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Title: Entropic Origin of Pseudogap Physics and a Mott-Slater Transition in Cuprates

Abstract

Here, we propose a new approach to understand the origin of the pseudogap in the cuprates, in terms of bosonic entropy. The near-simultaneous softening of a large number of different q-bosons yields an extended range of short-range order, wherein the growth of magnetic correlations with decreasing temperature T is anomalously slow. These entropic effects cause the spectral weight associated with the Van Hove singularity (VHS) to shift rapidly and nearly linearly toward half filling at higher T, consistent with a picture of the VHS driving the pseudogap transition at a temperature ~T*. As a byproduct, we develop an order-parameter classification scheme that predicts supertransitions between families of order parameters. As one example, we find that by tuning the hopping parameters, it is possible to drive the cuprates across a transition between Mott and Slater physics, where a spin-frustrated state emerges at the crossover.

Authors:
 [1];  [1];  [1];  [1];  [1]
  1. Northeastern Univ., Boston, MA (United States). Dept. of Physics
Publication Date:
Research Org.:
Northeastern Univ., Boston, MA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). National Energy Research Scientific Computing Center (NERSC) and Advanced Light Source (ALS); Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
OSTI Identifier:
1423568
Grant/Contract Number:  
FG02-07ER46352; AC02-05CH11231
Resource Type:
Journal Article: Accepted Manuscript
Journal Name:
Scientific Reports
Additional Journal Information:
Journal Volume: 7; Journal ID: ISSN 2045-2322
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; Electronic properties and materials; Phase transitions and critical phenomena

Citation Formats

Markiewicz, R. S., Buda, I. G., Mistark, P., Lane, C., and Bansil, A. Entropic Origin of Pseudogap Physics and a Mott-Slater Transition in Cuprates. United States: N. p., 2017. Web. doi:10.1038/srep44008.
Markiewicz, R. S., Buda, I. G., Mistark, P., Lane, C., & Bansil, A. Entropic Origin of Pseudogap Physics and a Mott-Slater Transition in Cuprates. United States. doi:10.1038/srep44008.
Markiewicz, R. S., Buda, I. G., Mistark, P., Lane, C., and Bansil, A. Wed . "Entropic Origin of Pseudogap Physics and a Mott-Slater Transition in Cuprates". United States. doi:10.1038/srep44008. https://www.osti.gov/servlets/purl/1423568.
@article{osti_1423568,
title = {Entropic Origin of Pseudogap Physics and a Mott-Slater Transition in Cuprates},
author = {Markiewicz, R. S. and Buda, I. G. and Mistark, P. and Lane, C. and Bansil, A.},
abstractNote = {Here, we propose a new approach to understand the origin of the pseudogap in the cuprates, in terms of bosonic entropy. The near-simultaneous softening of a large number of different q-bosons yields an extended range of short-range order, wherein the growth of magnetic correlations with decreasing temperature T is anomalously slow. These entropic effects cause the spectral weight associated with the Van Hove singularity (VHS) to shift rapidly and nearly linearly toward half filling at higher T, consistent with a picture of the VHS driving the pseudogap transition at a temperature ~T*. As a byproduct, we develop an order-parameter classification scheme that predicts supertransitions between families of order parameters. As one example, we find that by tuning the hopping parameters, it is possible to drive the cuprates across a transition between Mott and Slater physics, where a spin-frustrated state emerges at the crossover.},
doi = {10.1038/srep44008},
journal = {Scientific Reports},
number = ,
volume = 7,
place = {United States},
year = {Wed Mar 22 00:00:00 EDT 2017},
month = {Wed Mar 22 00:00:00 EDT 2017}
}

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