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Title: Nonequilibrium Synthesis of Highly Porous Single-Crystalline Oxide Nanostructures

Journal Article · · Advanced Materials Interfaces
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  1. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
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A novel synthesis route to the formation of vertically aligned single–crystalline oxide nanostructures is found by precisely controlling the nonequilibrium pulsed laser deposition process. Here, the columnar nanostructures with deep crevices offering a large surface area are generated owing to the diffusion limited geometric shadowing effect.

Research Organization:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC05-00OR22725
OSTI ID:
1436958
Alternate ID(s):
OSTI ID: 1401742
Journal Information:
Advanced Materials Interfaces, Vol. 4, Issue 3; ISSN 2196-7350
Publisher:
Wiley-VCHCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 11 works
Citation information provided by
Web of Science

References (47)

Pulsed laser deposition of tungsten and tungsten oxide thin films with tailored structure at the nano- and mesoscale journal July 2007
One-Dimensional Nanostructures: Synthesis, Characterization, and Applications journal June 2003
Atomic and electronic structure of unreduced and reduced CeO2 surfaces: A first-principles study journal April 2004
Mantid—Data analysis and visualization package for neutron scattering and μ SR experiments
  • Arnold, O.; Bilheux, J. C.; Borreguero, J. M.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 764 https://doi.org/10.1016/j.nima.2014.07.029
journal November 2014
Thin-Film Transistor Fabricated in Single-Crystalline Transparent Oxide Semiconductor journal May 2003
On diffusion limited deposition journal January 2016
Thin-film solid oxide fuel cell with high performance at low-temperature journal June 1997
Columnar growth and kinetic roughening in electrochemical deposition journal June 1992
Reversible redox reactions in an epitaxially stabilized SrCoOx oxygen sponge journal August 2013
Growth and characterization of non-c-oriented epitaxial ferroelectric SrBi2Ta2O9 films on buffered Si(100) journal November 2000
Diffusion-Limited Aggregation, a Kinetic Critical Phenomenon journal November 1981
Nucleation and growth of thin films journal April 1984
Angular laser cleaning for effective removal of particles. from a solid surface journal December 2000
One-Dimensional Nanostructures: Synthesis, Characterization, and Applications journal March 2003
Growth of aligned ZnO nanorod arrays by catalyst-free pulsed laser deposition methods journal September 2004
Diffusion-limited aggregation: A kinetic critical phenomenon? journal July 2000
Multiparticle biased diffusion-limited aggregation with surface diffusion: A comprehensive model of electrodeposition journal July 2000
Hierarchical TiO 2 Photoanode for Dye-Sensitized Solar Cells journal July 2010
Repeated temperature modulation epitaxy for p-type doping and light-emitting diode based on ZnO journal December 2004
Imposed layer-by-layer growth by pulsed laser interval deposition journal June 1999
High electrochemical activity of the oxide phase in model ceria–Pt and ceria–Ni composite anodes journal December 2011
Growth control of oxygen stoichiometry in homoepitaxial SrTiO3 films by pulsed laser epitaxy in high vacuum journal January 2016
Epitaxial yttria‐stabilized zirconia on hydrogen‐terminated Si by pulsed laser deposition journal September 1990
Characterization of Thin-Film Rechargeable Lithium Batteries with Lithium Cobalt Oxide Cathodes journal January 1996
Microstructures of CGO and YSZ Thin Films by Pulsed Laser Deposition journal December 2007
Microscopic view of epitaxial metal growth: nucleation and aggregation journal January 1998
Resonant tunnelling in a quantum oxide superlattice journal June 2015
Plasma plume characteristics and properties of pulsed laser deposited diamond-like carbon films journal March 2003
High power density thin film SOFCs with YSZ/GDC bilayer electrolyte journal June 2011
Nucleation And Growth Of Thin Films journal June 1984
Electrical conductivity of thin film ceria grown by pulsed laser deposition journal January 2007
Thin-Film Growth and the Shadow Instability journal February 1989
Instabilities in crystal growth by atomic or molecular beams journal February 2000
Structure, stability and work functions of the low index surfaces of pure indium oxide and Sn-doped indium oxide (ITO) from density functional theory journal January 2010
Columnar growth in oblique incidence ballistic deposition: Faceting, noise reduction, and mean-field theory journal January 1991
Thin-Film Growth and the Shadow Instability journal June 1989
High proton conduction in grain-boundary-free yttrium-doped barium zirconate films grown by pulsed laser deposition journal September 2010
Atomic Layer Engineering of Perovskite Oxides for Chemically Sharp Heterointerfaces journal October 2012
Thousandfold Change in Resistivity in Magnetoresistive La-Ca-Mn-O Films journal April 1994
Oxygen Reduction Kinetics Enhancement on a Heterostructured Oxide Surface for Solid Oxide Fuel Cells journal October 2010
Morphological instability of a terrace edge during step-flow growth journal March 1990
Chemistry and Physics in One Dimension: Synthesis and Properties of Nanowires and Nanotubes journal February 1999
High electrode activity of nanostructured, columnar ceria films for solid oxide fuel cells journal January 2012
Microscopic view of epitaxial metal growth: Nucleation and aggregation journal May 1998
Atomic layer engineering of perovskite oxides for chemically sharp heterointerfaces text January 2012
Growth control of oxygen stoichiometry in homoepitaxial SrTiO3 films by pulsed laser epitaxy in high vacuum text January 2016
Instabilities in crystal growth by atomic or molecular beams text January 1999

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36 MATERIALS SCIENCE
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
vertical oxide nanostructures
pulsed laser deposition
diffusion limited aggregation
binary oxides
porous nanostructures