MoS2-on-MXene Heterostructures as Highly Reversible Anode Materials for Lithium-Ion Batteries

Chen, Chi; Xie, Xiuqiang; Anasori, Babak; Sarycheva, Asya; Makaryan, Taron; Zhao, Mengqiang; Urbankowski, Patrick; Miao, Ling; Jiang, Jianjun; Gogotsi, Yury

doi:10.1002/anie.201710616

Title: MoS₂-on-MXene Heterostructures as Highly Reversible Anode Materials for Lithium-Ion Batteries

Journal Article · Tue Jan 02 00:00:00 EST 2018 · Angewandte Chemie (International Edition)

DOI:https://doi.org/10.1002/anie.201710616· OSTI ID:1435245

Chen, Chi ^[1]; Xie, Xiuqiang ^[2];

^[2]; Sarycheva, Asya ^[2];

^[2]; Zhao, Mengqiang ^[2]; Urbankowski, Patrick ^[2]; Miao, Ling ^[3]; Jiang, Jianjun ^[3];

^[2]

Drexel Univ., Philadelphia, PA (United States). A. J. Drexel Nanomaterials Inst., Materials Science and Engineering Dept.; Huazhong Univ. of Science and Technology, Wuhan (China). School of Optical and Electronic Information
Drexel Univ., Philadelphia, PA (United States). A. J. Drexel Nanomaterials Inst., Materials Science and Engineering Dept.
Huazhong Univ. of Science and Technology, Wuhan (China). School of Optical and Electronic Information

Two-dimensional (2D) heterostructured materials, combining the collective advantages of individual building blocks and synergistic properties, have spurred great interest as a new paradigm in materials science. The family of 2D transition-metal carbides and nitrides, MXenes, has emerged as an attractive platform to construct functional materials with enhanced performance for diverse applications. Here, we synthesized 2D MoS₂-on-MXene heterostructures through in situ sulfidation of Mo₂TiC₂Tx MXene. The computational results show that MoS₂-on-MXene heterostructures have metallic properties. Moreover, the presence of MXene leads to enhanced Li and Li2S adsorption during the intercalation and conversion reactions. These characteristics render the as-prepared MoS₂-on-MXene heterostructures stable Li-ion storage performance. In conclusion, this work paves the way to use MXene to construct 2D heterostructures for energy storage applications.

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Research Organization:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Energy Frontier Research Centers (EFRC) (United States). Fluid Interface Reactions, Structures and Transport Center (FIRST)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1435245

Journal Information:: Angewandte Chemie (International Edition), Vol. 57, Issue 7; ISSN 1433-7851

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 414 works

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2D Stacks of MXene Ti ₃ C ₂ and 1T‐Phase WS ₂ with Enhanced Capacitive Behavior Vyskočil, Jan; Mayorga‐Martinez, Carmen C.; Szőkölová, Kateřina ChemElectroChem, Vol. 6, Issue 15 https://doi.org/10.1002/celc.201900643	journal	May 2019
Surface Modified MXene‐Based Nanocomposites for Electrochemical Energy Conversion and Storage Yu, Hong; Wang, Yonghui; Jing, Yao Small, Vol. 15, Issue 25 https://doi.org/10.1002/smll.201901503	journal	May 2019
A synergetic stabilization and strengthening strategy for two-dimensional ordered hybrid transition metal carbides Fu, Zhongheng; Zhang, Shihao; Legut, Dominik Physical Chemistry Chemical Physics, Vol. 20, Issue 47 https://doi.org/10.1039/c8cp06458j	journal	January 2018
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A general way to fabricate transition metal dichalcogenide/oxide-sandwiched MXene nanosheets as flexible film anodes for high-performance lithium storage Wang, Chuang; Zhu, Xiao-Dong; Wang, Ke-Xin Sustainable Energy & Fuels, Vol. 3, Issue 10 https://doi.org/10.1039/c9se00635d	journal	January 2019
The dual-function sacrificing template directed formation of MoS ₂ /C hybrid nanotubes enabling highly stable and ultrafast sodium storage Gao, Jingyu; Li, Yapeng; Liu, Yi Journal of Materials Chemistry A, Vol. 7, Issue 32 https://doi.org/10.1039/c9ta05666a	journal	January 2019
Multiple roles of a heterointerface in two-dimensional van der Waals heterostructures: insights into energy-related applications Zhu, Yuanzhi; Peng, Wenchao; Li, Yang Journal of Materials Chemistry A, Vol. 7, Issue 41 https://doi.org/10.1039/c9ta06395a	journal	January 2019
H‐/dT‐MoS ₂ ‐on‐MXene Heterostructures as Promising 2D Anode Materials for Lithium‐Ion Batteries: Insights from First Principles Shao, Yangfan; Gong, Penglai; Pan, Hui Advanced Theory and Simulations, Vol. 2, Issue 8 https://doi.org/10.1002/adts.201900045	journal	May 2019
V ₄ C ₃ T _x MXene: A promising active substrate for reactive surface modification and the enhanced electrocatalytic oxygen evolution activity Du, Cheng‐Feng; Sun, Xiaoli; Yu, Hong InfoMat, Vol. 2, Issue 5 https://doi.org/10.1002/inf2.12078	journal	January 2020

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