skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Interlayer bond polarizability model for stacking-dependent low-frequency Raman scattering in layered materials

Journal Article · · Nanoscale
DOI:https://doi.org/10.1039/c7nr05839j· OSTI ID:1399929

A simple model is developed to reveal the stacking dependence of Raman intensities of interlayer vibrations in 2D materials.

Research Organization:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
USDOE Office of Science (SC)
Grant/Contract Number:
AC05-00OR22725
OSTI ID:
1399929
Journal Information:
Nanoscale, Vol. 9; ISSN 2040-3364
Publisher:
Royal Society of ChemistryCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 31 works
Citation information provided by
Web of Science

References (74)

Raman characterization of AB- and ABC-stacked few-layer graphene by interlayer shear modes journal April 2016
Mapping of Low-Frequency Raman Modes in CVD-Grown Transition Metal Dichalcogenides: Layer Number, Stacking Orientation and Resonant Effects journal January 2016
Coupled Spin and Valley Physics in Monolayers of MoS 2 and Other Group-VI Dichalcogenides journal May 2012
Relation between Photoelasticity, Electrostriction, and First-Order Raman Effect in Crystals of the Diamond Structure journal December 1967
Interface Coupling in Twisted Multilayer Graphene by Resonant Raman Spectroscopy of Layer Breathing Modes journal June 2015
Progress, Challenges, and Opportunities in Two-Dimensional Materials Beyond Graphene journal March 2013
Phonon and Raman scattering of two-dimensional transition metal dichalcogenides from monolayer, multilayer to bulk material journal January 2015
Spin and pseudospins in layered transition metal dichalcogenides journal April 2014
Strongly enhanced charge-density-wave order in monolayer NbSe2 journal July 2015
Stacking-Dependent Interlayer Coupling in Trilayer MoS 2 with Broken Inversion Symmetry journal November 2015
Stacking-dependent band gap and quantum transport in trilayer graphene journal September 2011
Low-Frequency Interlayer Raman Modes to Probe Interface of Twisted Bilayer MoS 2 journal January 2016
Raman Signature of Graphene Superlattices journal November 2011
Observation of an electrically tunable band gap in trilayer graphene journal September 2011
Ultralow-frequency Raman system down to 10 cm −1 with longpass edge filters and its application to the interface coupling in t(2+2)LGs journal May 2016
Interlayer Electronic Coupling in Arbitrarily Stacked MoS 2 Bilayers Controlled by Interlayer S–S Interaction journal December 2014
The experimental observation of quantum Hall effect of l=3 chiral quasiparticles in trilayer graphene journal September 2011
The ABC of 2D materials journal July 2015
Raman spectroscopy of shear and layer breathing modes in multilayer MoS 2 journal March 2013
Lattice vibrations and Raman scattering in two-dimensional layered materials beyond graphene journal September 2016
Coupling and Stacking Order of ReS 2 Atomic Layers Revealed by Ultralow-Frequency Raman Spectroscopy journal January 2016
Interlayer interactions in anisotropic atomically thin rhenium diselenide journal October 2015
Valley-dependent spin polarization in bulk MoS2 with broken inversion symmetry journal July 2014
Low frequency Raman spectroscopy of few-atomic-layer thick hBN crystals journal June 2017
The shear mode of multilayer graphene journal February 2012
Observation of piezoelectricity in free-standing monolayer MoS2 journal December 2014
Raman Spectroscopy Study of Rotated Double-Layer Graphene: Misorientation-Angle Dependence of Electronic Structure journal June 2012
Raman spectroscopy as a versatile tool for studying the properties of graphene journal April 2013
Evolution of interlayer coupling in twisted molybdenum disulfide bilayers journal September 2014
First-principles Raman spectra of MoS2, WS2 and their heterostructures journal January 2014
Filter-based ultralow-frequency Raman measurement down to 2 cm −1 for fast Brillouin spectroscopy measurement journal May 2017
Stacking-dependent shear modes in trilayer graphene journal January 2015
Large Frequency Change with Thickness in Interlayer Breathing Mode—Significant Interlayer Interactions in Few Layer Black Phosphorus journal May 2015
Low-Frequency Raman Fingerprints of Two-Dimensional Metal Dichalcogenide Layer Stacking Configurations journal May 2015
Interlayer breathing and shear modes in NbSe 2 atomic layers journal August 2016
Identifying different stacking sequences in few-layer CVD-grown Mo S 2 by low-energy atomic-resolution scanning transmission electron microscopy journal January 2016
Tailoring the Electronic Structure in Bilayer Molybdenum Disulfide via Interlayer Twist journal June 2014
Review on the Raman spectroscopy of different types of layered materials journal January 2016
Stacking sequence determines Raman intensities of observed interlayer shear modes in 2D layered materials – A general bond polarizability model journal October 2015
Revealing the Preferred Interlayer Orientations and Stackings of Two-Dimensional Bilayer Gallium Selenide Crystals journal January 2015
Anomalous Lattice Vibrations of Single- and Few-Layer MoS 2 journal March 2010
Measurement of layer breathing mode vibrations in few-layer graphene journal March 2013
Interlayer Breathing and Shear Modes in Few-Trilayer MoS 2 and WSe 2 journal February 2013
Probing the Interlayer Coupling of Twisted Bilayer MoS 2 Using Photoluminescence Spectroscopy journal September 2014
Plasma-assisted fabrication of monolayer phosphorene and its Raman characterization journal May 2014
Hofstadter’s butterfly and the fractal quantum Hall effect in moiré superlattices journal May 2013
Piezoelectricity of single-atomic-layer MoS2 for energy conversion and piezotronics journal October 2014
Van der Waals heterostructures journal July 2013
Electric Field Effect in Atomically Thin Carbon Films journal October 2004
Spectroscopic Signatures of AA′ and AB Stacking of Chemical Vapor Deposited Bilayer MoS 2 journal October 2015
Anisotropic Electron-Photon and Electron-Phonon Interactions in Black Phosphorus journal March 2016
Recent Advances in Two-Dimensional Materials beyond Graphene journal October 2015
Raman Signatures of Polytypism in Molybdenum Disulfide journal January 2016
Low-frequency interlayer vibration modes in two-dimensional layered materials journal June 2016
Low-Frequency Interlayer Breathing Modes in Few-Layer Black Phosphorus journal May 2015
Crystal structure and interatomic distances in GaSe journal October 1975
Volume Bragg gratings as ultra-narrow and multiband optical filters conference June 2012
Unusual Angular Dependence of the Raman Response in Black Phosphorus journal February 2015
Twisted MoSe 2 Bilayers with Variable Local Stacking and Interlayer Coupling Revealed by Low-Frequency Raman Spectroscopy journal January 2016
Multiwall Nanotubes, Multilayers, and Hybrid Nanostructures: New Frontiers for Technology and Raman Spectroscopy journal March 2013
Observation of interlayer phonon modes in van der Waals heterostructures journal April 2015
The chemistry of two-dimensional layered transition metal dichalcogenide nanosheets journal April 2013
Trilayer graphene is a semimetal with a gate-tunable band overlap journal April 2009
Stacking effects on the electronic and optical properties of bilayer transition metal dichalcogenides MoS 2 , MoSe 2 , WS 2 , and WSe 2 journal February 2014
Stacking in Bulk and Bilayer Hexagonal Boron Nitride journal July 2013
Raman scattering intensities in α-quartz: A first-principles investigation journal February 2001
Single-layer MoS2 transistors journal January 2011
Observation of Van Hove singularities in twisted graphene layers journal November 2009
Control of valley polarization in monolayer MoS2 by optical helicity journal June 2012
Monolayer behaviour in bulk ReS2 due to electronic and vibrational decoupling journal February 2014
Valley and band structure engineering of folded MoS2 bilayers journal August 2014
Low-frequency Raman modes and electronic excitations in atomically thin MoS 2 films journal December 2012
Rapid and Nondestructive Identification of Polytypism and Stacking Sequences in Few-Layer Molybdenum Diselenide by Raman Spectroscopy journal July 2015
Polytypism and unexpected strong interlayer coupling in two-dimensional layered ReS 2 journal January 2016

Cited By (10)

Characterization of two‐dimensional materials from Raman spectral data journal October 2019
Laser Synthesis, Processing, and Spectroscopy of Atomically-Thin Two Dimensional Materials book January 2018
Cross-dimensional electron-phonon coupling in van der Waals heterostructures journal June 2019
Suppression of the shear Raman mode in defective bilayer MoS 2 journal February 2019
Band-edges and band-gap in few-layered transition metal dichalcogenides journal May 2018
Anomalous interlayer vibrations in strongly coupled layered PdSe 2 journal May 2018
Davydov splitting and polytypism in few-layer MoS 2 journal October 2018
Stacking-dependent interlayer phonons in 3R and 2H MoS 2 journal February 2019
Suppression of the Shear Raman Mode in Defective Bilayer MoS2 text January 2018
A Universal Length-Dependent Vibrational Mode in Graphene Nanoribbons text January 2019