Field-induced antiferroelectric to ferroelectric transitions in (Pb1–xLax)(Zr0.90Ti0.10)1–x/4O3 investigated by in situ X-ray diffraction

Ciuchi, Ioana V.; Chung, Ching -Chang; Fancher, Christopher M.; Guerrier, Jonathon; Forrester, Jennifer S.; Jones, Jacob L.; Mitoseriu, L.; Galassi, C.

doi:10.1016/j.jeurceramsoc.2017.06.018

Title: Field-induced antiferroelectric to ferroelectric transitions in (Pb_1–xLa_x)(Zr_0.90Ti_0.10)_1–x/₄O₃ investigated by in situ X-ray diffraction

Journal Article · Sat Jun 17 00:00:00 EDT 2017 · Journal of the European Ceramic Society

DOI:https://doi.org/10.1016/j.jeurceramsoc.2017.06.018· OSTI ID:1414716

Ciuchi, Ioana V. ^[1]; Chung, Ching -Chang ^[2];

^[3]; Guerrier, Jonathon ^[2]; Forrester, Jennifer S. ^[4]; Jones, Jacob L. ^[2]; Mitoseriu, L. ^[5]; Galassi, C. ^[6]

Istituto di Scienza e Tecnologia dei Materiali Ceramici, Faenza (Italy); "A. I. Cuza" Univ., Iasi (Romania)
North Carolina State Univ., Raleigh, NC (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Univ. of Leeds, Leeds (United Kingdom)
"A. I. Cuza" Univ., Iasi (Romania)
Istituto di Scienza e Tecnologia dei Materiali Ceramici, Faenza (Italy)

Phase transitions and field-induced preferred orientation in (Pb_1-xLa_x)(Zr_0.90Ti_0.10)_1–x/₄O₃ (PLZT x/90/10) ceramics upon electric field cycling using in situ X-ray diffraction were studied. The evolution of the {200}_pc and {111}_pc diffraction line profiles indicate that PLZT 4/90/10 and PLZT 3/90/10 compositions undergo an antiferroelectric (AFE)–ferroelectric (FE) phase switching. Both PLZT 4/90/10 and PLZT 3/90/10 exhibit irreversible preferred orientation after experiencing the field-induced AFE-to-FE phase switching. An electric field-induced structure develops in both compositions which has a reversible character during the field decreasing in PLZT 4/90/10 and an irreversible character in PLZT 3/90/10. In addition, structural analysis of pre-poled PLZT 3/90/10 ceramics show that it is possible to induce consecutive FE-to-AFE and AFE-to-FE transitions when fields of reversed polarity are applied in sequence. The field range required to induce the AFE phase is broad, and the phase transition is kinetically slow. In conclusion, this kind of transition has rarely been reported before.

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Research Organization:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1414716

Journal Information:: Journal of the European Ceramic Society, Vol. 37, Issue 15; ISSN 0955-2219

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 17 works

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Crystal Phase Distribution and Ferroelectricity in Ultrathin HfO ₂ –ZrO ₂ Bilayers McBriarty, Martin E.; Narasimhan, Vijay K.; Weeks, Stephen L. physica status solidi (b), Vol. 257, Issue 1 https://doi.org/10.1002/pssb.201900285	journal	September 2019

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Title: Field-induced antiferroelectric to ferroelectric transitions in (Pb1–xLax)(Zr0.90Ti0.10)1–x/4O3 investigated by in situ X-ray diffraction

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Title: Field-induced antiferroelectric to ferroelectric transitions in (Pb_1–xLa_x)(Zr_0.90Ti_0.10)_1–x/₄O₃ investigated by in situ X-ray diffraction