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Title: Highly efficient luminescent solar concentrators based on earth-abundant indirect-bandgap silicon quantum dots

Authors:
; ; ; ; ORCiD logo; ORCiD logo; ; ORCiD logo;
Publication Date:
Research Org.:
Energy Frontier Research Centers (EFRC) (United States). Center for Advanced Solar Photophysics (CASP)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1388304
DOE Contract Number:  
AC52-06NA25396
Resource Type:
Journal Article
Journal Name:
Nature Photonics
Additional Journal Information:
Journal Volume: 11; Journal Issue: 3; Related Information: CASP partners with Los Alamos National Laboratory (lead); University of California, Irvine; University of Colorado; Colorado School of Mines; George Mason University; Los Alamos National Laboratory; University of Minnesota; National Renewable Energy Laboratory; Journal ID: ISSN 1749-4885
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
solar (photovoltaic), solar (fuels), solid state lighting, bio-inspired, electrodes - solar, defects, charge transport, materials and chemistry by design, optics, synthesis (novel materials), synthesis (scalable processing)

Citation Formats

Meinardi, Francesco, Ehrenberg, Samantha, Dhamo, Lorena, Carulli, Francesco, Mauri, Michele, Bruni, Francesco, Simonutti, Roberto, Kortshagen, Uwe, and Brovelli, Sergio. Highly efficient luminescent solar concentrators based on earth-abundant indirect-bandgap silicon quantum dots. United States: N. p., 2017. Web. doi:10.1038/nphoton.2017.5.
Meinardi, Francesco, Ehrenberg, Samantha, Dhamo, Lorena, Carulli, Francesco, Mauri, Michele, Bruni, Francesco, Simonutti, Roberto, Kortshagen, Uwe, & Brovelli, Sergio. Highly efficient luminescent solar concentrators based on earth-abundant indirect-bandgap silicon quantum dots. United States. doi:10.1038/nphoton.2017.5.
Meinardi, Francesco, Ehrenberg, Samantha, Dhamo, Lorena, Carulli, Francesco, Mauri, Michele, Bruni, Francesco, Simonutti, Roberto, Kortshagen, Uwe, and Brovelli, Sergio. Mon . "Highly efficient luminescent solar concentrators based on earth-abundant indirect-bandgap silicon quantum dots". United States. doi:10.1038/nphoton.2017.5.
@article{osti_1388304,
title = {Highly efficient luminescent solar concentrators based on earth-abundant indirect-bandgap silicon quantum dots},
author = {Meinardi, Francesco and Ehrenberg, Samantha and Dhamo, Lorena and Carulli, Francesco and Mauri, Michele and Bruni, Francesco and Simonutti, Roberto and Kortshagen, Uwe and Brovelli, Sergio},
abstractNote = {},
doi = {10.1038/nphoton.2017.5},
journal = {Nature Photonics},
issn = {1749-4885},
number = 3,
volume = 11,
place = {United States},
year = {2017},
month = {2}
}

Works referenced in this record:

Long-term optical stability of fluorescent solar concentrator plates: Long-term optical stability of fluorescent solar concentrator plates
journal, February 2014

  • Slooff, Lenneke H.; Bakker, Nicolaas J.; Sommeling, Paul M.
  • physica status solidi (a), Vol. 211, Issue 5
  • DOI: 10.1002/pssa.201330447

Near-Unity Internal Quantum Efficiency of Luminescent Silicon Nanocrystals with Ligand Passivation
journal, June 2015


Effect on the output of a luminescent solar concentrator on application of organic wavelength-selective mirrors
journal, January 2010

  • Debije, Michael G.; Van, My-Phung; Verbunt, Paul P. C.
  • Applied Optics, Vol. 49, Issue 4
  • DOI: 10.1364/AO.49.000745

Solar energy conversion with fluorescent collectors
journal, October 1977


An efficient room-temperature silicon-based light-emitting diode
journal, March 2001

  • Ng, Wai Lek; Lourenço, M. A.; Gwilliam, R. M.
  • Nature, Vol. 410, Issue 6825
  • DOI: 10.1038/35065571

Photostability of thermally-hydrosilylated silicon quantum dots
journal, January 2015

  • Wu, Jeslin J.; Kortshagen, Uwe R.
  • RSC Advances, Vol. 5, Issue 126
  • DOI: 10.1039/C5RA22827A

Monocrystalline silicon photovoltaic luminescent solar concentrator with 42% power conversion efficiency
journal, January 2012

  • Desmet, L.; Ras, A. J. M.; de Boer, D. K. G.
  • Optics Letters, Vol. 37, Issue 15
  • DOI: 10.1364/OL.37.003087

Tackling self-absorption in luminescent solar concentrators with type-II colloidal quantum dots
journal, April 2013

  • Krumer, Zachar; Pera, Suzanne J.; van Dijk-Moes, Relinde J. A.
  • Solar Energy Materials and Solar Cells, Vol. 111
  • DOI: 10.1016/j.solmat.2012.12.028

Highly efficient large-area colourless luminescent solar concentrators using heavy-metal-free colloidal quantum dots
journal, August 2015

  • Meinardi, Francesco; McDaniel, Hunter; Carulli, Francesco
  • Nature Nanotechnology, Vol. 10, Issue 10
  • DOI: 10.1038/nnano.2015.178

Highly Luminescent Silicon Nanocrystals with Discrete Optical Transitions
journal, April 2001

  • Holmes, Justin D.; Ziegler, Kirk J.; Doty, R. Christopher
  • Journal of the American Chemical Society, Vol. 123, Issue 16
  • DOI: 10.1021/ja002956f

Single-dot absorption spectroscopy and theory of silicon nanocrystals
journal, April 2016


A comparison of performance of flat and bent photovoltaic luminescent solar concentrators
journal, February 2015


Silicon nanoparticles: Absorption, emission, and the nature of the electronic bandgap
journal, May 2007

  • Meier, Cedrik; Gondorf, Andreas; Lüttjohann, Stephan
  • Journal of Applied Physics, Vol. 101, Issue 10
  • DOI: 10.1063/1.2720095

Electron-phonon coupling and optical transitions for indirect-gap semiconductor nanocrystals
journal, October 2001


Large-area luminescent solar concentrators based on ‘Stokes-shift-engineered’ nanocrystals in a mass-polymerized PMMA matrix
journal, April 2014

  • Meinardi, Francesco; Colombo, Annalisa; Velizhanin, Kirill A.
  • Nature Photonics, Vol. 8, Issue 5, p. 392-399
  • DOI: 10.1038/nphoton.2014.54

Bright CuInS 2 /CdS nanocrystal phosphors for high-gain full-spectrum luminescent solar concentrators
journal, January 2015

  • Knowles, Kathryn E.; Kilburn, Troy B.; Alzate, Dane G.
  • Chemical Communications, Vol. 51, Issue 44
  • DOI: 10.1039/C5CC02007G

In Vivo Targeted Cancer Imaging, Sentinel Lymph Node Mapping and Multi-Channel Imaging with Biocompatible Silicon Nanocrystals
journal, December 2010

  • Erogbogbo, Folarin; Yong, Ken-Tye; Roy, Indrajit
  • ACS Nano, Vol. 5, Issue 1
  • DOI: 10.1021/nn1018945

Silicon nanocrystals with ensemble quantum yields exceeding 60%
journal, June 2006

  • Jurbergs, David; Rogojina, Elena; Mangolini, Lorenzo
  • Applied Physics Letters, Vol. 88, Issue 23
  • DOI: 10.1063/1.2210788

A luminescent solar concentrator with 7.1% power conversion efficiency
journal, December 2008

  • Slooff, L. H.; Bende, E. E.; Burgers, A. R.
  • physica status solidi (RRL) - Rapid Research Letters, Vol. 2, Issue 6
  • DOI: 10.1002/pssr.200802186

Synthesis of Ligand-Stabilized Silicon Nanocrystals with Size-Dependent Photoluminescence Spanning Visible to Near-Infrared Wavelengths
journal, December 2011

  • Hessel, Colin M.; Reid, Dariya; Panthani, Matthew G.
  • Chemistry of Materials, Vol. 24, Issue 2
  • DOI: 10.1021/cm2032866

Luminescent Solar Concentration with Semiconductor Nanorods and Transfer-Printed Micro-Silicon Solar Cells
journal, December 2013

  • Bronstein, Noah D.; Li, Lanfang; Xu, Lu
  • ACS Nano, Vol. 8, Issue 1
  • DOI: 10.1021/nn404418h

Flexible and fluorophore-doped luminescent solar concentrators based on polydimethylsiloxane
journal, January 2016

  • Tummeltshammer, Clemens; Taylor, Alaric; Kenyon, Anthony J.
  • Optics Letters, Vol. 41, Issue 4
  • DOI: 10.1364/OL.41.000713

Solar Energy Collectors with Tunable Transmission
journal, April 2010


Increasing the efficiency of fluorescent concentrator systems
journal, February 2009

  • Goldschmidt, Jan Christoph; Peters, Marius; Bösch, Armin
  • Solar Energy Materials and Solar Cells, Vol. 93, Issue 2
  • DOI: 10.1016/j.solmat.2008.09.048

Spectroscopic and Device Aspects of Nanocrystal Quantum Dots
journal, September 2016


High-Efficiency Silicon Nanocrystal Light-Emitting Devices
journal, May 2011

  • Cheng, Kai-Yuan; Anthony, Rebecca; Kortshagen, Uwe R.
  • Nano Letters, Vol. 11, Issue 5
  • DOI: 10.1021/nl2001692

Ray-trace simulation of CuInS(Se)_2 quantum dot based luminescent solar concentrators
journal, January 2015

  • Hu, Xiangmin; Kang, Ruidan; Zhang, Yongyou
  • Optics Express, Vol. 23, Issue 15
  • DOI: 10.1364/OE.23.00A858

Routes to Achieving High Quantum Yield Luminescence from Gas-Phase-Produced Silicon Nanocrystals
journal, August 2011

  • Anthony, Rebecca J.; Rowe, David J.; Stein, Matthias
  • Advanced Functional Materials, Vol. 21, Issue 21
  • DOI: 10.1002/adfm.201100784

On the Origin of Photoluminescence in Silicon Nanocrystals: Pressure-Dependent Structural and Optical Studies
journal, July 2012

  • Hannah, Daniel C.; Yang, Jihua; Podsiadlo, Paul
  • Nano Letters, Vol. 12, Issue 8
  • DOI: 10.1021/nl301787g

Thirty Years of Luminescent Solar Concentrator Research: Solar Energy for the Built Environment
journal, December 2011

  • Debije, Michael G.; Verbunt, Paul P. C.
  • Advanced Energy Materials, Vol. 2, Issue 1
  • DOI: 10.1002/aenm.201100554

Luminescent greenhouse collector for solar radiation
journal, January 1976


Absorption and emission of light in nanoscale silicon structures
journal, March 1994


Quantum Confinement in Size-Selected, Surface-Oxidized Silicon Nanocrystals
journal, November 1993


Fabrication and spectroscopic studies on highly luminescent CdSe/CdS nanorod polymer composites
journal, January 2010

  • Bomm, Jana; Büchtemann, Andreas; Fiore, Angela
  • Beilstein Journal of Nanotechnology, Vol. 1
  • DOI: 10.3762/bjnano.1.11

Zero-Reabsorption Doped-Nanocrystal Luminescent Solar Concentrators
journal, March 2014

  • Erickson, Christian S.; Bradshaw, Liam R.; McDowall, Stephen
  • ACS Nano, Vol. 8, Issue 4
  • DOI: 10.1021/nn406360w

Resonance-shifting to circumvent reabsorption loss in luminescent solar concentrators
journal, September 2011

  • Giebink, Noel C.; Wiederrecht, Gary P.; Wasielewski, Michael R.
  • Nature Photonics, Vol. 5, Issue 11
  • DOI: 10.1038/nphoton.2011.236

Core/Shell Quantum Dot Based Luminescent Solar Concentrators with Reduced Reabsorption and Enhanced Efficiency
journal, June 2014

  • Coropceanu, Igor; Bawendi, Moungi G.
  • Nano Letters, Vol. 14, Issue 7
  • DOI: 10.1021/nl501627e

Quasi-Direct Optical Transitions in Silicon Nanocrystals with Intensity Exceeding the Bulk
journal, February 2016


Doctor-blade deposition of quantum dots onto standard window glass for low-loss large-area luminescent solar concentrators
journal, October 2016


High-Yield Plasma Synthesis of Luminescent Silicon Nanocrystals
journal, April 2005

  • Mangolini, L.; Thimsen, E.; Kortshagen, U.
  • Nano Letters, Vol. 5, Issue 4
  • DOI: 10.1021/nl050066y

Near Infrared, Highly Efficient Luminescent Solar Concentrators
journal, March 2016

  • Zhou, Yufeng; Benetti, Daniele; Fan, Zhiyuan
  • Advanced Energy Materials, Vol. 6, Issue 11
  • DOI: 10.1002/aenm.201501913

Luminescent solar concentrators – A low cost photovoltaics alternative
journal, January 2013


Nanocrystals for Luminescent Solar Concentrators
journal, January 2015

  • Bradshaw, Liam R.; Knowles, Kathryn E.; McDowall, Stephen
  • Nano Letters, Vol. 15, Issue 2
  • DOI: 10.1021/nl504510t

Plasma-Assisted Synthesis of Silicon Nanocrystal Inks
journal, September 2007

  • Mangolini, L.; Kortshagen, U.
  • Advanced Materials, Vol. 19, Issue 18, p. 2513-2519
  • DOI: 10.1002/adma.200700595

Photoluminescence quantum yields of amorphous and crystalline silicon nanoparticles
journal, September 2009