skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Anomalies in the Charge Yields of Fission Fragments from the U ( n , f ) 238 Reaction

Journal Article · · Physical Review Letters
 [1];  [1];  [1];  [2];  [3];  [4];  [5];  [5];  [6];  [7];  [2];  [8];  [1];  [8];  [9];  [8];  [10];  [11];  [8];  [8] more »;  [8];  [12];  [8];  [13];  [14];  [1];  [7];  [15];  [16];  [17];  [7];  [5];  [4];  [18];  [10];  [6];  [11];  [11];  [10];  [19];  [18];  [10];  [11];  [20];  [11];  [1];  [10];  [11];  [7] « less
  1. Univ. Paris-Sud, Orsay (France). Inst. de Physique Nucleaire
  2. European Commission, Karlsruhe (Germany). Joint Research Centre
  3. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
  4. Subatech/Ecole des Mines, Nantes (France)
  5. Univ. of Surrey, Guildford (United Kingdom). Dept. of Physics
  6. Katholieke Univ. Leuven, Leuven (Belgium). Inst. for Nuclear and Radiation Physics
  7. Univ. Paris-Saclay, Gif-sur-Yvette (France)
  8. Centre National de la Recherche Scientifique (CNRS), Orsay (France). Inst. National de Physique Nucleaire et de Physique des Particules (IN2P3), Centre de Sciences Nucleaires et de Sciences de la Matiere (CSNSM)
  9. National Inst. of Nuclear Physics (INFN), Legnaro (Italy). National Lab. of Legnaro (INFN-LNL)
  10. Inst. fur Kernphysik, Koln (Deutschland)
  11. Univ. of Oslo (Norway). Dept. of Physics
  12. National Physical Lab., Middlesex (United Kingdom)
  13. Ludwig Maximilian Univ., Munich (Germany)
  14. Alternative Energies and Atomic Energy Commission (CEA), Arpajon (France)
  15. Centre d'Etudes Nucleaires de Bordeaux-Gradignan, Gradignan (France)
  16. Extreme Light Infrastructure-Nuclear Physics (ELI-NP), Bucharest-Magurele (Romania)
  17. European Commission, Geel (Belgium). Joint Research Centre
  18. Univ. of Surrey, Guildford (United Kingdom). Dept. of Physics; National Physical Lab., Middlesex (United Kingdom)
  19. Alternative Energies and Atomic Energy Commission (CEA), Cadarache (France)
  20. Univ. of Manchester (United Kingdom). Dept. of Physics

Fast-neutron-induced fission of 238U at an energy just above the fission threshold is studied with a novel technique which involves the coupling of a high-efficiency γ-ray spectrometer (MINIBALL) to an inverse-kinematics neutron source (LICORNE) to extract charge yields of fission fragments via γ-γ coincidence spectroscopy. Experimental data and fission models are compared and found to be in reasonable agreement for many nuclei; however, significant discrepancies of up to 600% are observed, particularly for isotopes of Sn and Mo. This indicates that these models significantly overestimate the standard 1 fission mode and suggests that spherical shell effects in the nascent fission fragments are less important for low-energy fast-neutron-induced fission than for thermal neutron-induced fission. Finally, this has consequences for understanding and modeling the fission process, for experimental nuclear structure studies of the most neutron-rich nuclei, for future energy applications (e.g., Generation IV reactors which use fast-neutron spectra), and for the reactor antineutrino anomaly.

Research Organization:
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Sponsoring Organization:
USDOE; Research Council of Norway; Science and Technology Facilities Council (STFC), UK
Grant/Contract Number:
AC52-07NA27344; 05P15PKCIA; 222287
OSTI ID:
1378544
Report Number(s):
LLNL-JRNL-737167; PRLTAO; TRN: US1702815
Journal Information:
Physical Review Letters, Vol. 118, Issue 22; ISSN 0031-9007
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 24 works
Citation information provided by
Web of Science

References (25)

Nuclear-fission studies with relativistic secondary beams: Analysis of fission channels journal April 2008
Determination of antineutrino spectra from nuclear reactors journal August 2011
New insights from studies of spontaneous fission with large detector arrays journal January 1995
New excited states in Ge 82 : Possible weakening of the N = 50 closed shell journal August 2007
Development of a kinematically focused neutron source with the p(7Li,n)7Be inverse reaction
  • Lebois, M.; Wilson, J. N.; Halipré, P.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 735 https://doi.org/10.1016/j.nima.2013.07.061
journal January 2014
ENDF/B-VII.1 Nuclear Data for Science and Technology: Cross Sections, Covariances, Fission Product Yields and Decay Data journal December 2011
Prompt Emission in Fission Induced with Fast Neutrons journal January 2015
Prompt neutron multiplicity in correlation with fragments from spontaneous fission of Cf 252 journal December 2014
Identification of the γ transitions in Tc and Cs products of 252 Cf fission and possible 7 / 2 + [413] bands in 105 109 Tc isotopes journal May 1998
Fission fragment properties obtained in the γ - γ - γ coincidence method in the reaction 208Pb(18O, f ) journal October 2007
Possible origins and implications of the shoulder in reactor neutrino spectra journal August 2015
Fragment yields from the fission of 238U by fast neutrons journal November 1998
Yields of correlated fragment pairs in spontaneous fission of 252 Cf journal March 1997
Measurement of prompt X-rays in 238U(n,f) from threshold to 400 MeV: Investigation of fission charge yield evolution journal September 2013
Correlated spins of complementary fragment pairs in the spontaneous fission of 252 Cf journal November 1999
Geant4—a simulation toolkit
  • Agostinelli, S.; Allison, J.; Amako, K.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 506, Issue 3 https://doi.org/10.1016/S0168-9002(03)01368-8
journal July 2003
Isomeric gamma rays from U 235 ( n , f ) and Pu 239 ( n , f ) for times less than 1 μsec after fission journal August 1974
Spectroscopy of neutron rich nuclei using cold neutron induced fission of actinide targets at the ILL: the EXILL campaign journal January 2014
Mass distributions in monoenergetic-neutron-induced fission of U 238 journal January 1978
General Description of Fission Observables: GEF Model Code journal January 2016
Nuclear scission journal December 1990
The Miniball spectrometer journal March 2013
Near-yrast excitations in nucleus As 83 : Tracing the π g 9 / 2 orbital in the Ni 78 region journal April 2015
Spectroscopy of neutron rich nuclei using cold neutron induced fission of actinide targets at the ILL: The EXILL campaign journal January 2013
Nuclear-fission studies with relativistic secondary beams: analysis of fission channels text January 2007

Cited By (4)