Ice cloud formation potential by free tropospheric particles from long-range transport over the Northern Atlantic Ocean

China, Swarup; Alpert, Peter A.; Zhang, Bo; Schum, Simeon; Dzepina, Katja; Wright, Kendra; Owen, R. Chris; Fialho, Paulo; Mazzoleni, Lynn R.; Mazzoleni, Claudio; Knopf, Daniel A.

doi:10.1002/2016JD025817

Title: Ice cloud formation potential by free tropospheric particles from long-range transport over the Northern Atlantic Ocean

Journal Article · Mon Feb 27 00:00:00 EST 2017 · Journal of Geophysical Research: Atmospheres

DOI:https://doi.org/10.1002/2016JD025817· OSTI ID:1349629

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Michigan Technological Univ., Houghton, MI (United States); Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
Stony Brook Univ., Stony Brook, NY (United States); Paul Scherrer Inst. (PSI), Villigen (Switzerland)
Michigan Technological Univ., Houghton, MI (United States)
Michigan Technological Univ., Houghton, MI (United States); Univ. of Rijeka, Rijeka (Croatia)
Michigan Technological Univ., Houghton, MI (United States); U.S. Environmental Protection Agency, RTP, NC (United States)
Instituto de Investigacao em Vulcanologia e Avaliacao de Riscos da Univ. dos Acores, Acores (Portugal)
Stony Brook Univ., Stony Brook, NY (United States)

Abstract Long‐range transported free tropospheric particles can play a significant role on heterogeneous ice nucleation. Using optical and electron microscopy we examine the physicochemical characteristics of ice nucleating particles (INPs). Particles were collected on substrates from the free troposphere at the remote Pico Mountain Observatory in the Azores Islands, after long‐range transport and aging over the Atlantic Ocean. We investigate four specific events to study the ice formation potential by the collected particles with different ages and transport patterns. We use single‐particle analysis, as well as bulk analysis to characterize particle populations. Both analyses show substantial differences in particle composition between samples from the four events; in addition, single‐particle microscopy analysis indicates that most particles are coated by organic material. The identified INPs contained mixtures of dust, aged sea salt and soot, and organic material acquired either at the source or during transport. The temperature and relative humidity ( RH ) at which ice formed, varied only by 5% between samples, despite differences in particle composition, sources, and transport patterns. We hypothesize that this small variation in the onset RH may be due to the coating material on the particles. This study underscores and motivates the need to further investigate how long‐range transported and atmospherically aged free tropospheric particles impact ice cloud formation.

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Research Organization:: Stony Brook Univ., NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Biological and Environmental Research (BER)

Grant/Contract Number:: SC0016370; SC0008613

OSTI ID:: 1349629

Alternate ID(s):: OSTI ID: 1377929

Journal Information:: Journal of Geophysical Research: Atmospheres, Vol. 122, Issue 5; ISSN 2169-897X

Publisher:: American Geophysical UnionCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 28 works

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Title: Ice cloud formation potential by free tropospheric particles from long-range transport over the Northern Atlantic Ocean

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