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Title: Magnetoelastoelectric coupling in core-shell nanoparticles enabling directional and mode-selective magnetic control of THz beam propagation

Abstract

Magnetoelastoelectric coupling in an engineered biphasic multiferroic nanocomposite enables a novel magnetic field direction-defined propagation control of terahertz (THz) waves. These core–shell nanoparticles are comprised of a ferromagnetic cobalt ferrite core and a ferroelectric barium titanate shell. Furthermore, an assembly of these nanoparticles, when operated in external magnetic fields, exhibits a controllable amplitude modulation when the magnetic field is applied antiparallel to the THz wave propagation direction; yet the same assembly displays an additional phase modulation when the magnetic field is applied along the propagation direction. And while field-induced magnetostriction of the core leads to amplitude modulation, phase modulation is a result of stress-mediated piezoelectricity of the outer ferroelectric shell.

Authors:
 [1]; ORCiD logo [2];  [2];  [1];  [1];  [1]
  1. Univ. of Texas, San Antonio, TX (United States). Dept. of Electrical and Computer Engineering
  2. Los Alamos National Lab. (LANL), Los Alamos, NM (United States). Center for Integrated Nanotechnologies
Publication Date:
Research Org.:
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Sponsoring Org.:
USDOE Office of Science (SC). Basic Energy Sciences (BES) (SC-22); National Science Foundation (NSF); National Institutes of Health (NIH)
OSTI Identifier:
1392884
Report Number(s):
LA-UR-17-25491
Journal ID: ISSN 2040-3364 ; 2040-3372 (Electronic)
Grant/Contract Number:
AC52-06NA25396; W911NF-12-1-0082; 1002380; G12MD007591
Resource Type:
Journal Article: Accepted Manuscript
Journal Name:
Nanoscale
Additional Journal Information:
Journal Volume: 9; Journal Issue: 35; Journal ID: ISSN 2040-3364
Publisher:
Royal Society of Chemistry
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; Material Science

Citation Formats

Dutta, Moumita, Prasankumar, Rohit Prativadi, Natarajan, Kamaraju, Betal, Soutik, Bhalla, Amar S., and Guo, Ruyan. Magnetoelastoelectric coupling in core-shell nanoparticles enabling directional and mode-selective magnetic control of THz beam propagation. United States: N. p., 2017. Web. doi:10.1039/C7NR03504G.
Dutta, Moumita, Prasankumar, Rohit Prativadi, Natarajan, Kamaraju, Betal, Soutik, Bhalla, Amar S., & Guo, Ruyan. Magnetoelastoelectric coupling in core-shell nanoparticles enabling directional and mode-selective magnetic control of THz beam propagation. United States. doi:10.1039/C7NR03504G.
Dutta, Moumita, Prasankumar, Rohit Prativadi, Natarajan, Kamaraju, Betal, Soutik, Bhalla, Amar S., and Guo, Ruyan. Mon . "Magnetoelastoelectric coupling in core-shell nanoparticles enabling directional and mode-selective magnetic control of THz beam propagation". United States. doi:10.1039/C7NR03504G.
@article{osti_1392884,
title = {Magnetoelastoelectric coupling in core-shell nanoparticles enabling directional and mode-selective magnetic control of THz beam propagation},
author = {Dutta, Moumita and Prasankumar, Rohit Prativadi and Natarajan, Kamaraju and Betal, Soutik and Bhalla, Amar S. and Guo, Ruyan},
abstractNote = {Magnetoelastoelectric coupling in an engineered biphasic multiferroic nanocomposite enables a novel magnetic field direction-defined propagation control of terahertz (THz) waves. These core–shell nanoparticles are comprised of a ferromagnetic cobalt ferrite core and a ferroelectric barium titanate shell. Furthermore, an assembly of these nanoparticles, when operated in external magnetic fields, exhibits a controllable amplitude modulation when the magnetic field is applied antiparallel to the THz wave propagation direction; yet the same assembly displays an additional phase modulation when the magnetic field is applied along the propagation direction. And while field-induced magnetostriction of the core leads to amplitude modulation, phase modulation is a result of stress-mediated piezoelectricity of the outer ferroelectric shell.},
doi = {10.1039/C7NR03504G},
journal = {Nanoscale},
number = 35,
volume = 9,
place = {United States},
year = {Mon Aug 07 00:00:00 EDT 2017},
month = {Mon Aug 07 00:00:00 EDT 2017}
}

Journal Article:
Free Publicly Available Full Text
This content will become publicly available on August 7, 2018
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