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Title: Simultaneous detection of electronic structure changes from two elements of a bifunctional catalyst using wavelength-dispersive X-ray emission spectroscopy and in situ electrochemistry

Abstract

A method of simultaneously probing the electronic structure of multiple metal centers using wavelength-dispersive X-ray emission spectroscopy was developed.

Authors:
 [1];  [2];  [3];  [4];  [3];  [5];  [6];  [2];  [3];  [7];  [8];  [3];  [6];  [9];  [10]
  1. Physical Biosciences Division; Lawrence Berkeley National Laboratory; Berkeley; USA; Department of Chemistry
  2. Department of Chemical Engineering; Stanford University; Stanford; USA
  3. SLAC National Accelerator Laboratory; Menlo Park; USA
  4. Physical Biosciences Division; Lawrence Berkeley National Laboratory; Berkeley; USA; SLAC National Accelerator Laboratory
  5. Joint Center for Artificial Photosynthesis; Lawrence Berkeley National Laboratory; Berkeley; USA
  6. Physical Biosciences Division; Lawrence Berkeley National Laboratory; Berkeley; USA
  7. Advanced Light Source; Lawrence Berkeley National Laboratory; Berkeley; USA
  8. Department of Chemistry; University of California at Santa Cruz; Santa Cruz; USA
  9. Department of Chemical Engineering; Stanford University; Stanford; USA; Joint Center for Artificial Photosynthesis
  10. Physical Biosciences Division; Lawrence Berkeley National Laboratory; Berkeley; USA; Joint Center for Artificial Photosynthesis
Publication Date:
Research Org.:
Energy Frontier Research Centers (EFRC) (United States). Center on Nanostructuring for Efficient Energy Conversion (CNEEC)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1386136
DOE Contract Number:
SC0001060
Resource Type:
Journal Article
Resource Relation:
Journal Name: Physical Chemistry Chemical Physics. PCCP (Print); Journal Volume: 17; Journal Issue: 14; Related Information: CNEEC partners with Stanford University (lead); Carnegie Institution at Stanford; Technical University of Denmark
Country of Publication:
United States
Language:
English
Subject:
catalysis (heterogeneous), solar (fuels), photosynthesis (natural and artificial), bio-inspired, electrodes - solar, defects, charge transport, materials and chemistry by design, synthesis (novel materials)

Citation Formats

Gul, Sheraz, Ng, Jia Wei Desmond, Alonso-Mori, Roberto, Kern, Jan, Sokaras, Dimosthenis, Anzenberg, Eitan, Lassalle-Kaiser, Benedikt, Gorlin, Yelena, Weng, Tsu-Chien, Zwart, Petrus H., Zhang, Jin Z., Bergmann, Uwe, Yachandra, Vittal K., Jaramillo, Thomas F., and Yano, Junko. Simultaneous detection of electronic structure changes from two elements of a bifunctional catalyst using wavelength-dispersive X-ray emission spectroscopy and in situ electrochemistry. United States: N. p., 2015. Web. doi:10.1039/C5CP01023C.
Gul, Sheraz, Ng, Jia Wei Desmond, Alonso-Mori, Roberto, Kern, Jan, Sokaras, Dimosthenis, Anzenberg, Eitan, Lassalle-Kaiser, Benedikt, Gorlin, Yelena, Weng, Tsu-Chien, Zwart, Petrus H., Zhang, Jin Z., Bergmann, Uwe, Yachandra, Vittal K., Jaramillo, Thomas F., & Yano, Junko. Simultaneous detection of electronic structure changes from two elements of a bifunctional catalyst using wavelength-dispersive X-ray emission spectroscopy and in situ electrochemistry. United States. doi:10.1039/C5CP01023C.
Gul, Sheraz, Ng, Jia Wei Desmond, Alonso-Mori, Roberto, Kern, Jan, Sokaras, Dimosthenis, Anzenberg, Eitan, Lassalle-Kaiser, Benedikt, Gorlin, Yelena, Weng, Tsu-Chien, Zwart, Petrus H., Zhang, Jin Z., Bergmann, Uwe, Yachandra, Vittal K., Jaramillo, Thomas F., and Yano, Junko. Thu . "Simultaneous detection of electronic structure changes from two elements of a bifunctional catalyst using wavelength-dispersive X-ray emission spectroscopy and in situ electrochemistry". United States. doi:10.1039/C5CP01023C.
@article{osti_1386136,
title = {Simultaneous detection of electronic structure changes from two elements of a bifunctional catalyst using wavelength-dispersive X-ray emission spectroscopy and in situ electrochemistry},
author = {Gul, Sheraz and Ng, Jia Wei Desmond and Alonso-Mori, Roberto and Kern, Jan and Sokaras, Dimosthenis and Anzenberg, Eitan and Lassalle-Kaiser, Benedikt and Gorlin, Yelena and Weng, Tsu-Chien and Zwart, Petrus H. and Zhang, Jin Z. and Bergmann, Uwe and Yachandra, Vittal K. and Jaramillo, Thomas F. and Yano, Junko},
abstractNote = {A method of simultaneously probing the electronic structure of multiple metal centers using wavelength-dispersive X-ray emission spectroscopy was developed.},
doi = {10.1039/C5CP01023C},
journal = {Physical Chemistry Chemical Physics. PCCP (Print)},
number = 14,
volume = 17,
place = {United States},
year = {Thu Jan 01 00:00:00 EST 2015},
month = {Thu Jan 01 00:00:00 EST 2015}
}