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Title: Thermodynamics of thorium substitution in yttrium iron garnet: comparison of experimental and theoretical results

Abstract

The thermodynamic stability of Th-doped yttrium iron garnet (Y 3Fe 5O 12, YIG) as a possible actinide-bearing material has been investigated using calorimetric measurements and first-principles electronic-structure calculations.

Authors:
 [1];  [2];  [1];  [3];  [4];  [1]
  1. Peter A. Rock Thermochemistry Laboratory and Neat ORU; University of California; Davis, USA
  2. Department of Materials Science and Engineering; North Carolina State University; Raleigh, USA
  3. Department of Earth and Environmental Sciences; University of Michigan; Ann Arbor, USA
  4. Department of Geological and Environmental Sciences; Stanford University; Stanford, USA
Publication Date:
Research Org.:
Energy Frontier Research Centers (EFRC) (United States). Materials Science of Actinides (MSA)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1386626
DOE Contract Number:  
SC0001089
Resource Type:
Journal Article
Journal Name:
Journal of Materials Chemistry. A
Additional Journal Information:
Journal Volume: 2; Journal Issue: 40; Related Information: MSA partners with University of Notre Dame (lead); University of California, Davis; Florida State University; George Washington University; University of Michigan; University of Minnesota; Oak Ridge National Laboratory; Oregon state University; Rensselaer Polytechnic Institute; Savannah River National Laboratory; Journal ID: ISSN 2050-7488
Publisher:
Royal Society of Chemistry
Country of Publication:
United States
Language:
English
Subject:
nuclear (including radiation effects), materials and chemistry by design, synthesis (novel materials), synthesis (self-assembly)

Citation Formats

Guo, X., Rak, Zs., Tavakoli, A. H., Becker, U., Ewing, R. C., and Navrotsky, A. Thermodynamics of thorium substitution in yttrium iron garnet: comparison of experimental and theoretical results. United States: N. p., 2014. Web. doi:10.1039/C4TA03683B.
Guo, X., Rak, Zs., Tavakoli, A. H., Becker, U., Ewing, R. C., & Navrotsky, A. Thermodynamics of thorium substitution in yttrium iron garnet: comparison of experimental and theoretical results. United States. doi:10.1039/C4TA03683B.
Guo, X., Rak, Zs., Tavakoli, A. H., Becker, U., Ewing, R. C., and Navrotsky, A. Wed . "Thermodynamics of thorium substitution in yttrium iron garnet: comparison of experimental and theoretical results". United States. doi:10.1039/C4TA03683B.
@article{osti_1386626,
title = {Thermodynamics of thorium substitution in yttrium iron garnet: comparison of experimental and theoretical results},
author = {Guo, X. and Rak, Zs. and Tavakoli, A. H. and Becker, U. and Ewing, R. C. and Navrotsky, A.},
abstractNote = {The thermodynamic stability of Th-doped yttrium iron garnet (Y3Fe5O12, YIG) as a possible actinide-bearing material has been investigated using calorimetric measurements and first-principles electronic-structure calculations.},
doi = {10.1039/C4TA03683B},
journal = {Journal of Materials Chemistry. A},
issn = {2050-7488},
number = 40,
volume = 2,
place = {United States},
year = {2014},
month = {1}
}

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