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Title: Fe Stabilization by Intermetallic L1 0-FePt and Pt Catalysis Enhancement in L1 0-FePt/Pt Nanoparticles for Efficient Oxygen Reduction Reaction in Fuel Cells

Authors:
ORCiD logo [1]; ORCiD logo [1];  [2]; ORCiD logo [2];  [3]; ORCiD logo [4]; ORCiD logo [5]; ORCiD logo [1];  [1]; ORCiD logo [1]; ORCiD logo [2]; ORCiD logo [3]; ORCiD logo [1]
  1. Brown Univ., Providence, RI (United States). Dept. of Chemistry
  2. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
  3. Dalhousie Univ., Halifax, NS (Canada). Dept. of Chemistry
  4. Brookhaven National Lab. (BNL), Upton, NY (United States). Center for Functional Nanomaterials (CFN)
  5. Huazhong Univ. of Science and Technology, Hubei (People's Republic of China). School of Materials Science and Engineering
Publication Date:
Research Org.:
Brookhaven National Lab. (BNL), Upton, NY (United States); Argonne National Lab. (ANL), Argonne, IL (United States); Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22) Scientific User Facilities Division; USDOE Office of Energy Efficiency and Renewable Energy (EERE), Transportation Office. Fuel Cell Technologies Office; Canadian Light Sources, Inc., Saskatoon, SK (Canada); National Natural Science Foundation of China (NNSFC); Materials Genome Initiative
OSTI Identifier:
1438309
Alternate Identifier(s):
OSTI ID: 1461399
Report Number(s):
BNL-205665-2018-JAAM; LA-UR-18-20293
Journal ID: ISSN 0002-7863
Grant/Contract Number:  
SC0012704; AC52-06NA25396; AC02-06CH11357; 21603078; 2016YFB0700600
Resource Type:
Journal Article: Accepted Manuscript
Journal Name:
Journal of the American Chemical Society
Additional Journal Information:
Journal Volume: 140; Journal Issue: 8; Journal ID: ISSN 0002-7863
Publisher:
American Chemical Society (ACS)
Country of Publication:
United States
Language:
English
Subject:
29 ENERGY PLANNING, POLICY AND ECONOMY; L10-FePt; Oxygen Reduction Reaction; MPt alloy nanoparticle; Energy Sciences

Citation Formats

Li, Junrui, Xi, Zheng, Pan, Yung -Tin, Spendelow, Jacob S., Duchesne, Paul N., Su, Dong, Li, Qing, Yu, Chao, Yin, Zhouyang, Shen, Bo, Kim, Yu Seung, Zhang, Peng, and Sun, Shouheng. Fe Stabilization by Intermetallic L10-FePt and Pt Catalysis Enhancement in L10-FePt/Pt Nanoparticles for Efficient Oxygen Reduction Reaction in Fuel Cells. United States: N. p., 2018. Web. doi:10.1021/jacs.7b12829.
Li, Junrui, Xi, Zheng, Pan, Yung -Tin, Spendelow, Jacob S., Duchesne, Paul N., Su, Dong, Li, Qing, Yu, Chao, Yin, Zhouyang, Shen, Bo, Kim, Yu Seung, Zhang, Peng, & Sun, Shouheng. Fe Stabilization by Intermetallic L10-FePt and Pt Catalysis Enhancement in L10-FePt/Pt Nanoparticles for Efficient Oxygen Reduction Reaction in Fuel Cells. United States. doi:10.1021/jacs.7b12829.
Li, Junrui, Xi, Zheng, Pan, Yung -Tin, Spendelow, Jacob S., Duchesne, Paul N., Su, Dong, Li, Qing, Yu, Chao, Yin, Zhouyang, Shen, Bo, Kim, Yu Seung, Zhang, Peng, and Sun, Shouheng. Wed . "Fe Stabilization by Intermetallic L10-FePt and Pt Catalysis Enhancement in L10-FePt/Pt Nanoparticles for Efficient Oxygen Reduction Reaction in Fuel Cells". United States. doi:10.1021/jacs.7b12829. https://www.osti.gov/servlets/purl/1438309.
@article{osti_1438309,
title = {Fe Stabilization by Intermetallic L10-FePt and Pt Catalysis Enhancement in L10-FePt/Pt Nanoparticles for Efficient Oxygen Reduction Reaction in Fuel Cells},
author = {Li, Junrui and Xi, Zheng and Pan, Yung -Tin and Spendelow, Jacob S. and Duchesne, Paul N. and Su, Dong and Li, Qing and Yu, Chao and Yin, Zhouyang and Shen, Bo and Kim, Yu Seung and Zhang, Peng and Sun, Shouheng},
abstractNote = {},
doi = {10.1021/jacs.7b12829},
journal = {Journal of the American Chemical Society},
issn = {0002-7863},
number = 8,
volume = 140,
place = {United States},
year = {2018},
month = {2}
}

Journal Article:
Free Publicly Available Full Text
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Citation Metrics:
Cited by: 22 works
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Figures / Tables:

Figure 1 Figure 1: (A) TEM image of C-L10-FePt NPs. (B) 2D EELS elemental mapping image of L10-FePt NPs, where Fe is colored green and Pt is colored red. (C) STEM-EELS line scan of a L10FePt NP. (D) TEM image of C-L10-FePt/Pt NPs. (E) 2D EELS elemental mapping image a L10-FePt/Pt NP,more » where Fe is colored green and Pt is colored red. (F) STEM-EELS line scan of a L10FePt/Pt NP.« less

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Works referencing / citing this record:

Structurally Ordered Low‐Pt Intermetallic Electrocatalysts toward Durably High Oxygen Reduction Reaction Activity
journal, July 2019

  • Wang, Zhongxiang; Yao, Xiaozhang; Kang, Yongqiang
  • Advanced Functional Materials, Vol. 29, Issue 35
  • DOI: 10.1002/adfm.201902987

Highly active zigzag-like Pt-Zn alloy nanowires with high-index facets for alcohol electrooxidation
journal, April 2019


Pt-rare earth metal alloy/metal oxide catalysts for oxygen reduction and alcohol oxidation reactions: an overview
journal, January 2019

  • Peera, Shaik Gouse; Lee, Tae Gwan; Sahu, Akhila Kumar
  • Sustainable Energy & Fuels, Vol. 3, Issue 8
  • DOI: 10.1039/c9se00082h

The application of CeO 2 -based materials in electrocatalysis
journal, January 2019

  • Wang, Jianda; Xiao, Xiao; Liu, Yong
  • Journal of Materials Chemistry A, Vol. 7, Issue 30
  • DOI: 10.1039/c9ta04804a

Structurally Ordered Low‐Pt Intermetallic Electrocatalysts toward Durably High Oxygen Reduction Reaction Activity
journal, July 2019

  • Wang, Zhongxiang; Yao, Xiaozhang; Kang, Yongqiang
  • Advanced Functional Materials, Vol. 29, Issue 35
  • DOI: 10.1002/adfm.201902987

Highly active zigzag-like Pt-Zn alloy nanowires with high-index facets for alcohol electrooxidation
journal, April 2019


Pt-rare earth metal alloy/metal oxide catalysts for oxygen reduction and alcohol oxidation reactions: an overview
journal, January 2019

  • Peera, Shaik Gouse; Lee, Tae Gwan; Sahu, Akhila Kumar
  • Sustainable Energy & Fuels, Vol. 3, Issue 8
  • DOI: 10.1039/c9se00082h

The application of CeO 2 -based materials in electrocatalysis
journal, January 2019

  • Wang, Jianda; Xiao, Xiao; Liu, Yong
  • Journal of Materials Chemistry A, Vol. 7, Issue 30
  • DOI: 10.1039/c9ta04804a

    Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.