig, Malte 2D Materials, Vol. 5, Issue 2 https://doi.org/10.1088/2053-1583/aaaa8b	journal	February 2018
High optical quality of MoS ₂ monolayers grown by chemical vapor deposition Shree, Shivangi; George, Antony; Lehnert, Tibor 2D Materials, Vol. 7, Issue 1 https://doi.org/10.1088/2053-1583/ab4f1f	journal	November 2019
Roadmap on finding chiral valleys: screening 2D materials for valleytronics Bussolotti, Fabio; Kawai, Hiroyo; Ooi, Zi En Nano Futures, Vol. 2, Issue 3 https://doi.org/10.1088/2399-1984/aac9d7	journal	June 2018
Excitonic magneto-optics in monolayer transition metal dichalcogenides: From nanoribbons to two-dimensional response Have, J.; Peres, N. M. R.; Pedersen, T. G. Physical Review B, Vol. 100, Issue 4 https://doi.org/10.1103/physrevb.100.045411	journal	July 2019
Theory of second-order excitonic nonlinearities in transition metal dichalcogenides Mkrtchian, Garnik F.; Knorr, Andreas; Selig, Malte Physical Review B, Vol. 100, Issue 12 https://doi.org/10.1103/physrevb.100.125401	journal	September 2019
Valley trion dynamics in monolayer ${MoSe}_{2}$ Gao, Feng; Gong, Yongji; Titze, Michael Physical Review B, Vol. 94, Issue 24 https://doi.org/10.1103/physrevb.94.245413	journal	December 2016
Complexes of dipolar excitons in layered quasi-two-dimensional nanostructures Bondarev, Igor V.; Vladimirova, Maria R. Physical Review B, Vol. 97, Issue 16 https://doi.org/10.1103/physrevb.97.165419	journal	April 2018
Mapping of the dark exciton landscape in transition metal dichalcogenides Berghäuser, Gunnar; Steinleitner, Philipp; Merkl, Philipp Physical Review B, Vol. 98, Issue 2 https://doi.org/10.1103/physrevb.98.020301	journal	July 2018
Fundamental exciton linewidth broadening in monolayer transition metal dichalcogenides Gupta, Garima; Majumdar, Kausik Physical Review B, Vol. 99, Issue 8 https://doi.org/10.1103/physrevb.99.085412	journal	February 2019
Layer degree of freedom for excitons in transition metal dichalcogenides Das, Sarthak; Gupta, Garima; Majumdar, Kausik Physical Review B, Vol. 99, Issue 16 https://doi.org/10.1103/physrevb.99.165411	journal	April 2019
Enhanced screening and spectral diversity in many-body elastic scattering of excitons in two-dimensional hybrid metal-halide perovskites Thouin, Félix; Cortecchia, Daniele; Petrozza, Annamaria Physical Review Research, Vol. 1, Issue 3 https://doi.org/10.1103/physrevresearch.1.032032	journal	December 2019
Deconvolution of optical multidimensional coherent spectra Richter, Marten; Singh, Rohan; Siemens, Mark Science Advances, Vol. 4, Issue 6 https://doi.org/10.1126/sciadv.aar7697	journal	June 2018
Room temperature nanocavity laser with interlayer excitons in 2D heterostructures Liu, Yuanda; Fang, Hanlin; Rasmita, Abdullah Science Advances, Vol. 5, Issue 4 https://doi.org/10.1126/sciadv.aav4506	journal	April 2019
Broadband two-dimensional electronic spectroscopy in an actively phase stabilized pump-probe configuration Zhu, Weida; Wang, Rui; Zhang, Chunfeng Optics Express, Vol. 25, Issue 18 https://doi.org/10.1364/oe.25.021115	journal	January 2017
Chiral light-matter interactions using spin-valley states in transition metal dichalcogenides Yang, Zhili; Aghaeimeibodi, Shahriar; Waks, Edo Optics Express, Vol. 27, Issue 15 https://doi.org/10.1364/oe.27.021367	journal	January 2019
Observation of 2D semiconductor P-type dark-exciton lifetime using two-photon ultrafast spectroscopy Panna, Dmitry; Balasubramanian, Krishna; Khatei, Jayakrishna Optics Express, Vol. 27, Issue 23 https://doi.org/10.1364/oe.27.033427	journal	January 2019
Single-scan acquisition of multiple multidimensional spectra Autry, Travis M.; Moody, Galan; Fraser, James Optica, Vol. 6, Issue 6 https://doi.org/10.1364/optica.6.000735	journal	January 2019
Engineering Valley Polarization of Monolayer WS ₂ : A Physical Doping Approach Feng, Shun; Cong, Chunxiao; Konabe, Satoru Small, Vol. 15, Issue 12 https://doi.org/10.1002/smll.201805503	journal	February 2019
Direct optical-structure correlation in atomically thin dichalcogenides and heterostructures Singh, Akshay; Lee, Hae Yeon; Gradečak, Silvija Nano Research, Vol. 13, Issue 5 https://doi.org/10.1007/s12274-019-2601-7	journal	January 2020
Valleytronics in 2D materials Schaibley, John R.; Yu, Hongyi; Clark, Genevieve Nature Reviews Materials, Vol. 1, Issue 11 https://doi.org/10.1038/natrevmats.2016.55	journal	August 2016
Cascaded emission of single photons from the biexciton in monolayered WSe2 He, Yu-Ming; Iff, Oliver; Lundt, Nils Nature Communications, Vol. 7, Issue 1 https://doi.org/10.1038/ncomms13409	journal	November 2016
Directional interlayer spin-valley transfer in two-dimensional heterostructures Schaibley, John R.; Rivera, Pasqual; Yu, Hongyi Nature Communications, Vol. 7, Issue 1 https://doi.org/10.1038/ncomms13747	journal	December 2016
Slow cooling and efficient extraction of C-exciton hot carriers in MoS2 monolayer Wang, Lei; Wang, Zhuo; Wang, Hai-Yu Nature Communications, Vol. 8, Issue 1 https://doi.org/10.1038/ncomms13906	journal	January 2017
Direct measurement of exciton valley coherence in monolayer WSe2 Hao, Kai; Moody, Galan; Wu, Fengcheng Nature Physics, Vol. 12, Issue 7 https://doi.org/10.1038/nphys3674	journal	February 2016
The valley Zeeman effect in inter- and intra-valley trions in monolayer WSe2 Lyons, T. P.; Dufferwiel, S.; Brooks, M. Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-10228-7	journal	May 2019
Ultrafast dynamics in van der Waals heterostructures Jin, Chenhao; Ma, Eric Yue; Karni, Ouri Nature Nanotechnology, Vol. 13, Issue 11 https://doi.org/10.1038/s41565-018-0298-5	journal	November 2018
Biexcitonic optical Stark effects in monolayer molybdenum diselenide Yong, Chaw-Keong; Horng, Jason; Shen, Yuxia Nature Physics, Vol. 14, Issue 11 https://doi.org/10.1038/s41567-018-0216-7	journal	July 2018
Direct exciton emission from atomically thin transition metal dichalcogenide heterostructures near the lifetime limit Wierzbowski, Jakob; Klein, Julian; Sigger, Florian Scientific Reports, Vol. 7, Issue 1 https://doi.org/10.1038/s41598-017-09739-4	journal	September 2017
Polarimetry of photon echo on charged and neutral excitons in semiconductor quantum wells Poltavtsev, S. V.; Kapitonov, Yu. V.; Yugova, I. A. Scientific Reports, Vol. 9, Issue 1 https://doi.org/10.1038/s41598-019-42208-8	journal	April 2019
Physics of excitons and their transport in two dimensional transition metal dichalcogenide semiconductors Kaviraj, Bhaskar; Sahoo, Dhirendra RSC Advances, Vol. 9, Issue 44 https://doi.org/10.1039/c9ra03769a	journal	January 2019
Spin–flip processes and radiative decay of dark intravalley excitons in transition metal dichalcogenide monolayers Slobodeniuk, A. O.; Basko, D. M. 2D Materials, Vol. 3, Issue 3 https://doi.org/10.1088/2053-1583/3/3/035009	journal	August 2016
Impact of environment on dynamics of exciton complexes in a WS ₂ monolayer Jakubczyk, Tomasz; Nogajewski, Karol; Molas, Maciej R. 2D Materials, Vol. 5, Issue 3 https://doi.org/10.1088/2053-1583/aabc1c	journal	April 2018
Dark and bright exciton formation, thermalization, and photoluminescence in monolayer transition metal dichalcogenides Selig, Malte; Berghäuser, Gunnar; Richter, Marten 2D Materials, Vol. 5, Issue 3 https://doi.org/10.1088/2053-1583/aabea3	journal	May 2018
Exciton–phonon coupling in mono- and bilayer MoTe ₂ Helmrich, Sophia; Schneider, Robert; Achtstein, Alexander W. 2D Materials, Vol. 5, Issue 4 https://doi.org/10.1088/2053-1583/aacfb7	journal	July 2018
Coupled exciton-trion spin dynamics in a MoSe ₂ monolayer Anghel, S.; Passmann, F.; Ruppert, C. 2D Materials, Vol. 5, Issue 4 https://doi.org/10.1088/2053-1583/aadbd8	journal	September 2018
Triple sum frequency pump-probe spectroscopy of transition metal dichalcogenides Morrow, Darien J.; Kohler, Daniel D.; Zhao, Yuzhou Physical Review B, Vol. 100, Issue 23 https://doi.org/10.1103/physrevb.100.235303	journal	December 2019
Oxygen Passivation Mediated Tunability of Trion and Excitons in ${MoS}_{2}$ Gogoi, Pranjal Kumar; Hu, Zhenliang; Wang, Qixing Physical Review Letters, Vol. 119, Issue 7 https://doi.org/10.1103/physrevlett.119.077402	journal	August 2017
Valley Trion Dynamics in Monolayer MoSe2 Titze, Michael; Gao, Feng; Almeida, Raybel Frontiers in Optics 2016 https://doi.org/10.1364/fio.2016.jw4a.192	conference	January 2016
Engineering radiative coupling of excitons in 2D semiconductors Horng, Jason; Chou, Yu-Hsun; Chang, Tsu-Chi Optica, Vol. 6, Issue 11 https://doi.org/10.1364/optica.6.001443	journal	January 2019
Enhancing functionalities of atomically thin semiconductors with plasmonic nanostructures Cotrufo, Michele; Sun, Liuyang; Choi, Junho Nanophotonics, Vol. 8, Issue 4 https://doi.org/10.1515/nanoph-2018-0185	journal	March 2019
Dielectric Properties of NbxW1-xSe2 Alloys Rigosi, Albert F.; Hill, Heather; Krylyuk, Sergiy Journal of Research of the National Institute of Standards and Technology, Vol. 124 https://doi.org/10.6028/jres.124.035	journal	January 2019
Tuning the Fröhlich exciton-phonon scattering in monolayer MoS2 Miller, Bastian; Lindlau, Jessica; Bommert, Max Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-08764-3	journal	February 2019
Interlayer exciton dynamics in van der Waals heterostructures Ovesen, Simon; Brem, Samuel; Linderälv, Christopher Communications Physics, Vol. 2, Issue 1 https://doi.org/10.1038/s42005-019-0122-z	journal	February 2019
Coherent two-dimensional Fourier transform spectroscopy using a 25 Tesla resistive magnet Paul, Jagannath; Stevens, Christopher. E.; Smith, Ryan P. Review of Scientific Instruments, Vol. 90, Issue 6 https://doi.org/10.1063/1.5055891	journal	June 2019
Monolayered MoSe ₂ : a candidate for room temperature polaritonics Lundt, N.; Maryński, A.; Cherotchenko, E. 2D Materials, Vol. 4, Issue 1 https://doi.org/10.1088/2053-1583/4/1/015006	journal	October 2016
Optical nonlinearities of excitons in monolayer ${MoS}_{2}$ Soh, Daniel B. S.; Rogers, Christopher; Gray, Dodd J. Physical Review B, Vol. 97, Issue 16 https://doi.org/10.1103/physrevb.97.165111	journal	April 2018
Excitonic linewidth and coherence lifetime in monolayer transition metal dichalcogenides Selig, Malte; Berghäuser, Gunnar; Raja, Archana SPIE OPTO, SPIE Proceedings https://doi.org/10.1117/12.2252486	conference	February 2017
Polarimetry of photon echo on charged and neutral excitons in semiconductor quantum wells Poltavtsev, Sergey V.; Akimov, Ilya A.; Yakovlev, Dmitri R. Technische Universität Dortmund https://doi.org/10.17877/de290r-20152	text	January 2019
Valley-polarized exciton–polaritons in a monolayer semiconductor Chen, Yen-Jung; Cain, Jeffrey D.; Stanev, Teodor K. Nature Photonics, Vol. 11, Issue 7 https://doi.org/10.1038/nphoton.2017.86	journal	June 2017
2D semiconductor nonlinear plasmonic modulators Klein, Matthew; Badada, Bekele H.; Binder, Rolf Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-11186-w	journal	July 2019
Exciton physics and device application of two-dimensional transition metal dichalcogenide semiconductors Mueller, Thomas; Malic, Ermin npj 2D Materials and Applications, Vol. 2, Issue 1 https://doi.org/10.1038/s41699-018-0074-2	journal	September 2018
Ultrafast nonequilibrium dynamics of strongly coupled resonances in the intrinsic cavity of $W S_{2}$ nanotubes Višić, Bojana; Yadgarov, Lena; Pogna, Eva A. A. Physical Review Research, Vol. 1, Issue 3 https://doi.org/10.1103/physrevresearch.1.033046	journal	October 2019
Quantum interference in second-harmonic generation from monolayer WSe2 Lin, Kai-Qiang; Bange, Sebastian; Lupton, John M. Universität Regensburg https://doi.org/10.5283/epub.40543	text	January 2019
Trion valley coherence in monolayer semiconductors Hao, Kai; Xu, Lixiang; Wu, Fengcheng 2D Materials, Vol. 4, Issue 2 https://doi.org/10.1088/2053-1583/aa70f9	journal	May 2017
Theory of Two-Dimensional Spatially Indirect Equilibrium Exciton Condensates Wu, Feng-Cheng; Xue, Fei; MacDonald, A. H. arXiv https://doi.org/10.48550/arxiv.1506.01947	text	January 2015
Trion Formation Dynamics in Monolayer Transition Metal Dichalcogenides Singh, Akshay; Moody, Galan; Tran, Kha arXiv https://doi.org/10.48550/arxiv.1507.04463	text	January 2015
Exciton-plasmon Coupling and Electromagnetically Induced Transparency in Monolayer Semiconductors Hybridized with Ag Nanoparticles Weijie, Zhao; Shunfeng, Wang; Bo, Liu arXiv https://doi.org/10.48550/arxiv.1601.05573	text	January 2016
Exciton Radiative Lifetime in Transition Metal Dichalcogenide Monolayers Robert, C.; Lagarde, D.; Cadiz, F. arXiv https://doi.org/10.48550/arxiv.1603.00277	text	January 2016
Nonequilibrium Carrier Dynamics in Transition Metal Dichalcogenide Semiconductors Steinhoff, Alexander; Florian, Matthias; Rösner, Malte arXiv https://doi.org/10.48550/arxiv.1603.03633	text	January 2016
Two-dimensional Fröhlich interaction in transition-metal dichalcogenide monolayers: Theoretical modeling and first-principles calculations Sohier, Thibault; Calandra, Matteo; Mauri, Francesco arXiv https://doi.org/10.48550/arxiv.1605.08207	text	January 2016
Probing Many-Body Interactions in Monolayer Transition-Metal Dichalcogenides Van Tuan, Dinh; Scharf, Benedikt; Wang, Zefang arXiv https://doi.org/10.48550/arxiv.1606.07101	text	January 2016
Exciton-phonon relaxation bottleneck and radiative decay of thermal exciton reservoir in two-dimensional materials Slobodeniuk, A. O.; Basko, D. M. arXiv https://doi.org/10.48550/arxiv.1606.08213	text	January 2016
Many-body effects in nonlinear optical responses of 2D layered semiconductors Aivazian, Grant; Yu, Hongyi; Wu, Sanfeng arXiv https://doi.org/10.48550/arxiv.1612.02714	text	January 2016
Impact of environment on dynamics of exciton complexes in a WS$_2$ monolayer Jakubczyk, T.; Nogajewski, K.; Molas, M. R. arXiv https://doi.org/10.48550/arxiv.1709.02658	preprint	January 2017
Exciton Relaxation Cascade in Two-dimensional Transition-metal dichalcogenides Brem, Samuel; Berghaeuser, Gunnar; Selig, Malte arXiv https://doi.org/10.48550/arxiv.1712.04808	text	January 2017
Complexes of dipolar excitons in layered quasi-two-dimensional nanostructures Bondarev, Igor V.; Vladimirova, Maria R. arXiv https://doi.org/10.48550/arxiv.1712.10312	text	January 2017
Dynamical screening in monolayer transition-metal dichalcogenides and its manifestations in the exciton spectrum Scharf, Benedikt; Van Tuan, Dinh; Žutić, Igor arXiv https://doi.org/10.48550/arxiv.1801.06217	text	January 2018
Two-dimensional semiconductors in the regime of strong light-matter coupling Schneider, Christian; Glazov, Mikhail M.; Korn, Tobias arXiv https://doi.org/10.48550/arxiv.1804.06771	text	January 2018
Virtual trions in the photoluminescence of monolayer transition-metal dichalcogenides Van Tuan, Dinh; Jones, Aaron M.; Yang, Min arXiv https://doi.org/10.48550/arxiv.1805.08722	text	January 2018
Fundamental exciton linewidth broadening in monolayer transition metal dichalcogenides Gupta, Garima; Majumdar, Kausik arXiv https://doi.org/10.48550/arxiv.1901.04391	text	January 2019
Controlling excitons in an atomically thin membrane with a mirror Zhou, You; Scuri, Giovanni; Sung, Jiho arXiv https://doi.org/10.48550/arxiv.1901.08500	text	January 2019
Intrinsic Lifetime of Higher Excitonic States in Tungsten Diselenide Monolayers Brem, Samuel; Zipfel, Jonas; Selig, Malte arXiv https://doi.org/10.48550/arxiv.1904.04729	text	January 2019
Chiral light-matter interactions using spin-valley states in transition metal dichalcogenides Yang, Zhili; Aghaeimeibodi, Shahriar; Waks, Edo arXiv https://doi.org/10.48550/arxiv.1904.12349	text	January 2019
Enhanced screening and spectral diversity in many-body elastic scattering of excitons in two-dimensional hybrid metal-halide perovskites Thouin, Félix; Cortecchia, Daniele; Petrozza, Annamaria arXiv https://doi.org/10.48550/arxiv.1904.12402	text	January 2019
Excitonic magneto-optics in monolayer transition metal dichalcogenides: From nanoribbons to two-dimensional response Have, J.; Peres, N. M. R.; Pedersen, T. G. arXiv https://doi.org/10.48550/arxiv.1905.06651	text	January 2019
Room temperature nanocavity laser with interlayer excitons in 2D heterostructures Liu, Yuanda; Fang, Hanlin; Rasmita, Abdullah arXiv https://doi.org/10.48550/arxiv.1911.12629	preprint	January 2019
Mapping of the dark exciton landscape in transition metal dichalcogenides Berghäuser, Gunnar; Steinleitner, Philipp; Merkl, Philipp Universität Regensburg https://doi.org/10.5283/epub.37987	text	January 2018
Enabling valley selective exciton scattering in monolayer WSe$_2$ through upconversion Manca, M.; Glazov, M. M.; Robert, C. arXiv https://doi.org/10.48550/arxiv.1701.05800	text	January 2017
Encapsulation Narrows Excitonic Homogeneous Linewidth of Exfoliated MoSe$_2$ Monolayer Martin, Eric W.; Horng, Jason; Ruth, Hanna G. arXiv https://doi.org/10.48550/arxiv.1810.09834	text	January 2018

Similar Records

Excitonic linewidth and coherence lifetime in monolayer transition metal dichalcogenides

Journal Article · Mon Nov 07 00:00:00 EST 2016 · Nature Communications · OSTI ID:1441157

Selig, Malte; Berghäuser, Gunnar; Raja, Archana; +7 more

Population Pulsation Resonances of Excitons in Monolayer MoSe₂ with Sub-1 μeV Linewidths

Journal Article · Wed Apr 01 00:00:00 EDT 2015 · Physical Review Letters · OSTI ID:1441157

Schaibley, John R.; Karin, Todd; Yu, Hongyi; +9 more

Intrinsic donor-bound excitons in ultraclean monolayer semiconductors

Journal Article · Mon Feb 08 00:00:00 EST 2021 · Nature Communications · OSTI ID:1441157

Rivera, Pasqual; He, Minhao; Kim, Bumho; +16 more

Related Subjects

36 MATERIALS SCIENCE

Title: Intrinsic homogeneous linewidth and broadening mechanisms of excitons in monolayer transition metal dichalcogenides

Citation Formats

References (40)

Cited By (115)

Similar Records

Related Subjects