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Title: Advances in electrode materials for Li-based rechargeable batteries

Abstract

Rechargeable lithium-ion batteries store energy as chemical energy in electrode materials during charge and can convert the chemical energy into electrical energy when needed. Tremendous attention has been paid to screen electroactive materials, to evaluate their structural integrity and cycling reversibility, and to improve the performance of electrode materials. This review discusses recent advances in performance enhancement of both anode and cathode through nanoengineering active materials and applying surface coatings, in order to effectively deal with the challenges such as large volume variation, instable interface, limited cyclability and rate capability. We also introduce and discuss briefly the diversity and new tendencies in finding alternative lithium storage materials, safe operation enabled in aqueous electrolytes, and configuring novel symmetric electrodes and lithium-based flow batteries.

Authors:
 [1]; ORCiD logo [2]; ORCiD logo [3]; ORCiD logo [4]
  1. China Academy of Space Technology (CAST), Beijing (China)
  2. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  3. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Univ. of Tennessee, Knoxville, TN (United States)
  4. Korea Inst. of Science and Technology (KIST), Saarbrucken (Germany); Saarland Univ., Saarbrucken (Germany)
Publication Date:
Research Org.:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Org.:
USDOE Office of Energy Efficiency and Renewable Energy (EERE), Vehicle Technologies Office (EE-3V)
OSTI Identifier:
1376513
DOE Contract Number:  
AC05-00OR22725
Resource Type:
Journal Article
Journal Name:
RSC Advances
Additional Journal Information:
Journal Volume: 7; Journal Issue: 54; Journal ID: ISSN 2046-2069
Publisher:
Royal Society of Chemistry
Country of Publication:
United States
Language:
English
Subject:
25 ENERGY STORAGE

Citation Formats

Zhang, Hui, Mao, Chengyu, Li, Jianlin, and Chen, Ruiyong. Advances in electrode materials for Li-based rechargeable batteries. United States: N. p., 2017. Web. doi:10.1039/c7ra04370h.
Zhang, Hui, Mao, Chengyu, Li, Jianlin, & Chen, Ruiyong. Advances in electrode materials for Li-based rechargeable batteries. United States. doi:10.1039/c7ra04370h.
Zhang, Hui, Mao, Chengyu, Li, Jianlin, and Chen, Ruiyong. Wed . "Advances in electrode materials for Li-based rechargeable batteries". United States. doi:10.1039/c7ra04370h. https://www.osti.gov/servlets/purl/1376513.
@article{osti_1376513,
title = {Advances in electrode materials for Li-based rechargeable batteries},
author = {Zhang, Hui and Mao, Chengyu and Li, Jianlin and Chen, Ruiyong},
abstractNote = {Rechargeable lithium-ion batteries store energy as chemical energy in electrode materials during charge and can convert the chemical energy into electrical energy when needed. Tremendous attention has been paid to screen electroactive materials, to evaluate their structural integrity and cycling reversibility, and to improve the performance of electrode materials. This review discusses recent advances in performance enhancement of both anode and cathode through nanoengineering active materials and applying surface coatings, in order to effectively deal with the challenges such as large volume variation, instable interface, limited cyclability and rate capability. We also introduce and discuss briefly the diversity and new tendencies in finding alternative lithium storage materials, safe operation enabled in aqueous electrolytes, and configuring novel symmetric electrodes and lithium-based flow batteries.},
doi = {10.1039/c7ra04370h},
journal = {RSC Advances},
issn = {2046-2069},
number = 54,
volume = 7,
place = {United States},
year = {2017},
month = {7}
}

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