High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion

Kraus, D.; Hartley, N. J.; Frydrych, S.; Schuster, A. K.; Rohatsch, K.; Rodel, M.; Cowan, T. E.; Brown, S.; Cunningham, E.; van Driel, T.; Fletcher, L. B.; Galtier, E.; Gamboa, E. J.; Laso Garcia, A.; Gericke, D. O.; Granados, E.; Heimann, P. A.; Lee, H. J.; MacDonald, M. J.; MacKinnon, A. J.; McBride, E. E.; Nam, I.; Neumayer, P.; Pak, A.; Pelka, A.; Prencipe, I.; Ravasio, A.; Redmer, R.; Saunders, A. M.; Scholmerich, M.; Schorner, M.; Sun, P.; Turner, S. J.; Zettl, A.; Falcone, R. W.; Glenzer, S. H.; Doppner, T.; Vorberger, J.

doi:10.1063/1.5017908

Title: High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion

Journal Article · Wed May 23 00:00:00 EDT 2018 · Physics of Plasmas

DOI:https://doi.org/10.1063/1.5017908· OSTI ID:1458534

^[1];

^[2]; Frydrych, S. ^[3]; Schuster, A. K. ^[4]; Rohatsch, K. ^[4]; Rodel, M. ^[4];

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^[5]; Cunningham, E. ^[5];

^[5]; Fletcher, L. B. ^[5]; Galtier, E. ^[5]; Gamboa, E. J. ^[5];

^[4]; Gericke, D. O. ^[6]; Granados, E. ^[5]; Heimann, P. A. ^[5]; Lee, H. J. ^[5];

^[7]; MacKinnon, A. J. ^[5] more »

Helmholtz-Zentrum Dresden-Rossendorf, Dresden (Germany); Technische Univ. Dresden, Dresden (Germany)
Helmholtz-Zentrum Dresden-Rossendorf, Dresden (Germany); Osaka Univ., Osaka (Japan)
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Technische Univ. Darmstadt, Darmstadt (Germany)
Helmholtz-Zentrum Dresden-Rossendorf, Dresden (Germany)
SLAC National Accelerator Lab., Menlo Park, CA (United States)
Univ. of Warwick, Coventry (United Kingdom)
Univ. of California, Berkeley, CA (United States); Univ. of Michigan, Ann Arbor, MI (United States)
SLAC National Accelerator Lab., Menlo Park, CA (United States); European XFEL GmbH, Schenefeld (Germany)
GSI Helmholtzzentrum fur Schwerionenforschung GmbH, Darmstadt (Germany)
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Univ. Paris VI-Ecole Polytechnique, Palaiseau Cedex (France)
Univ. Rostock, Rostock (Germany)
Univ. of California, Berkeley, CA (United States)
European XFEL GmbH, Schenefeld (Germany)
SLAC National Accelerator Lab., Menlo Park, CA (United States); Univ. Rostock, Rostock (Germany)
Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)

Diamond formation in polystyrene (C8H8)n, which is laser-compressed and heated to conditions around 150 GPa and 5000 K, has recently been demonstrated in the laboratory [Kraus et al., Nat. Astron. 1, 606-611 (2017)]. Here, we show an extended analysis and comparison to first-principles simulations of the acquired data and their implications for planetary physics and inertial confinement fusion. Moreover, we discuss the advanced diagnostic capabilities of adding high-quality small angle X-ray scattering and spectrally resolved X-ray scattering to the platform, which shows great prospects of precisely studying the kinetics of chemical reactions in dense plasma environments at pressures exceeding 100 GPa.

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Research Organization:: SLAC National Accelerator Lab., Menlo Park, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Fusion Energy Sciences (FES)

Grant/Contract Number:: AC02-76SF00515; FOR 2440; AC02-05CH11231; AC52-07NA27344; FG52-10NA29649; NA0001859; FWP-100182; SF-00515; 05P15RDFA1; 18-ERD- 033; FA9550-14-1-0323; 16K17846; VH-NG-1141

OSTI ID:: 1458534

Alternate ID(s):: OSTI ID: 1438512; OSTI ID: 1461991

Journal Information:: Physics of Plasmas, Vol. 25, Issue 5; ISSN 1070-664X

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

Citation Metrics:

Cited by: 19 works

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Evidence for Crystalline Structure in Dynamically-Compressed Polyethylene up to 200 GPa Hartley, N. J.; Brown, S.; Cowan, T. E. Scientific Reports, Vol. 9, Issue 1 https://doi.org/10.1038/s41598-019-40782-5	journal	March 2019
Measurement of diamond nucleation rates from hydrocarbons at conditions comparable to the interiors of icy giant planets Schuster, A. K.; Hartley, N. J.; Vorberger, J. GSI Helmholtzzentrum fuer Schwerionenforschung, GSI, Darmstadt https://doi.org/10.15120/gsi-2020-00340	text	January 2020

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