NMR Study of the New Magnetic Superconductor CaK(Fe0:951Ni0:049)4As4: Microscopic Coexistence of Hedgehog Spin-vortex Crystal and Superconductivity

Ding, Q. P.; Meier, W. R.; Bohmer, A. E.; Bud'ko, S. L.; Canfield, Paul C.; Furukawa, Yuji

doi:10.1103/PhysRevB.96.220510

Title: NMR Study of the New Magnetic Superconductor CaK(Fe_0:951Ni0:049)₄As₄: Microscopic Coexistence of Hedgehog Spin-vortex Crystal and Superconductivity

Journal Article · Fri Dec 29 00:00:00 EST 2017 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.96.220510· OSTI ID:1415856

Ding, Q. P. ^[1]; Meier, W. R. ^[1]; Bohmer, A. E. ^[1]; Bud'ko, S. L. ^[1]; Canfield, Paul C. ^[1]; Furukawa, Yuji ^[1]

Ames Lab. and Iowa State Univ., Ames, IA (United States)

Coexistence of a new-type antiferromagnetic (AFM) state, the so-called hedgehog spin-vortex crystal (SVC), and superconductivity (SC) is evidenced by ⁷⁵As nuclear magnetic resonance study on single-crystalline CaK(Fe_0:951Ni0:049)₄As₄. The hedgehog SVC order is clearly demonstrated by the direct observation of the internal magnetic induction along the c axis at the As1 site (close to K) and a zero net internal magnetic induction at the As2 site (close to Ca) below an AFM ordering temperature T_N ~ 52 K. The nuclear spin-lattice relaxation rate 1/T₁ shows a distinct decrease below T_c ~ 10 K, providing also unambiguous evidence for the microscopic coexistence. Furthermore, based on the analysis of the 1/T₁ data, the hedgehog SVC-type spin correlations are found to be enhanced below T ~ 150 K in the paramagnetic state. Furthermore, these results indicate the hedgehog SVC-type spin correlations play an important role for the appearance of SC in the new magnetic superconductor.

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Research Organization:: Ames Lab., Ames, IA (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC02-07CH11358

OSTI ID:: 1415856

Alternate ID(s):: OSTI ID: 1416432

Report Number(s):: IS-J-9543

Journal Information:: Physical Review B, Vol. 96, Issue 22; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 14 works

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Odd and Even Modes of Neutron Spin Resonance in the Bilayer Iron-Based Superconductor ${CaKFe}_{4} {As}_{4}$ Xie, Tao; Wei, Yuan; Gong, Dongliang Physical Review Letters, Vol. 120, Issue 26 https://doi.org/10.1103/physrevlett.120.267003	journal	June 2018
Preferred Magnetic Excitations in the Iron-Based ${Sr}_{1 - x} {Na}_{x} {Fe}_{2} {As}_{2}$ Superconductor Guo, Jianqing; Yue, Li; Iida, Kazuki Physical Review Letters, Vol. 122, Issue 1 https://doi.org/10.1103/physrevlett.122.017001	journal	January 2019

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Title: NMR Study of the New Magnetic Superconductor CaK(Fe0:951Ni0:049)4As4: Microscopic Coexistence of Hedgehog Spin-vortex Crystal and Superconductivity

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