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Title: Tc removal from the waste treatment and immobilization plant low-activity waste vitrification off-gas recycle

Abstract

Vitrification of Low Activity Waste in the Hanford Waste Treatment and Immobilization Plant generates a condensate stream from the off-gas processes. Components in this stream are partially volatile and accumulate to high concentrations through recycling, which impacts the waste glass loading and facility throughput. The primary radionuclide that vaporizes and accumulates in the stream is 99Tc. This program is investigating Tc removal via reductive precipitation with stannous chloride to examine the potential for diverting this stream to an alternate disposition path. As a result, research has shown stannous chloride to be effective, and this paper describes results of recent experiments performed to further mature the technology.

Authors:
 [1];  [1];  [1]
  1. Savannah River National Lab., Aiken, SC (United States)
Publication Date:
Research Org.:
Savannah River Site (SRS), Aiken, SC (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1406492
Report Number(s):
SRNL-STI-2016-00389
Journal ID: ISSN 0149-6395
Grant/Contract Number:  
AC09-08SR22470
Resource Type:
Journal Article: Accepted Manuscript
Journal Name:
Separation Science and Technology
Additional Journal Information:
Journal Volume: 53; Journal Issue: 12; Journal ID: ISSN 0149-6395
Publisher:
Taylor & Francis
Country of Publication:
United States
Language:
English
Subject:
12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE WASTES FROM NUCLEAR FACILITIES; decontamination; stannous chloride; technetium; WTP

Citation Formats

Taylor-Pashow, Kathryn M. L., McCabe, Daniel J., and Nash, Charles A. Tc removal from the waste treatment and immobilization plant low-activity waste vitrification off-gas recycle. United States: N. p., 2017. Web. doi:10.1080/01496395.2017.1302952.
Taylor-Pashow, Kathryn M. L., McCabe, Daniel J., & Nash, Charles A. Tc removal from the waste treatment and immobilization plant low-activity waste vitrification off-gas recycle. United States. doi:10.1080/01496395.2017.1302952.
Taylor-Pashow, Kathryn M. L., McCabe, Daniel J., and Nash, Charles A. Thu . "Tc removal from the waste treatment and immobilization plant low-activity waste vitrification off-gas recycle". United States. doi:10.1080/01496395.2017.1302952. https://www.osti.gov/servlets/purl/1406492.
@article{osti_1406492,
title = {Tc removal from the waste treatment and immobilization plant low-activity waste vitrification off-gas recycle},
author = {Taylor-Pashow, Kathryn M. L. and McCabe, Daniel J. and Nash, Charles A.},
abstractNote = {Vitrification of Low Activity Waste in the Hanford Waste Treatment and Immobilization Plant generates a condensate stream from the off-gas processes. Components in this stream are partially volatile and accumulate to high concentrations through recycling, which impacts the waste glass loading and facility throughput. The primary radionuclide that vaporizes and accumulates in the stream is 99Tc. This program is investigating Tc removal via reductive precipitation with stannous chloride to examine the potential for diverting this stream to an alternate disposition path. As a result, research has shown stannous chloride to be effective, and this paper describes results of recent experiments performed to further mature the technology.},
doi = {10.1080/01496395.2017.1302952},
journal = {Separation Science and Technology},
number = 12,
volume = 53,
place = {United States},
year = {Thu Mar 16 00:00:00 EDT 2017},
month = {Thu Mar 16 00:00:00 EDT 2017}
}

Journal Article:
Free Publicly Available Full Text
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