skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Multi-pass cell-assisted photoacoustic/photothermal spectroscopy of gases using quantum cascade laser excitation and heterodyne interferometric signal detection

Journal Article · · Applied Physics. B, Lasers and Optics

A heterodyne interferometer-based signal retrieval in photoacoustic/photothermal gas spectrometer using mid-infrared quantum cascade laser excitation is demonstrated. This new method for all-optical photoacoustic/photothermal signal detection allows for sensitivity enhancement using standard multi-pass cells, commonly used in absorption-based spectrometers. Two types of multi-pass cell are examined: a Herriott type with up to 33 passes and a White type with up to 46 passes. Good agreement between experimental results and numerical analysis is obtained.

Research Organization:
Princeton Univ., NJ (United States)
Sponsoring Organization:
USDOE
Grant/Contract Number:
FE0029059
OSTI ID:
1432130
Alternate ID(s):
OSTI ID: 1545788
Journal Information:
Applied Physics. B, Lasers and Optics, Journal Name: Applied Physics. B, Lasers and Optics Vol. 124 Journal Issue: 5; ISSN 0946-2171
Publisher:
SpringerCopyright Statement
Country of Publication:
Germany
Language:
English
Citation Metrics:
Cited by: 26 works
Citation information provided by
Web of Science

References (15)

Cavity-enhanced optical feedback-assisted photo-acoustic spectroscopy with a 10.4 μm external cavity quantum cascade laser journal November 2012
Ultralow Gas Concentration Infrared Absorption Spectroscopy journal June 1971
Quantum cascade laser-based analyzer for hydrogen sulfide detection at sub-parts-per-million levels journal October 2017
A photocoustic spectroscopy system for gas detection based on the multi-pass cell conference November 2016
A Photothermal Interferometer for Gas-Phase Ammonia Detection journal April 1999
Trace detection in gases using phase fluctuation optical heterodyne spectroscopy journal April 1980
High finesse optical cavity coupled with a quartz-enhanced photoacoustic spectroscopic sensor journal January 2015
Pulsed photothermal interferometry for spectroscopic gas detection with hollow-core optical fibre journal December 2016
A quantum cascade laser-based water vapor isotope analyzer for environmental monitoring journal September 2014
2f-wavelength modulation Fabry-Perot photothermal interferometry journal January 2016
Quartz-enhanced photoacoustic spectroscopy journal January 2002
Multipass acoustically open photoacoustic detector for trace gas measurements journal January 2006
Ultra-sensitive all-fibre photothermal spectroscopy with large dynamic range journal April 2015
Heterodyne interferometric signal retrieval in photoacoustic spectroscopy journal January 2018
Mid-infrared fiber-optic photothermal interferometry journal January 2017

Cited By (3)

Photothermal spectroscopy of CO 2 in an intracavity mode-locked fiber laser configuration journal January 2018
Quartz-tuning-fork enhanced photothermal spectroscopy for ultra-high sensitive trace gas detection journal January 2018
Integration of T-type half-open photoacoustic cell and fiber-optic acoustic sensor for trace gas detection journal January 2019