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Title: Two decades of laccases: Advancing sustainability in the chemical industry

Abstract

Given the current state of environmental affairs and that our future on this planet as we know it is in jeopardy, research and development into greener and more sustainable technologies within the chemical and forest products industries is at its peak. Given the global scale of these industries, the need for environmentally benign practices is propelling new green processes. These challenges are also impacting academic research and our reagents of interest are laccases. These enzymes are employed in a variety of biotechnological applications due to their native function as catalytic oxidants. They are about as green as it gets when it comes to chemical processes, requiring O 2 as their only co-substrate and producing H 2O as the sole by-product. Furthermore, the following account will review our twenty year journey on the use of these enzymes within our research group, from their initial use in biobleaching of kraft pulps and for fiber modification within the pulp and paper industry, to their current application as green catalytic oxidants in the field of synthetic organic chemistry.

Authors:
 [1];  [2]
  1. Georgia Inst. of Technology, Atlanta, GA (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  2. Georgia Inst. of Technology, Atlanta, GA (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Univ. of Tennessee, Knoxville, TN (United States)
Publication Date:
Research Org.:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Joint Institute for Biological Sciences (JIBS); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Biological and Environmental Research (BER) (SC-23)
OSTI Identifier:
1376597
Grant/Contract Number:
AC05-00OR22725
Resource Type:
Journal Article: Accepted Manuscript
Journal Name:
Chemical Record
Additional Journal Information:
Journal Name: Chemical Record; Journal ID: ISSN 1527-8999
Publisher:
Wiley
Country of Publication:
United States
Language:
English
Subject:
54 ENVIRONMENTAL SCIENCES; 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; biotechnology; green chemistry; laccases; organic synthesis; sustainability

Citation Formats

Cannatelli, Mark D., and Ragauskas, Arthur J.. Two decades of laccases: Advancing sustainability in the chemical industry. United States: N. p., 2016. Web. doi:10.1002/tcr.201600033.
Cannatelli, Mark D., & Ragauskas, Arthur J.. Two decades of laccases: Advancing sustainability in the chemical industry. United States. doi:10.1002/tcr.201600033.
Cannatelli, Mark D., and Ragauskas, Arthur J.. 2016. "Two decades of laccases: Advancing sustainability in the chemical industry". United States. doi:10.1002/tcr.201600033. https://www.osti.gov/servlets/purl/1376597.
@article{osti_1376597,
title = {Two decades of laccases: Advancing sustainability in the chemical industry},
author = {Cannatelli, Mark D. and Ragauskas, Arthur J.},
abstractNote = {Given the current state of environmental affairs and that our future on this planet as we know it is in jeopardy, research and development into greener and more sustainable technologies within the chemical and forest products industries is at its peak. Given the global scale of these industries, the need for environmentally benign practices is propelling new green processes. These challenges are also impacting academic research and our reagents of interest are laccases. These enzymes are employed in a variety of biotechnological applications due to their native function as catalytic oxidants. They are about as green as it gets when it comes to chemical processes, requiring O2 as their only co-substrate and producing H2O as the sole by-product. Furthermore, the following account will review our twenty year journey on the use of these enzymes within our research group, from their initial use in biobleaching of kraft pulps and for fiber modification within the pulp and paper industry, to their current application as green catalytic oxidants in the field of synthetic organic chemistry.},
doi = {10.1002/tcr.201600033},
journal = {Chemical Record},
number = ,
volume = ,
place = {United States},
year = 2016,
month = 7
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

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