Band Dependent Interlayer f -Electron Hybridization in CeRhIn5

Chen, Q. Y.; Xu, D. F.; Niu, X. H.; Peng, R.; Xu, H. C.; Wen, C. H.  P.; Liu, X.; Shu, L.; Tan, S. Y.; Lai, X. C.; Zhang, Y. J.; Lee, H.; Strocov, V. N.; Bisti, F.; Dudin, P.; Zhu, Jianxin; Yuan, H. Q.; Kirchner, Stefan; Feng, D. L.

doi:10.1103/PhysRevLett.120.066403

Title: Band Dependent Interlayer $f$ -Electron Hybridization in ${CeRhIn}_{5}$

Journal Article · Fri Feb 09 00:00:00 EST 2018 · Physical Review Letters

DOI:https://doi.org/10.1103/PhysRevLett.120.066403· OSTI ID:1525818

Chen, Q. Y. ^[1]; Xu, D. F. ^[2]; Niu, X. H. ^[2]; Peng, R. ^[2]; Xu, H. C. ^[2]; Wen, C. H. P. ^[2]; Liu, X. ^[2]; Shu, L. ^[2]; Tan, S. Y. ^[3]; Lai, X. C. ^[3]; Zhang, Y. J. ^[4]; Lee, H. ^[4]; Strocov, V. N. ^[5]; Bisti, F. ^[5]; Dudin, P. ^[6];

^[7]; Yuan, H. Q. ^[8]; Kirchner, Stefan ^[4]; Feng, D. L. ^[9]

Fudan Univ., Shanghai (China); China Academy of Engineering Physics, Mianyang (China)
Fudan Univ., Shanghai (China)
China Academy of Engineering Physics, Mianyang (China)
Zhejiang Univ., Hangzhou (China)
Paul Scherrer Inst. (PSI), Villigen (Switzerland)
Harwell Science and Innovation Campus, Didcot (United Kingdom)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Zhejiang Univ., Hangzhou (China); Collaborative Innovation Center of Advanced Microstructures, Nanjing (China)
Fudan Univ., Shanghai (China); Collaborative Innovation Center of Advanced Microstructures, Nanjing (China)

A key issue in heavy fermion research is how subtle changes in the hybridization between the 4 $f$ (5 $f$ ) and conduction electrons can result in fundamentally different ground states. ${CeRhIn}_{5}$ stands out as a particularly notable example: when replacing Rh with either Co or Ir, antiferromagnetism gives way to superconductivity. In this photoemission study of ${CeRhIn}_{5}$ , we demonstrate that the use of resonant angle-resolved photoemission spectroscopy with polarized light allows us to extract detailed information on the 4 $f$ crystal field states and details on the 4 $f$ and conduction electron hybridization, which together determine the ground state. We directly observe weakly dispersive Kondo resonances of $f$ electrons and identify two of the three Ce4 $f$ $$^{1}_{5/2}$$ crystal-electric-field levels and band-dependent hybridization, which signals that the hybridization occurs primarily between the Ce 4 $f$ states in the CeIn₃ layer and two more three-dimensional bands composed of the Rh 4 $d$ and In 5 $p$ orbitals in the RhIn₂ layer. Our conclusions allow us to connect the properties observed at elevated temperatures with the unusual low-temperature properties of this enigmatic heavy fermion compound.

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Research Organization:: Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE Office of Science (SC). Basic Energy Sciences (BES) (SC-22); National Natural Science Foundation of China (NSFC); USDOE

Grant/Contract Number:: 89233218CNA000001

OSTI ID:: 1525818

Alternate ID(s):: OSTI ID: 1422863

Report Number(s):: LA-UR-18-21614; PRLTAO

Journal Information:: Physical Review Letters, Vol. 120, Issue 6; ISSN 0031-9007

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 37 works

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