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Title: Seasonal Variations in Mercury Deposition over the Yellow Sea, July 2007 through April 2008

Abstract

Spatial and temporal variations of mercury, including dry and wet deposition fluxes, were assessed over Northeast Asia, targeting the Yellow Sea, using meteorology and chemistry models. Four modeling periods, each representative of one of the four seasons, were selected. Modeling results captured general patterns and behaviors, and fell within similar ranges with respect to observations. However, temporal variations of mercury were not closely matched, possibly owing to the effects of localized emissions. Modeling results indicated that dry deposition is correlated with wind speed, while wet deposition is correlated with precipitation amount. Overall, the wet deposition flux of 66 ng/m2-day was about twice as large as the dry deposition flux of 32 ng/m2-day, when averaged over the four modeling periods. Dry deposition occurred predominantly in the form of reactive gaseous mercury (RGM). In contrast, RGM accounted for only about two-thirds of wet deposition, while particulate mercury accounted for the remainder.

Authors:
; ; ; ;
Publication Date:
Research Org.:
Argonne National Lab. (ANL), Argonne, IL (United States)
Sponsoring Org.:
Hankuk University of Foreign Studies, Korea
OSTI Identifier:
1395960
DOE Contract Number:  
AC02-06CH11357
Resource Type:
Journal Article
Resource Relation:
Journal Name: Asian Journal of Atmospheric Environment; Journal Volume: 10; Journal Issue: 3
Country of Publication:
United States
Language:
English
Subject:
58 GEOSCIENCES; 54 ENVIRONMENTAL SCIENCES; CMAQ-Hg/WRF; Dry deposition; Precipitation amount; Wet deposition; Wind speed

Citation Formats

Ghim, Young Sung, Oh, Hyun Sun, Kim, Jin Young, Woo, Jung-Hun, and Chang, Young-Soo. Seasonal Variations in Mercury Deposition over the Yellow Sea, July 2007 through April 2008. United States: N. p., 2016. Web. doi:10.5572/ajae.2016.10.3.146.
Ghim, Young Sung, Oh, Hyun Sun, Kim, Jin Young, Woo, Jung-Hun, & Chang, Young-Soo. Seasonal Variations in Mercury Deposition over the Yellow Sea, July 2007 through April 2008. United States. doi:10.5572/ajae.2016.10.3.146.
Ghim, Young Sung, Oh, Hyun Sun, Kim, Jin Young, Woo, Jung-Hun, and Chang, Young-Soo. Fri . "Seasonal Variations in Mercury Deposition over the Yellow Sea, July 2007 through April 2008". United States. doi:10.5572/ajae.2016.10.3.146.
@article{osti_1395960,
title = {Seasonal Variations in Mercury Deposition over the Yellow Sea, July 2007 through April 2008},
author = {Ghim, Young Sung and Oh, Hyun Sun and Kim, Jin Young and Woo, Jung-Hun and Chang, Young-Soo},
abstractNote = {Spatial and temporal variations of mercury, including dry and wet deposition fluxes, were assessed over Northeast Asia, targeting the Yellow Sea, using meteorology and chemistry models. Four modeling periods, each representative of one of the four seasons, were selected. Modeling results captured general patterns and behaviors, and fell within similar ranges with respect to observations. However, temporal variations of mercury were not closely matched, possibly owing to the effects of localized emissions. Modeling results indicated that dry deposition is correlated with wind speed, while wet deposition is correlated with precipitation amount. Overall, the wet deposition flux of 66 ng/m2-day was about twice as large as the dry deposition flux of 32 ng/m2-day, when averaged over the four modeling periods. Dry deposition occurred predominantly in the form of reactive gaseous mercury (RGM). In contrast, RGM accounted for only about two-thirds of wet deposition, while particulate mercury accounted for the remainder.},
doi = {10.5572/ajae.2016.10.3.146},
journal = {Asian Journal of Atmospheric Environment},
number = 3,
volume = 10,
place = {United States},
year = {Fri Sep 30 00:00:00 EDT 2016},
month = {Fri Sep 30 00:00:00 EDT 2016}
}