Stripes developed at the strong limit of nematicity in FeSe film

Li, Wei; Zhang, Yan; Deng, Peng; Xu, Zhilin; Mo, S. -K.; Yi, Ming; Ding, Hao; Hashimoto, M.; Moore, R. G.; Lu, D. -H.; Chen, Xi; Shen, Z. -X.; Xue, Qi-Kun

doi:10.1038/nphys4186

Title: Stripes developed at the strong limit of nematicity in FeSe film

Journal Article · Mon Jul 17 00:00:00 EDT 2017 · Nature Physics

DOI:https://doi.org/10.1038/nphys4186· OSTI ID:1425888

^[1]; Zhang, Yan ^[2]; Deng, Peng ^[3]; Xu, Zhilin ^[3];

^[4];

^[5]; Ding, Hao ^[3]; Hashimoto, M. ^[6]; Moore, R. G. ^[5];

^[6]; Chen, Xi ^[7];

^[8]; Xue, Qi-Kun ^[7]

Tsinghua Univ., Beijing (China). State Key Lab. of Low-Dimensional Quantum Physics. Dept. of Physics; Collaborative Innovation Center of Quantum Matter, Beijing (China); SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., CA (United States). Stanford Inst. for Materials and Energy Sciences
Collaborative Innovation Center of Quantum Matter, Beijing (China); SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., CA (United States). Stanford Inst. for Materials and Energy Sciences; Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source; Peking Univ., Beijing (China). International Center for Quantum Materials. School of Physics
Tsinghua Univ., Beijing (China). State Key Lab. of Low-Dimensional Quantum Physics. Dept. of Physics
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source
SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., CA (United States). Stanford Inst. for Materials and Energy Sciences
SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Synchrotron Radiation Lightsource
Tsinghua Univ., Beijing (China). State Key Lab. of Low-Dimensional Quantum Physics. Dept. of Physics; Collaborative Innovation Center of Quantum Matter, Beijing (China)
SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., CA (United States). Stanford Inst. for Materials and Energy Sciences. Dept. of Physics and Applied Physics. Geballe Lab. for Advanced Materials

A single monolayer of iron selenide grown on strontium titanate shows an impressive enhancement of superconductivity compared with the bulk, as well as a novel Fermi surface topology 2-5, extreme two-dimensionality, and the possibility of phonon-enhanced electron pairing. For films thicker than one unit cell, however, the electronic structure is markedly different, with a drastically suppressed superconductivity and strong nematicity appearing 1,5. The physics driving this extraordinary dichotomy of superconducting behaviour is far from clear. Here, we use low-temperature scanning tunnelling microscopy to study multilayers of iron selenide grown by molecular beam epitaxy, and find a stripe-type charge ordering instability that develops beneath the nematic state. The charge ordering is visible and pinned in the vicinity of impurities. And as it emerges in the strong limit of nematicity, it suggests that a magnetic fluctuation with a rather small wavevector may be competing with the ordinary collinear antiferromagnetic ordering in multilayer films. The existence of stripes in iron-based superconductors, which resemble the stripe order in cuprates, not only suggests that electronic anisotropy and correlation are playing an important role, but also provides a platform for probing the complex interactions between nematicity, charge ordering, magnetism and superconductivity in high-temperature superconductors.

View Accepted Manuscript (DOE)

Cite

Export

Save

Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States); Tsinghua Univ., Beijing (China)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF); Ministry of Science and Technology of China

Grant/Contract Number:: AC02-76SF00515; AC02-05CH11231; 11674191; 2016YFA0301002

OSTI ID:: 1425888

Alternate ID(s):: OSTI ID: 1437971

Journal Information:: Nature Physics, Vol. 13, Issue 10; ISSN 1745-2473

Publisher:: Nature Publishing Group (NPG)Copyright Statement

Country of Publication:: United States

Language:: English

Citation Metrics:

Cited by: 26 works

Citation information provided by
Web of Science

References (33)

Symmetry-breaking orbital anisotropy observed for detwinned Ba(Fe1-xCox)2As2 above the spin density wave transition Yi, M.; Lu, D.; Chu, J. -H. Proceedings of the National Academy of Sciences, Vol. 108, Issue 17 https://doi.org/10.1073/pnas.1015572108	journal	April 2011
Itinerancy-Enhanced Quantum Fluctuation of Magnetic Moments in Iron-Based Superconductors Tam, Yu-Ting; Yao, Dao-Xin; Ku, Wei Physical Review Letters, Vol. 115, Issue 11 https://doi.org/10.1103/PhysRevLett.115.117001	journal	September 2015
Field-induced superconducting phase of FeSe in the BCS-BEC cross-over Kasahara, Shigeru; Watashige, Tatsuya; Hanaguri, Tetsuo Proceedings of the National Academy of Sciences, Vol. 111, Issue 46 https://doi.org/10.1073/pnas.1413477111	journal	November 2014
Interface-induced superconductivity and strain-dependent spin density waves in FeSe/SrTiO3 thin films Tan, Shiyong; Zhang, Yan; Xia, Miao Nature Materials, Vol. 12, Issue 7 https://doi.org/10.1038/nmat3654	journal	May 2013
Superconductivity in the PbO-type structure -FeSe Hsu, F. -C.; Luo, J. -Y.; Yeh, K. -W. Proceedings of the National Academy of Sciences, Vol. 105, Issue 38 https://doi.org/10.1073/pnas.0807325105	journal	September 2008
Spin waves and magnetic exchange interactions in CaFe2As2 Zhao, Jun; Adroja, D. T.; Yao, Dao-Xin Nature Physics, Vol. 5, Issue 8 https://doi.org/10.1038/nphys1336	journal	July 2009
Ferro-Orbital Order and Strong Magnetic Anisotropy in the Parent Compounds of Iron-Pnictide Superconductors Lee, Chi-Cheng; Yin, Wei-Guo; Ku, Wei Physical Review Letters, Vol. 103, Issue 26 https://doi.org/10.1103/PhysRevLett.103.267001	journal	December 2009
Direct observation of spin–orbit coupling in iron-based superconductors Borisenko, S. V.; Evtushinsky, D. V.; Liu, Z. -H. Nature Physics, Vol. 12, Issue 4 https://doi.org/10.1038/nphys3594	journal	December 2015
Dumbbell Defects in FeSe Films: A Scanning Tunneling Microscopy and First-Principles Investigation Huang, Dennis; Webb, Tatiana A.; Song, Can-Li Nano Letters, Vol. 16, Issue 7 https://doi.org/10.1021/acs.nanolett.6b01163	journal	June 2016
Interface-Induced High-Temperature Superconductivity in Single Unit-Cell FeSe Films on SrTiO ₃ Wang, Qing-Yan; Li, Zhi; Zhang, Wen-Hao Chinese Physics Letters, Vol. 29, Issue 3 https://doi.org/10.1088/0256-307X/29/3/037402	journal	March 2012
Electronic liquid-crystal phases of a doped Mott insulator Kivelson, S. A.; Fradkin, E.; Emery, V. J. Nature, Vol. 393, Issue 6685 https://doi.org/10.1038/31177	journal	June 1998
Suppression of Superconductivity by Twin Boundaries in FeSe Song, Can-Li; Wang, Yi-Lin; Jiang, Ye-Ping Physical Review Letters, Vol. 109, Issue 13 https://doi.org/10.1103/PhysRevLett.109.137004	journal	September 2012
Phase diagram and electronic indication of high-temperature superconductivity at 65 K in single-layer FeSe films He, Shaolong; He, Junfeng; Zhang, Wenhao Nature Materials, Vol. 12, Issue 7 https://doi.org/10.1038/nmat3648	journal	May 2013
Uniaxial-strain mechanical detwinning of ${CaFe}_{2} {As}_{2}$ and ${BaFe}_{2} {As}_{2}$ crystals: Optical and transport study Tanatar, M. A.; Blomberg, E. C.; Kreyssig, A. Physical Review B, Vol. 81, Issue 18 https://doi.org/10.1103/PhysRevB.81.184508	journal	May 2010
Electronic origin of high-temperature superconductivity in single-layer FeSe superconductor Liu, Defa; Zhang, Wenhao; Mou, Daixiang Nature Communications, Vol. 3, Issue 1 https://doi.org/10.1038/ncomms1946	journal	January 2012
Interfacial mode coupling as the origin of the enhancement of Tc in FeSe films on SrTiO3 Lee, J. J.; Schmitt, F. T.; Moore, R. G. Nature, Vol. 515, Issue 7526 https://doi.org/10.1038/nature13894	journal	November 2014
Electronic nematicity above the structural and superconducting transition in BaFe2(As1−xP x )2 Kasahara, S.; Shi, H. J.; Hashimoto, K. Nature, Vol. 486, Issue 7403 https://doi.org/10.1038/nature11178	journal	June 2012
Impurity-induced electronic nematic state and $C_{2}$ -symmetric nanostructures in iron pnictide superconductors Inoue, Yoshio; Yamakawa, Youichi; Kontani, Hiroshi Physical Review B, Vol. 85, Issue 22 https://doi.org/10.1103/PhysRevB.85.224506	journal	June 2012
In-Plane Resistivity Anisotropy in an Underdoped Iron Arsenide Superconductor Chu, J. -H.; Analytis, J. G.; De Greve, K. Science, Vol. 329, Issue 5993 https://doi.org/10.1126/science.1190482	journal	August 2010
Evidence for unidirectional nematic bond ordering in FeSe Watson, M. D.; Kim, T. K.; Rhodes, L. C. Physical Review B, Vol. 94, Issue 20 https://doi.org/10.1103/PhysRevB.94.201107	journal	November 2016
Dome-shaped magnetic order competing with high-temperature superconductivity at high pressures in FeSe Sun, J. P.; Matsuura, K.; Ye, G. Z. Nature Communications, Vol. 7, Issue 1 https://doi.org/10.1038/ncomms12146	journal	July 2016
Coexistence of superconductivity and magnetism in FeSe $_{1 - x}$ under pressure Bendele, M.; Ichsanow, A.; Pashkevich, Yu. Physical Review B, Vol. 85, Issue 6 https://doi.org/10.1103/PhysRevB.85.064517	journal	February 2012
Visualization of electron nematicity and unidirectional antiferroic fluctuations at high temperatures in NaFeAs Rosenthal, E. P.; Andrade, E. F.; Arguello, C. J. Nature Physics, Vol. 10, Issue 3 https://doi.org/10.1038/nphys2870	journal	February 2014
Strong cooperative coupling of pressure-induced magnetic order and nematicity in FeSe Kothapalli, K.; Böhmer, A. E.; Jayasekara, W. T. Nature Communications, Vol. 7, Issue 1 https://doi.org/10.1038/ncomms12728	journal	September 2016
Nematic Electronic Structure in the “Parent” State of the Iron-Based Superconductor Ca(Fe _1– _x Co _x ) ₂ As ₂ Chuang, T. -M.; Allan, M. P.; Lee, Jinho Science, Vol. 327, Issue 5962 https://doi.org/10.1126/science.1181083	journal	January 2010
Spin Waves and Magnetic Exchange Interactions in CaFe2As2 Zhao, Jun; Adroja, D. T.; Yao, Dao-Xin arXiv https://doi.org/10.48550/arxiv.0903.2686	text	January 2009
Interface induced high temperature superconductivity in single unit-cell FeSe films on SrTiO3 Wang, Qing-Yan; Li, Zhi; Zhang, Wen-Hao arXiv https://doi.org/10.48550/arxiv.1201.5694	text	January 2012
Electronic Origin of High Temperature Superconductivity in Single-Layer FeSe Superconductor Liu, Defa; Zhang, Wenhao; Mou, Daixiang arXiv https://doi.org/10.48550/arxiv.1202.5849	text	January 2012
Visualization of Electron Nematicity and Unidirectional Antiferroic Fluctuations at High Temperatures in NaFeAs Rosenthal, E. P.; Andrade, E. F.; Arguello, C. J. arXiv https://doi.org/10.48550/arxiv.1307.3526	text	January 2013
Interfacial mode coupling as the origin of the enhancement of Tc in FeSe films on SrTiO3 Lee, J. J.; Schmitt, F. T.; Moore, R. G. arXiv https://doi.org/10.48550/arxiv.1312.2633	text	January 2013
Reconstruction of Band Structure Induced by Electronic Nematicity in an FeSe Superconductor Nakayama, K.; Miyata, Y.; Phan, G. N. arXiv https://doi.org/10.48550/arxiv.1404.0857	text	January 2014
Direct observation of spin-orbit coupling in iron-based superconductors Borisenko, Sergey; Evtushinsky, Danil; Morozov, Igor arXiv https://doi.org/10.48550/arxiv.1409.8669	text	January 2014
Field-induced superconducting phase of FeSe in the BCS-BEC cross-over Kasahara, S.; Watashige, T.; Hanaguri, T. arXiv https://doi.org/10.48550/arxiv.1411.1232	text	January 2014

Cited By (12)

Discovery of a strain-stabilised smectic electronic order in LiFeAs Yim, Chi Ming; Trainer, Christopher; Aluru, Ramakrishna Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-04909-y	journal	July 2018
Nematicity, magnetism and superconductivity in FeSe Böhmer, Anna E.; Kreisel, Andreas Journal of Physics: Condensed Matter, Vol. 30, Issue 2 https://doi.org/10.1088/1361-648x/aa9caa	journal	December 2017
Superconducting selenides intercalated with organic molecules: synthesis, crystal structure, electric and magnetic properties, superconducting properties, and phase separation in iron based-chalcogenides and hybrid organic-inorganic superconductors Krzton-Maziopa, Anna; Pesko, Edyta; Puzniak, Roman Journal of Physics: Condensed Matter, Vol. 30, Issue 24 https://doi.org/10.1088/1361-648x/aabeb5	journal	May 2018
Charge ordering in high-temperature superconductors visualized by scanning tunneling microscopy Wang, Xintong; Yuan, Yonghao; Xue, Qi-Kun Journal of Physics: Condensed Matter, Vol. 32, Issue 1 https://doi.org/10.1088/1361-648x/ab41c5	journal	October 2019
Spectroscopic evidence of nematic fluctuations in LiFeAs Sun, Zhixiang; Nag, Pranab Kumar; Sykora, Steffen Physical Review B, Vol. 100, Issue 2 https://doi.org/10.1103/physrevb.100.024506	journal	July 2019
Study of intrinsic defect states of FeSe with scanning tunneling microscopy Bu, Kunliang; Wang, Bo; Zhang, Wenhao Physical Review B, Vol. 100, Issue 15 https://doi.org/10.1103/physrevb.100.155127	journal	October 2019
Theoretical study of impurity-induced magnetism in FeSe Martiny, Johannes H. J.; Kreisel, Andreas; Andersen, Brian M. Physical Review B, Vol. 99, Issue 1 https://doi.org/10.1103/physrevb.99.014509	journal	January 2019
Antiferromagnetic Order in Epitaxial FeSe Films on ${SrTiO}_{3}$ Zhou, Y.; Miao, L.; Wang, P. Physical Review Letters, Vol. 120, Issue 9 https://doi.org/10.1103/physrevlett.120.097001	journal	February 2018
Orbital Origin of Extremely Anisotropic Superconducting Gap in Nematic Phase of FeSe Superconductor Liu, Defa; Li, Cong; Huang, Jianwei Physical Review X, Vol. 8, Issue 3 https://doi.org/10.1103/physrevx.8.031033	journal	August 2018
Charge Density Wave and Spin Density Wave in Two-Orbital Model for Iron-Based Superconductors Pradhan, B. SPIN, Vol. 08, Issue 02 https://doi.org/10.1142/s2010324718500078	journal	June 2018
Theoretical study of impurity-induced magnetism in FeSe Martiny, Johannes H. J.; Kreisel, Andreas; Andersen, Brian M. arXiv https://doi.org/10.48550/arxiv.1811.01788	text	January 2018
Discovery of a strain-stabilised smectic electronic order in LiFeAs Yim, Chi Ming; Trainer, Christopher; Aluru, Ramakrishna arXiv https://doi.org/10.48550/arxiv.1802.05019	text	January 2018

Similar Records

Strong interplay between stripe spin fluctuations, nematicity and superconductivity in FeSe

Journal Article · Mon Dec 07 00:00:00 EST 2015 · Nature Materials · OSTI ID:1425888

Wang, Qisi; Shen, Yao; Pan, Bingying; +14 more

Nematicity in stripe ordered cuprates probed via resonant x-ray scattering

Journal Article · Fri Feb 05 00:00:00 EST 2016 · Science · OSTI ID:1425888

Achkar, A. J.; Zwiebler, M.; McMahon, Christopher; +11 more

Distinctive orbital anisotropy observed in the nematic state of a FeSe thin film

Journal Article · Mon Sep 26 00:00:00 EDT 2016 · Physical Review B · OSTI ID:1425888

Zhang, Y.; Yi, M.; Liu, Z. -K.; +11 more

Related Subjects

36 MATERIALS SCIENCE
superconducting properties and materials
surfaces
interfaces and thin films

Title: Stripes developed at the strong limit of nematicity in FeSe film

Citation Formats

References (33)

Cited By (12)

Similar Records

Related Subjects