Narrowing the Gap between Theoretical and Practical Capacities in Li-Ion Layered Oxide Cathode Materials

Radin, Maxwell D.; Hy, Sunny; Sina, Mahsa; Fang, Chengcheng; Liu, Haodong; Vinckeviciute, Julija; Zhang, Minghao; Whittingham, M. Stanley; Meng, Y. Shirley; Van der Ven, Anton

doi:10.1002/aenm.201602888

Title: Narrowing the Gap between Theoretical and Practical Capacities in Li-Ion Layered Oxide Cathode Materials

Journal Article · Tue Jul 04 00:00:00 EDT 2017 · Advanced Energy Materials

DOI:https://doi.org/10.1002/aenm.201602888· OSTI ID:1388252

^[1]; Hy, Sunny ^[2]; Sina, Mahsa ^[2]; Fang, Chengcheng ^[2]; Liu, Haodong ^[2];

^[1]; Zhang, Minghao ^[2]; Whittingham, M. Stanley ^[3]; Meng, Y. Shirley ^[2]; Van der Ven, Anton ^[1]

Univ. of California Santa Barbara, Santa Barbara, CA (United States)
Univ. of California San Diego, La Jolla, CA (United States)
State Univ. of New York, Binghamton, NY (United States)

Abstract Although layered lithium oxides have become the cathode of choice for state‐of‐the‐art Li‐ion batteries, substantial gaps remain between the practical and theoretical energy densities. With the aim of supporting efforts to close this gap, this work reviews the fundamental operating mechanisms and challenges of Li intercalation in layered oxides, contrasts how these challenges play out differently for different materials (with emphasis on Ni–Co–Al (NCA) and Ni–Mn–Co (NMC) alloys), and summarizes the extensive corpus of modifications and extensions to the layered lithium oxides. Particular emphasis is given to the fundamental mechanisms behind the operation and degradation of layered intercalation electrode materials as well as novel modifications and extensions, including Na‐ion and cation‐disordered materials.

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Research Organization:: Energy Frontier Research Centers (EFRC) (United States). Northeastern Center for Chemical Energy Storage (NECCES)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0001294; DE‐SC0012583

OSTI ID:: 1388252

Alternate ID(s):: OSTI ID: 1400638

Journal Information:: Advanced Energy Materials, Vol. 7, Issue 20; Related Information: NECCES partners with Stony Brook University (lead); Argonne National Laboratory; Binghamton University; Brookhaven National University; University of California, San Diego; University of Cambridge, UK; Lawrence Berkeley National Laboratory; Massachusetts Institute of Technology; University of Michigan; Rutgers University; ISSN 1614-6832

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 404 works

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Kinetic Stability of Bulk LiNiO ₂ and Surface Degradation by Oxygen Evolution in LiNiO ₂ -Based Cathode Materials Kong, Fantai; Liang, Chaoping; Wang, Luhua Advanced Energy Materials, Vol. 9, Issue 2 https://doi.org/10.1002/aenm.201802586	journal	November 2018
Investigating the Effects of Magnesium Doping in Various Ni-Rich Positive Electrode Materials for Lithium Ion Batteries Liu, Aaron; Zhang, Ning; Li, Hongyang Journal of The Electrochemical Society, Vol. 166, Issue 16 https://doi.org/10.1149/2.1101915jes	journal	January 2019
Aqueous Li-ion battery enabled by halogen conversion–intercalation chemistry in graphite Yang, Chongyin; Chen, Ji; Ji, Xiao Nature, Vol. 569, Issue 7755 https://doi.org/10.1038/s41586-019-1175-6	journal	May 2019
Li ₃ BN ₂ as a Transition Metal Free, High Capacity Cathode for Li-ion Batteries Emani, Satyanarayana; Liu, Caihong; Ashuri, Maziar ChemElectroChem, Vol. 6, Issue 2 https://doi.org/10.1002/celc.201801415	journal	November 2018
Impact of Dopants (Al, Mg, Mn, Co) on the Reactivity of Li _x NiO ₂ with the Electrolyte of Li-Ion Batteries Cormier, Marc M. E.; Zhang, Ning; Liu, Aaron Journal of The Electrochemical Society, Vol. 166, Issue 13 https://doi.org/10.1149/2.0491913jes	journal	January 2019
Structural water and disordered structure promote aqueous sodium-ion energy storage in sodium-birnessite Shan, Xiaoqiang; Guo, Fenghua; Charles, Daniel S. Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-12939-3	journal	October 2019
Ti‐Gradient Doping to Stabilize Layered Surface Structure for High Performance High‐Ni Oxide Cathode of Li‐Ion Battery Kong, Defei; Hu, Jiangtao; Chen, Zhefeng Advanced Energy Materials, Vol. 9, Issue 41 https://doi.org/10.1002/aenm.201901756	journal	September 2019
Structural Insight into Layer Gliding and Lattice Distortion in Layered Manganese Oxide Electrodes for Potassium‐Ion Batteries Zhang, Qing; Didier, Christophe; Pang, Wei Kong Advanced Energy Materials, Vol. 9, Issue 30 https://doi.org/10.1002/aenm.201900568	journal	June 2019
Manganese oxidation as the origin of the anomalous capacity of Mn-containing Li-excess cathode materials Radin, Maxwell D.; Vinckeviciute, Julija; Seshadri, Ram Nature Energy, Vol. 4, Issue 8 https://doi.org/10.1038/s41560-019-0439-6	journal	July 2019
Increase and discretization of the energy barrier for individual LiNi _x Co _y Mn _y O ₂ ( x + 2 y =1) particles with the growth of a Li ₂ CO ₃ surface film Qian, Kun; Huang, Binhua; Liu, Yuxiu Journal of Materials Chemistry A, Vol. 7, Issue 20 https://doi.org/10.1039/c9ta01443h	journal	January 2019
Impact of the Synthesis Conditions on the Performance of LiNi _x Co _y Al _z O ₂ with High Ni and Low Co Content Li, Jing; Zhang, Ning; Li, Hongyang Journal of The Electrochemical Society, Vol. 165, Issue 14 https://doi.org/10.1149/2.0931814jes	journal	January 2018
The Formation of Layered Double Hydroxide Phases in the Coprecipitation Syntheses of [Ni0.80Co0.15](1−x)/0.95Alx(OH)2(anionn−)x/n (x = 0–0.2, n = 1, 2) Liu, Aaron; Dahn, J. ChemEngineering, Vol. 3, Issue 2 https://doi.org/10.3390/chemengineering3020038	journal	April 2019
Electrochemical surface passivation of LiCoO2 particles at ultrahigh voltage and its applications in lithium-based batteries Qian, Jiawei; Liu, Lei; Yang, Jixiang Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-07296-6	journal	November 2018
A versatile single molecular precursor for the synthesis of layered oxide cathode materials for Li-ion batteries Li, Maofan; Liu, Jiajie; Liu, Tongchao Chemical Communications, Vol. 54, Issue 11 https://doi.org/10.1039/c7cc08505b	journal	January 2018
Understanding ageing in Li-ion batteries: a chemical issue Palacín, M. Rosa Chemical Society Reviews, Vol. 47, Issue 13 https://doi.org/10.1039/c7cs00889a	journal	January 2018
A routine for the determination of the microstructure of stacking-faulted nickel cobalt aluminium hydroxide precursors for lithium nickel cobalt aluminium oxide battery materials Bette, Sebastian; Hinrichsen, Bernd; Pfister, Daniela Journal of Applied Crystallography, Vol. 53, Issue 1 https://doi.org/10.1107/s1600576719016212	journal	February 2020
Li-Rich Layered/Spinel Cathode Composite 3/4[Li ₂ MnO ₃ ·LiCxO ₂ ]·1/4[LiCxMnO ₄ ] (Cx = Cr _1-y Co _y ) for Li-Ion Batteries Ma, Zhijie; Li, Dan; Han, Yan Journal of The Electrochemical Society, Vol. 166, Issue 3 https://doi.org/10.1149/2.0111903jes	journal	November 2018
Effect of Low-Temperature Al2O3 ALD Coating on Ni-Rich Layered Oxide Composite Cathode on the Long-Term Cycling Performance of Lithium-Ion Batteries Neudeck, Sven; Mazilkin, Andrey; Reitz, Christian Scientific Reports, Vol. 9, Issue 1 https://doi.org/10.1038/s41598-019-41767-0	journal	March 2019
Investigating the Removal of Layered Double Hydroxides in [Ni _0.80 Co _0.15 ] _0.95-x Al _0.05+x (OH) ₂ (x = 0, 0.05) Prepared by Coprecipitation Liu, Aaron; Zhang, Ning; Li, Jing Journal of The Electrochemical Society, Vol. 165, Issue 11 https://doi.org/10.1149/2.0731811jes	journal	January 2018
Degradation and Aging Routes of Ni-Rich Cathode Based Li-Ion Batteries Teichert, Philipp; Eshetu, Gebrekidan Gebresilassie; Jahnke, Hannes RWTH Aachen University https://doi.org/10.18154/rwth-2020-04543	text	January 2020
Cooling Induced Surface Reconstruction during Synthesis of High‐Ni Layered Oxides Zhang, Ming‐Jian; Hu, Xiaobing; Li, Maofan Advanced Energy Materials, Vol. 9, Issue 43 https://doi.org/10.1002/aenm.201901915	journal	October 2019
X‐ray Nano‐computed Tomography of Electrochemical Conversion in Lithium‐ion Battery Di Lecce, Daniele; Levchenko, Stanislav; Iacoviello, Francesco ChemSusChem, Vol. 12, Issue 15 https://doi.org/10.1002/cssc.201901123	journal	July 2019
Understanding intercalation compounds for sodium-ion batteries and beyond Kaufman, Jonas L.; Vinckevičiūtė, Julija; Krishna Kolli, Sanjeev Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 377, Issue 2152 https://doi.org/10.1098/rsta.2019.0020	journal	July 2019
Effect of Choices of Positive Electrode Material, Electrolyte, Upper Cut-Off Voltage and Testing Temperature on the Life Time of Lithium-Ion Cells Li, Jing; Glazier, Stephen L.; Nelson, Kathlyne Journal of The Electrochemical Society, Vol. 165, Issue 13 https://doi.org/10.1149/2.0931813jes	journal	January 2018
Structural evolution at the oxidative and reductive limits in the first electrochemical cycle of Li1.2Ni0.13Mn0.54Co0.13O2 Yin, Wei; Grimaud, Alexis; Rousse, Gwenaelle Nature Communications, Vol. 11, Issue 1 https://doi.org/10.1038/s41467-020-14927-4	journal	March 2020

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