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Title: Four-Wave-Mixing Approach to In Situ Detection of Nanoparticles

Journal Article · · Physical Review Applied
 [1];  [2];  [2];  [1];  [1];  [1]
  1. Princeton Plasma Physics Lab. (PPPL), Princeton, NJ (United States)
  2. Princeton Univ., Princeton, NJ (United States)

Here, we report on the development and experimental validation of a laser-based technique which uses coherent Rayleigh-Brillouin scattering (CRBS) to detect nanoparticles with characteristic sizes ranging from the atomic scale to tens of nanometers. This technique is aimed (nonexclusively) at the detection of nanoparticles produced by volumetric nanoparticle synthesis methods. Using CRBS, carbon nanoparticles of dimensions less than 10 nm and concentrations of 1010 cm–3 are detected in situ in a carbon arc discharge with graphite electrodes. This four-wave-mixing approach should enable advances in the understanding of nanoparticle growth that could potentially lead to improved modeling of the growth mechanisms, and thus to improve synthesis selectivity of nanoparticles and yield.

Research Organization:
Princeton Plasma Physics Laboratory (PPPL), Princeton, NJ (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC02-09CH11466
OSTI ID:
1420375
Alternate ID(s):
OSTI ID: 1418392
Journal Information:
Physical Review Applied, Vol. 9, Issue 1; ISSN 2331-7019
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 12 works
Citation information provided by
Web of Science

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Cited By (5)

Nanofabrication by thermal plasma jets: From nanoparticles to low-dimensional nanomaterials journal February 2019
Multiparametric diagnostic in the synthesis of carbon nanostructures via submerged arc discharge: Stability, nucleation and yield journal November 2019
In situ diagnostics for nanomaterial synthesis in carbon arc plasma journal August 2018
High-Gain and Narrow-Bandwidth Optical Amplifier via Optomechanical Four-Wave Mixing journal June 2019
Synthesis of nanoparticles in carbon arc: measurements and modeling journal May 2018

Figures / Tables (5)


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